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Reliability of spin-to-charge conversion measurements in graphene-based lateral spin valves

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 Added by Felix Casanova
 Publication date 2021
  fields Physics
and research's language is English




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Understanding spin physics in graphene is crucial for developing future two-dimensional spintronic devices. Recent studies show that efficient spin-to-charge



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We employ the spin absorption technique in lateral spin valves to extract the spin diffusion length of Permalloy (Py) as a function of temperature and resistivity. A linear dependence of the spin diffusion length with conductivity of Py is observed, evidencing that Elliott-Yafet is the dominant spin relaxation mechanism in Permalloy. Completing the data set with additional data found in literature, we obtain $lambda_{Py}= (0.91pm 0.04) (fOmega m^2)/rho_{Py}$.
The spin injection and accumulation in metallic lateral spin valves with transparent interfaces is studied using d.c. injection current. Unlike a.c.-based techniques, this allows investigating the effects of the direction and magnitude of the injected current. We find that the spin accumulation is reversed by changing the direction of the injected current, whereas its magnitude does not change. The injection mechanism for both current directions is thus perfectly symmetric, leading to the same spin injection efficiency for both spin types. This result is accounted for by a spin-dependent diffusion model. Joule heating increases considerably the local temperature in the spin valves when high current densities are injected ($sim$80--105 K for 1--2$times10^{7}$A cm$^{-2}$), strongly affecting the spin accumulation.
A high reproducibility in the performance of cobalt/copper and permalloy/copper lateral spin valves with transparent contacts is obtained by optimizing the interface quality and the purity of copper. This allows us to study comprehensively the spin injection properties of both ferromagnetic materials, as well as the spin transport properties of copper, which are not affected by the used ferromagnetic material, leading to long spin diffusion lengths. Spin polarizations of permalloy and cobalt are obtained as a function of temperature. Analysis of the temperature dependence of both the spin polarization and conductivity of permalloy using the standard two-channel model for ferromagnetic metals suggests that a correction factor of ~2 is needed for the spin polarization values obtained by lateral spin valve experiments.
The role of the growth conditions in the spin transport properties of silver (Ag) have been studied by using lateral spin valve structures. By changing the deposition conditions of Ag from polycrystalline to epitaxial growth, we have observed a considerable enhancement of the spin diffusion length, from $lambda_{Ag}$ = 449 $pm$ 30 to 823 $pm$ 59 nm. This study shows that diminishing the grain boundary contribution to the spin relaxation mechanism is an effective way to improve the spin diffusion length in metallic nanostructures.
We have succeeded in fully describing dynamic properties of spin current including the different spin absorption mechanism for longitudinal and transverse spins in lateral spin valves, which enables to elucidate intrinsic spin transport and relaxation mechanism in the nonmagnet. The deduced spin lifetimes are found independent of the contact type. From the transit-time distribution of spin current extracted from the Fourier transform in Hanle measurement data, the velocity of the spin current in Ag with Py/Ag Ohmic contact turns out much faster than that expected from the widely used model.
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