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Register a new userMulti-window SRS imaging using a rapid widely tunable fiber laser
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Spectroscopic stimulated Raman scattering (SRS) imaging has become a useful tool finding a broad range of applications. Yet, wider adoption is hindered by the bulky and environmentally-sensitive solid-state optical parametric oscillator (OPO) in current SRS microscope. Moreover, chemically-informative multi-window SRS imaging across C-H, C-D and fingerprint Raman regions is challenging due to the slow wavelength tuning speed of the solid-state OPO. In this work, we present a multi-window SRS imaging system based on a compact and robust fiber laser with rapid and widely tuning capability. To address the relative intensity noise intrinsic to fiber laser, we implemented auto-balanced detection which enhances the signal-to-noise ratio of stimulated Raman loss imaging by 23 times. We demonstrate high-quality SRS metabolic imaging of fungi, cancer cells, and Caenorhabditis elegans across the C-H, C-D and fingerprint Raman windows. Our re-sults showcase the potential of the compact multi-window SRS system for a broad range of applications.
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Pulse generation often requires a stabilized cavity and its corresponding mode structure for initial phase-locking. Contrastingly, modeless cavity-free random lasers provide new possibilities for high quantum efficiency lasing that could potentially be widely tunable spectrally and temporally. Pulse generation in random lasers, however, has remained elusive since the discovery of modeless gain lasing. Here we report coherent pulse generation with modeless random lasers based on the unique polarization selectivity and broadband saturable absorption of monolayer graphene. Simultaneous temporal compression of cavity-free pulses are observed with such a polarization modulation, along with a broadly-tunable pulsewidth across two orders of magnitude down to 900 ps, a broadly-tunable repetition rate across three orders of magnitude up to 3 MHz, and a singly-polarized pulse train at 41 dB extinction ratio, about an order of magnitude larger than conventional pulsed fiber lasers. Moreover, our graphene-based pulse formation also demonstrates robust pulse-to-pulse stability and wide-wavelength operation due to the cavity-less feature. Such a graphene-based architecture not only provides a tunable pulsed random laser for fiber-optic sensing, speckle-free imaging, and laser-material processing, but also a new way for the non-random CW fiber lasers to generate widely tunable and singly-polarized pulses.
We report on the first experimental demonstration of widely-tunable parametric sideband generation in a Kerr microresonator. Specifically, by pumping a silica microsphere in the normal dispersion regime, we achieve the generation of phase-matched four-wave mixing sidebands at large frequency detunings from the pump. Thanks to the role of higher-order dispersion in enabling phase matching, small variations of the pump wavelength translate into very large and controllable changes in the wavelengths of the generated sidebands: we experimentally demonstrate over 720 nm of tunability using a low-power continuous-wave pump laser in the C-band. We also derive simple theoretical predictions for the phase-matched sideband frequencies, and discuss the predictions in light of the discrete cavity resonance frequencies. Our experimentally measured sideband wavelengths are in very good agreement with theoretical predictions obtained from our simple phase matching analysis.
We introduce a model for spatiotemporal modelocking in multimode fiber lasers, which is based on the (3+1)-dimensional cubic-quintic complex Ginzburg-Landau equation (cGLE) with conservative and dissipative nonlinearities and a 2-dimensional transverse trapping potential. Systematic numerical analysis reveals a variety of stable nonlinear modes, including stable fundamental solitons and breathers, as well as solitary vortices with winding number $n=1$, while vortices with $n=2$ are unstable, splitting into persistently rotating bound states of two unitary vortices. A characteristic feature of the system is bistability between the fundamental and vortex spatiotemporal solitons.
We investigate the effects of two dimensional confinement on the lasing properties of a classical random laser system operating in the incoherent feedback (diffusive) regime. A suspension of 250nm rutile (TiO2) particles in a Rhodamine 6G solution was inserted into the hollow core of a photonic crystal fiber (PCF) generating the first random fiber laser and a novel quasi-one-dimensional RL geometry. Comparison with similar systems in bulk format shows that the random fiber laser presents an efficiency that is at least two orders of magnitude higher.
Self-heterodyne fiber interferometers have been shown to be capable of stabilizing lasers to ultra-narrow linewidths and present an excellent alternative to high finesse cavities for frequency stabilization. In addition to suppressing frequency noise, these devices are highly tunable, and can be manipulated to produce high speed frequency sweeps over the entire range of the laser. We present an analytic approach for choosing a delay-line length for both optimal noise suppression and highest in-loop frequency sweep rate. Using this model we have implemented a fiber-based active Michelson interferometer as a frequency discriminator for a conventional diode laser and demonstrated a linewidth of 700 Hz over millisecond timescales. We also demonstrate a frequency scan rate of 1 THz/s and independently measure the maximum deviation in frequency from the linear sweep to be 100 kHz, predominantly limited by acoustic resonances in the apparatus.
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