Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userRoom-Temperature Anisotropic Plasma Mirror and Polarization-Controlled Optical Switch Based on Type-II Weyl Semimetal WP2
93
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
Anisotropy in electronic structures may ignite intriguing anisotropic optical responses, as has been well demonstrated in various systems including superconductors, semiconductors, and even topological Weyl semimetals. Meanwhile, it is well established in metal optics that the metal reflectance declines from one to zero when the photon frequency is above the plasma frequency {omega}p , behaving as a plasma mirror. However, the exploration of anisotropic plasma mirrors and corresponding applications remains elusive, especially at room temperature. Here, we discover a pronounced anisotropic plasma reflectance edge in the type-II Weyl semimetal WP2, with an anisotropy ratio of {omega}p up to 1.5. Such anisotropic plasma mirror behavior and its robustness against temperature promise optical device applications over a wide temperature range. For example, the high sensitivity of polarization-resolved plasma reflectance edge renders WP2 an inherent polarization detector. We further achieve a room-temperature WP2-based optical switch, effectively controlled by simply tuning the light polarization. These findings extend the frontiers of metal optics as a discipline and promise the design of multifunctional devices combining both topological and optical features.
rate research
Read More
Weyl semimetal emerges as a new topologically nontrivial phase of matter, hosting low-energy excitations of massless Weyl fermions. Here, we present a comprehensive study of the type-II Weyl semimetal WP2. Transport studies show a butterfly-like magnetoresistance at low temperature, reflecting the anisotropy of the electron Fermi surfaces. The four-lobed feature gradually evolves into a two-lobed one upon increasing temperature, mainly due to the reduced relative contribution of electron Fermi surfaces compared to hole Fermi surfaces for the magnetoresistance. Moreover, angle-dependent Berry phase is further discovered from the quantum oscillations, which is ascribed to the effective manipulation of the extremal Fermi orbits by the magnetic field to feel the nearby topological singularities in the momentum space. The revealed topological characters and anisotropic Fermi surfaces of WP2 substantially enrich the physical properties of Weyl semimetals and hold great promises in topological electronic and Fermitronic device applications.
Distinct to type-I Weyl semimetals (WSMs) that host quasiparticles described by the Weyl equation, the energy dispersion of quasiparticles in type-II WSMs violates Lorentz invariance and the Weyl cones in the momentum space are tilted. Since it was proposed that type-II Weyl fermions could emerge from (W,Mo)Te2 and (W,Mo)P2 families of materials, a large numbers of experiments have been dedicated to unveil the possible manifestation of type-II WSM, e.g. the surface-state Fermi arcs. However, the interpretations of the experimental results are very controversial. Here, using angle-resolved photoemission spectroscopy supported by the first-principles calculations, we probe the tilted Weyl cone bands in the bulk electronic structure of WP2 directly, which are at the origin of Fermi arcs at the surfaces and transport properties related to the chiral anomaly in type-II WSMs. Our results ascertain that due to the spin-orbit coupling the Weyl nodes originate from the splitting of 4-fold degenerate band-crossing points with Chern numbers C = $pm$2 induced by the crystal symmetries of WP2, which is unique among all the discovered WSMs. Our finding also provides a guiding line to observe the chiral anomaly which could manifest in novel transport properties.
Using Hall photovoltage measurements, we demonstrate that an anomalous Hall-voltage can be induced in few layer WTe2 under circularly polarized light illumination. By applying a bias voltage along different crystal axes, we find that the photo-induced anomalous Hall conductivity coincides with a particular crystal axis. Our results are consistent with the underlying Berry-curvature exhibiting a dipolar distribution due to the breaking of crystal inversion symmetry. Using a time-resolved optoelectronic auto-correlation spectroscopy, we find that the decay time of the anomalous Hall voltage exceeds the electron-phonon scattering time by orders of magnitude but is consistent with the comparatively long spin-lifetime of carriers in the momentum-indirect electron and hole pockets in WTe2. Our observation suggests, that a helical modulation of an otherwise isotropic spin-current is the underlying mechanism of the anomalous Hall effect.
TaIrTe$_4$ is an example of a candidate Weyl type-II semimetal with a minimal possible number of Weyl nodes. Four nodes are reported to exist a single plane in $k$-space. The existence of a conical dispersion linked to Weyl nodes has yet to be shown experimentally. Here we use optical spectroscopy as a probe of the band structure on a low-energy scale. Studying optical conductivity allows us to probe intraband and interband transitions with zero momentum. In TaIrTe$_4$, we observe a narrow Drude contribution and an interband conductivity that may be consistent with a tilted linear band dispersion up to 40~meV. The interband conductivity allows us to establish the effective parameters of the conical dispersion; effective velocity $v=1.1cdot 10^{4}$~m/s and tilt $gamma=0.37$. The transport data, Seebeck and Hall coefficients, are qualitatively consistent with conical features in the band structure. Quantitative disagreement may be linked to the multiband nature of TaIrTe$_4$.
The peculiar band structure of semimetals exhibiting Dirac and Weyl crossings can lead to spectacular electronic properties such as large mobilities accompanied by extremely high magnetoresistance. In particular, two closely neighbouring Weyl points of the same chirality are protected from annihilation by structural distortions or defects, thereby significantly reducing the scattering probability between them. Here we present the electronic properties of the transition metal diphosphides, WP2 and MoP2, that are type-II Weyl semimetals with robust Weyl points. We present transport and angle resolved photoemission spectroscopy measurements, and first principles calculations. Our single crystals of WP2 display an extremely low residual low-temperature resistivity of 3 nohm-cm accompanied by an enormous and highly anisotropic magnetoresistance above 200 million % at 63 T and 2.5 K. These properties are likely a consequence of the novel Weyl fermions expressed in this compound. We observe a large suppression of charge carrier backscattering in WP2 from transport measurements.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
