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High Phase-Space Density of Laser-Cooled Molecules in an Optical Lattice

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 Added by Shiqian Ding
 Publication date 2021
  fields Physics
and research's language is English




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We report laser cooling and trapping of yttrium monoxide (YO) molecules in an optical lattice. We show that gray molasses cooling remains exceptionally efficient for YO molecules inside the lattice with a molecule temperature as low as 6.1(6) $mu$K. This approach has produced a trapped sample of 1200 molecules, with a peak spatial density of $sim1.2times10^{10}$ cm$^{-3}$, and a peak phase-space density of $sim3.1times10^{-6}$. By adiabatically ramping down the lattice depth, we cool the molecules further to 1.0(2) $mu$K, twenty times colder than previously reported for laser-cooled molecules in a trap.



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124 - N. J. Fitch , M. R. Tarbutt 2021
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The study of ultracold molecules tightly trapped in an optical lattice can expand the frontier of precision measurement and spectroscopy, and provide a deeper insight into molecular and fundamental physics. Here we create, probe, and image microkelvin $^{88}$Sr$_2$ molecules in a lattice, and demonstrate precise measurements of molecular parameters as well as coherent control of molecular quantum states using optical fields. We discuss the sensitivity of the system to dimensional effects, a new bound-to-continuum spectroscopy technique for highly accurate binding energy measurements, and prospects for new physics with this rich experimental system.
We demonstrate coherent microwave control of the rotational, hyperfine and Zeeman states of ultracold CaF molecules, and the magnetic trapping of these molecules in a single, selectable quantum state. We trap about $5times 10^{3}$ molecules for 2 s at a temperature of 65(11) $mu$K and a density of $1.2 times 10^{5}$ cm$^{-3}$. We measure the state-specific loss rate due to collisions with background helium.
Barium monohydride (BaH) is an attractive candidate for extending laser cooling and trapping techniques to diatomic hydrides. The apparatus and high-resolution optical spectroscopy presented here demonstrate progress toward this goal. A cryogenic buffer-gas-cooled molecular beam of BaH was constructed and characterized. Pulsed laser ablation into cryogenic helium buffer gas delivers $sim1times10^{10}$ molecules/sr/pulse in the X$^2Sigma^+$ ($v=0,N=1$) state of primary interest. More than $1times10^7$ of these molecules per pulse enter the downstream science region with forward velocities below 100 m/s and transverse temperature of 0.1 K. This molecular beam enabled high-resolution optical spectra of BaH in quantum states relevant to laser slowing and cooling. The reported measurements include hyperfine structure and magnetic $g$ factors in the X$^2Sigma^+$, B$^2Sigma^+$, and A$^2Pi_{1/2}$ states.
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