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Register a new userThe Dynamics of Ions on Phased Radio-frequency Carpets in High Pressure Gases and Application for Barium Tagging in Xenon Gas Time Projection Chambers
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Radio-frequency carpets with ultra-fine pitches are examined for ion transport in gases at atmospheric pressures and above. We develop new analytic and computational methods for modeling ion behavior on phased radio-frequency (RF) carpets in gas densities where ion dynamics are strongly influenced by buffer gas collisions. The analytic theory of phased RF arrays is obtained by generalizing the conventional Dehmelt potential treatment, and the emergence of levitating and sweeping forces from a single RF wave is demonstrated. We consider the effects of finite electrode width and demonstrate the existence of a surface of no return at around 0.25 times the carpet pitch. We then apply thermodynamic and kinetic theory arguments to calculate ion loss rates from RF carpets in the presence of stochastic effects from ion-neutral collisions. Comparison to collision-by-collision simulations in SIMION validate this new and efficient approach to calculation of transport efficiencies. We establish the dependence of transport properties on array phasing, and explore a parameter space that is of special interest to neutrinoless double beta decay experiments using xenon gas: RF transport of barium ions in xenon gas at pressures from 1 to 10 bar, which could represent a promising technique for barium daughter ion tagging. We explore the allowed parameter space for efficient transport, accounting for the detailed microphysics of molecular ion formation and pressure dependent mobility, as well as finite temperature effects for both room temperature and cooled gases. The requirements of such systems lie significantly beyond those of existing devices in terms of both voltage and electrode pitch, and we discuss the challenges associated with achieving these operating conditions with presently available or near-future technologies.
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We present an update on the development of techniques to adapt Single Molecule Fluorescent Imaging for the tagging of individual barium ions in high pressure xenon gas detectors, with the goal of realizing a background-free neutrinoless double beta decay technology. Previously reported progress is reviewed, including the recent demonstration of single barium dication sensitivity using SMFI. We then describe two important advances: 1) the development of a new class of custom barium sensing fluorescent dyes, which exhibit a significantly stronger response to barium than commercial calcium sensing compounds in aqueous solution; 2) the first demonstration of a dry-phase chemosensor for barium ions. This proceeding documents work presented at the 9th Symposium on Large TPCs for Rare Event Detection in Paris, France.
Dielectric breakdown strength is one of the critical performance metrics for gases and mixtures used in large, high pressure gas time projection chambers. In this paper we experimentally study dielectric breakdown strengths of several important time projection chamber working gases and gas-phase insulators over the pressure range 100 mbar to 10 bar, and gap sizes ranging from 0.1to 10 mm. Gases characterized include argon, xenon, CO2, CF4, and mixtures 90-10 argon-CH4,90-10 argon-CO2and 99-1 argon-CF4. We develop a theoretical model for high voltage breakdown based on microphysical simulations that use PyBoltz electron swarm Monte Carlo results as input to Townsend- and Meek-like discharge criteria. This model is shown to be highly predictive at high pressure, out-performing traditional Paschen-Townsend and Meek-Raether models significantly. At lower pressure-times-distance, the Townsend-like model is an excellent description for noble gases whereas the Meek-like model provides a highly accurate prediction for insulating gases.
The search for neutrinoless double beta decay probes the fundamental properties of neutrinos, including whether or not the neutrino and antineutrino are distinct. Double beta detectors are large and expensive, so background reduction is essential for extracting the highest sensitivity. The identification, or tagging, of the $^{136}$Ba daughter atom from double beta decay of $^{136}$Xe provides a technique for eliminating backgrounds in the nEXO neutrinoless double beta decay experiment. The tagging scheme studied in this work utilizes a cryogenic probe to trap the barium atom in solid xenon, where the barium atom is tagged via fluorescence imaging in the solid xenon matrix. Here we demonstrate imaging and counting of individual atoms of barium in solid xenon by scanning a focused laser across a solid xenon matrix deposited on a sapphire window. When the laser sits on an individual atom, the fluorescence persists for $sim$30~s before dropping abruptly to the background level, a clear confirmation of one-atom imaging. No barium fluorescence persists following evaporation of a barium deposit to a limit of $leq$0.16%. This is the first time that single atoms have been imaged in solid noble element. It establishes the basic principle of a barium tagging technique for nEXO.
Motivated by the possibility of guiding daughter ions from double beta decay events to single-ion sensors for barium tagging, the NEXT collaboration is developing a program of R&D to test radio frequency (RF) carpets for ion transport in high pressure xenon gas. This would require carpet functionality in regimes at higher pressures than have been previously reported, implying correspondingly larger electrode voltages than in existing systems. This mode of operation appears plausible for contemporary RF-carpet geometries due to the higher predicted breakdown strength of high pressure xenon relative to low pressure helium, the working medium in most existing RF carpet devices. In this paper we present the first measurements of the high voltage dielectric strength of xenon gas at high pressure and at the relevant RF frequencies for ion transport (in the 10 MHz range), as well as new DC and RF measurements of the dielectric strengths of high pressure argon and helium gases at small gap sizes. We find breakdown voltages that are compatible with stable RF carpet operation given the gas, pressure, voltage, materials and geometry of interest.
High pressure gas time projection chambers (HPGTPCs) are made with a variety of materials, many of which have not been well characterized in high pressure noble gas environments. As HPGTPCs are scaled up in size toward ton-scale detectors, assemblies become larger and more complex, creating a need for detailed understanding of how structural supports and high voltage insulators behave. This includes the identification of materials with predictable mechanical properties and without surface charge accumulation that may lead to field deformation or sparking. This paper explores the mechanical and electrical effects of high pressure gas environments on insulating polymers PTFE, HDPE, PEEK, POM and UHMW in Argon and Xenon, including studying absorption, swelling and high voltage insulation strength.
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