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High-speed hyperspectral four-wave-mixing microscopy with frequency combs

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 Added by Steven Cundiff
 Publication date 2021
  fields Physics
and research's language is English




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A four-wave-mixing, frequency-comb-based, hyperspectral imaging technique that is spectrally precise, potentially rapid, and can in principle be applied to any material, is demonstrated in a near-diffraction-limited microscopy application.

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We investigate the generation of optical frequency combs through a cascade of four-wave mixing processes in nonlinear fibres with optimised parameters. The initial optical field consists of two continuous-wave lasers with frequency separation larger than 40 GHz (312.7 pm at 1531 nm). It propagates through three nonlinear fibres. The first fibre serves to pulse shape the initial sinusoidal-square pulse, while a strong pulse compression down to sub-100 fs takes place in the second fibre which is an amplifying erbium-doped fibre. The last stage is a low-dispersion highly nonlinear fibre where the frequency comb bandwidth is increased and the line intensity is equalised. We model this system using the generalised nonlinear Schrodinger equation and investigate it in terms of fibre lengths, fibre dispersion, laser frequency separation and input powers with the aim to minimise the frequency comb noise. With the support of the numerical results, a frequency comb is experimentally generated, first in the near infra-red and then it is frequency-doubled into the visible spectral range. Using a MUSE-type spectrograph, we evaluate the comb performance for astronomical wavelength calibration in terms of equidistancy of the comb lines and their stability.
95 - Thibaut Sylvestre 2015
This work reports the experimental observation of a new type of four-wave mixing in which frequency-degenerate weak signal and idler waves are generated by mixing two pump waves of different frequencies in a normally dispersive birefringent optical fiber. This parametric frequency fusion is what we believed the first experimental evidence of inverse four-wave mixing.
Microresonator-based Kerr frequency comb (microcomb) generation can potentially revolutionize a variety of applications ranging from telecommunications to optical frequency synthesis. However, phase-locked microcombs have generally had low conversion efficiency limited to a few percent. Here we report experimental results that achieve ~30% conversion efficiency (~200 mW on-chip comb power excluding the pump) in the fiber telecommunication band with broadband mode-locked dark-pulse combs. We present a general analysis on the efficiency which is applicable to any phase-locked microcomb state. The effective coupling condition for the pump as well as the duty cycle of localized time-domain structures play a key role in determining the conversion efficiency. Our observation of high efficiency comb states is relevant for applications such as optical communications which require high power per comb line.
Stimulated Brillouin scattering (SBS) and Kerr-nonlinear four wave-mixing (FWM) are among the most important and widely studied nonlinear effects in optical fibres. At high powers SBS can be cascaded producing multiple Stokes waves spaced by the Brillouin frequency shift. Here, we investigate the complex nonlinear interaction of the cascade of Stokes waves, generated in a Fabry-Perot chalcogenide fibre resonator through the combined action of SBS and FWM. We demonstrate the existence of parameter regimes, in which pump and Stokes waves attain a phase-locked steady state. Real-time measurements of 40ps pulses with 8GHz repetition rate are presented, confirming short-and long-term stability. Numerical simulations qualitatively agree with experiments and show the significance of FWM in phase-locking of pump and Stokes waves. Our findings can be applied for the design of novel picosecond pulse sources with GHz repetition rate for optical communication systems.
We suggest a scheme to manipulate paraxial diffraction by utilizing the dependency of a four-wave mixing process on the relative angle between the light fields. A microscopic model for four-wave mixing in a Lambda-type level structure is introduced and compared to recent experimental data. We show that images with feature size as low as 10 micrometers can propagate with very little or even negative diffraction. The mechanism is completely different from that conserving the shape of spatial solitons in nonlinear media, as here diffraction is suppressed for arbitrary spatial profiles. At the same time, the gain inherent to the nonlinear process prevents loss and allows for operating at high optical depths. Our scheme does not rely on atomic motion and is thus applicable to both gaseous and solid media.
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