We demonstrate theoretically that the thermal Hall effect of magnons in collinear antiferromagnetic insulators is an indicator of magnetic and topological phase transitions in the magnon spectrum. The transversal heat current of magnons caused by a thermal gradient is calculated for an antiferromagnet on a honeycomb lattice. An applied magnetic field drives the system from the antiferromagnetic phase via a spin-flop phase into the field-polarized phase. Besides these magnetic phase transitions we find topological phase transitions within the spin-flop phase. Both types of transitions manifest themselves in prominent and distinguishing features in the thermal conductivities; depending on the temperature, the conductivity changes by several orders of magnitude, providing a tool to discern experimentally the two types of phase transitions. We include numerical results for the van der Waals magnet MnPS$_3$.
The anomalous Hall effect (AHE), a Hall signal occurring without an external magnetic field, is one of the most significant phenomena. However, understanding the AHE mechanism has been challenging and largely restricted to ferromagnetic metals. Here, we investigate the recently discovered AHE in the chiral antiferromagnet Mn3Sn by measuring a thermal analog of the AHE, known as an anomalous thermal Hall effect (ATHE). The amplitude of the ATHE scales with the anomalous Hall conductivity of Mn3Sn over a wide temperature range, demonstrating that the AHE of Mn3Sn arises from a dissipationless intrinsic mechanism associated with the Berry curvature. Moreover, we find that the dissipationless AHE is significantly stabilized by shifting the Fermi level toward the magnetic Weyl points. Thus, in Mn3Sn, the Berry curvature emerging from the proposed magnetic Weyl fermion state is a key factor for the observed AHE and ATHE.
We consider nonlinear magnon interactions in collinear antiferromagnetic (AF) insulators at finite temperatures. In AF systems with biaxial magnetocrystalline anisotropy, we implement a self-consistent Hartree-Fock mean-field approximation to explore the nonlinear interactions. The resulting nonlinear magnon interactions separate into two-magnon intra- and interband scattering processes. Furthermore, we compute the temperature dependence of the magnon spectrum due to nonlinear magnon interactions for square and hexagonal lattices. Measurements of the predicted AF resonance at different temperatures can probe nonlinear interactions close to the magnetic phase transitions. Our findings establish a framework for exploring magnonic phenomena where interactions are essential, e.g., magnon transport and Bose-Einstein condensation of magnons.
Recent small angle neutron scattering suggests, that the spin structure in the A-phase of MnSi is a so-called triple-$Q$ state, i.e., a superposition of three helices under 120 degrees. Model calculations suggest that this structure in fact is a lattice of so-called skyrmions, i.e., a lattice of topologically stable knots in the spin structure. We report a distinct additional contribution to the Hall effect in the temperature and magnetic field range of the proposed skyrmion lattice, where such a contribution is neither seen nor expected for a normal helical state. Our Hall effect measurements constitute a direct observation of a topologically quantized Berry phase that identifies the spin structure seen in neutron scattering as the proposed skyrmion lattice.
We propose that non-collinear magnetic order in quantum magnets can harbor a novel higher-order topological magnon phase with non-Hermitian topology and hinge magnon modes. We consider a three-dimensional system of interacting local moments on stacked-layers of honeycomb lattice. It initially favors a collinear magnetic order along an in-plane direction, which turns into a non-collinear order upon applying an external magnetic field perpendicular to the easy axis. We exploit the non-Hermitian nature of the magnon Hamiltonian to show that this field-induced transition corresponds to the transformation from a topological magnon insulator to a higher-order topological magnon state with a one-dimensional hinge mode. As a concrete example, we discuss the recently-discovered monoclinic phase of the thin chromium trihalides, which we propose as the first promising material candidate of the higher-order topological magnon phase.
Motivated by the discovery of the quantum anomalous Hall effect in Cr-doped ce{(Bi,Sb)2Te3} thin films, we study the generic states for magnetic topological insulators and explore the physical properties for both magnetism and itinerant electrons. First-principles calculations are exploited to investigate the magnetic interactions between magnetic Co atoms adsorbed on the ce{Bi2Se3} (111) surface. Due to the absence of inversion symmetry on the surface, there are Dzyaloshinskii-Moriya-like twisted spin interactions between the local moments of Co ions. These nonferromagnetic interactions twist the collinear spin configuration of the ferromagnet and generate various magnetic orders beyond a simple ferromagnet. Among them, the spin spiral state generates alternating counterpropagating modes across each period of spin states, and the skyrmion lattice even supports a chiral mode around the core of each skyrmion. The skyrmion lattice opens a gap at the surface Dirac point, resulting in the anomalous Hall effect. These results may inspire further experimental investigation of magnetic topological insulators.
Robin R. Neumann
,Alexander Mook
,Jurgen Henk
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(2021)
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"Thermal Hall effect of magnons in collinear antiferromagnetic insulators: signatures of magnetic and topological phase transitions"
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Robin Richard Neumann
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