No Arabic abstract
It is well known that energy-time entanglement can enhance two photon absorption (TPA) by simultaneously optimizing the two photon resonance and the coincidence rate of photons at the absorber. However, the precise relation between entanglement and the TPA rate depends on the coherences of intermediate states involved in the transition, making it a rather challenging task to identify universal features of TPA processes. In the present paper, we show that the theory can be simplified greatly by separating the two photon resonance from the temporal dynamics of the intermediate levels. The result is a description of the role of entanglement in the TPA process by a one-dimensional coherence in the Hilbert space defined by the arrival time difference of the two photons. Transformation into the frequency difference basis results in Kramers-Kronig relations for the TPA process, separating off-resonant contributions of virtual levels from resonant contributions. In particular, it can be shown that off-resonant contributions are insensitive to the frequencies of the associated virtual states, indicating that virtual-state spectroscopy of levels above the final two photon excited state is not possible.
Two-photon excited fluorescence (TPEF) is a standard technique in modern microscopy but still affected by photo-damage of the probe. It was proposed that TPEF can be enhanced by using entangled photons, but has proven to be challenging. Recently it was shown that some features of entangled photons can be mimicked with thermal light, which finds application in ghost imaging, sub-wavelength lithography and metrology. Here, we utilize true thermal light from a super-luminescence diode to demonstrate enhanced TPEF compared to coherent light using two common fluorophores and luminescent quantum dots. We find that the two-photon absorption rate is directly proportional to the measured degree of second-order coherence, as predicted by theory. Our results show that photon bunching can be exploited in two-photon microscopy with the photon statistic providing a new degree of freedom.
The phenomenon of entanglement is the basis of quantum information and quantum communication processes. Entangled systems with a large number of photons are of great interest at present because they provide a platform for streaming technologies based on photonics. In this paper we present a device which operates with four-photons and based on the Hong-Ou-Mandel (HOM) interference. The presented device allows to maximize the degree of spatial entanglement and generate the highly entangled four-dimensional Bell states. Furthermore, the use of the interferometer in different regimes leads to fast interference fringes in the coincidence probability with period of oscillations twice smaller than the pump wavelength. We have a good agreement between theoretical simulations and experimental results.
Quantum entanglement plays a vital role in many quantum information and communication tasks. Entangled states of higher dimensional systems are of great interest due to the extended possibilities they provide. For example, they allow the realisation of new types of quantum information schemes that can offer higher information-density coding and greater resilience to errors than can be achieved with entangled two-dimensional systems. Closing the detection loophole in Bell test experiments is also more experimentally feasible when higher dimensional entangled systems are used. We have measured previously untested correlations between two photons to experimentally demonstrate high-dimensional entangled states. We obtain violations of Bell-type inequalities generalised to d-dimensional systems with up to d = 12. Furthermore, the violations are strong enough to indicate genuine 11-dimensional entanglement. Our experiments use photons entangled in orbital angular momentum (OAM), generated through spontaneous parametric down-conversion (SPDC), and manipulated using computer controlled holograms.
When a low flux of time-frequency-entangled photon pairs (EPP) illuminates a two-photon transition, the rate of two-photon absorption (TPA) can be enhanced considerably by the quantum nature of photon number correlations and frequency correlations. We present a quantum-theoretic derivation of entangled TPA (ETPA) and calculate an upper bound on the amount of quantum enhancement that is possible in such systems. The derived bounds indicate that in order to observe ETPA the experiments would need to operate at a combination of significantly higher rates of EPP illumination, molecular concentrations, and conventional TPA cross sections than are achieved in typical experiments.
Topological insulators combine insulating properties in the bulk with scattering-free transport along edges, supporting dissipationless unidirectional energy and information flow even in the presence of defects and disorder. The feasibility of engineering quantum Hamiltonians with photonic tools, combined with the availability of entangled photons, raises the intriguing possibility of employing topologically protected entangled states in optical quantum computing and information processing. However, while two-photon states built as a product of two topologically protected single-photon states inherit full protection from their single-photon parents, high degree of non-separability may lead to rapid deterioration of the two-photon states after propagation through disorder. We identify physical mechanisms which contribute to the vulnerability of entangled states in topological photonic lattices and present clear guidelines for maximizing entanglement without sacrificing topological protection.