Do you want to publish a course? Click here

Towards Single Atom Computing via High Harmonic Generation

142   0   0.0 ( 0 )
 Added by Gerard McCaul
 Publication date 2021
  fields Physics
and research's language is English




Ask ChatGPT about the research

The development of alternative platforms for computing has been a longstanding goal for physics, and represents a particularly pressing concern as conventional transistors approach the limit of miniaturization. A potential alternatice paradigm is that of reservoir computing, which leverages unknown, but highly non-linear transformations of input-data to perform computations. This has the advantage that many physical systems exhibit precisely the type of non-linear input-output relationships necessary for them to function as reservoirs. Consequently, the quantum effects which obstruct the further development of silicon electronics become an advantage for a reservoir computer. Here we demonstrate that even the most basic constituents of matter - atoms - can act as a reservoir for optical computers, thanks to the phenomenon of High Harmonic Generation (HHG). A prototype single-atom computer for classification problems is proposed, where parameters of the classification model are mapped to optical elements. We numerically demonstrate that this `all-optical computer can successfully classify data with an accuracy that is strongly dependent on dynamical non-linearities. This may pave the way for the development of petahertz information processing platforms.



rate research

Read More

We present an experimental study on the photoionization dynamics of non-resonant one-color two-photon single valence ionization of neutral argon atoms. Using 9.3 eV photons produced via high harmonic generation and a 3-D momentum imaging spectrometer, we detect the photoelectrons and ions produced from non-resonant two-photon ionization in coincidence. Photoionization from the $3p$ orbital produces a photoelectron scattering wave function with $p$ and $f$ partial wave components, which interfere and result in a photoelectron angular distribution with peak amplitude perpendicular to the VUV polarization. The comparison between the present results and two previous sets of theoretical calculations [Pan, C. & Starace, A. F. (1991). $textit{Physical Review A}$, 44(1), 324., and Moccia, R., Rahman, N. K., & Rizzo, A. (1983). $textit{Journal of Physics B: Atomic and Molecular Physics}$, 16(15), 2737.] indicates that electron-electron correlation contributes appreciably to the two-photon ionization dynamics.
VUV radiation around 159 nm is obtained toward direct excitation of a single trapped $^{115}$In$^{+}$ ion. An efficient fluoride-based VUV output-coupler is employed for intracavity high-harmonic generation of a Ti:S oscillator. Using this coupler, where we measured its reflectance to be about 90%, an average power reaching $6.4,mu$W is coupled out from a modest fundamental power of 650 mW. When a single comb component out of $1.9times10^{5}$ teeth is resonant to the atomic transition, hundreds of fluorescence photons per second will be detectable under a realistic condition.
We show that the dependence of high-order harmonic generation (HHG) on the molecular orientation can be understood within a theoretical treatment that does not involve the strong field of the laser. The results for H_2 show excellent agreement with time-dependent strong field calculations for model molecules, and this motivates a prediction for the orientation dependence of HHG from the N_2 3s_g valence orbital. For both molecules, we find that the polarization of recombination photons is influenced by the molecular orientation. The variations are particularly pronounced for the N_2 valence orbital, which can be explained by the presence of atomic p-orbitals.
High-order harmonic generation by few-cycle 800 nm laser pulses in neon gas in the presence of a strong terahertz (THz) field is investigated numerically with propagation effects taken into account. Our calculations show that the combination of THz fields with up to 12 fs laser pulses can be an effective gating technique to generate single attosecond pulses. We show that in the presence of the strong THz field only a single attosecond burst can be phase matched, whereas radiation emitted during other half-cycles disappears during propagation. The cutoff is extended and a wide supercontinuum appears in the near-field spectra, extending the available spectral width for isolated attosecond pulse generation from 23 to 93 eV. We demonstrate that phase matching effects are responsible for the generation of isolated attosecond pulses, even in conditions when single atom response yields an attosecond pulse train.
We produce oriented rotational wave packets in CO and measure their characteristics via high harmonic generation. The wavepacket is created using an intense, femtosecond laser pulse and its second harmonic. A delayed 800 nm pulse probes the wave packet, generating even-order high harmonics that arise from the broken symmetry induced by the orientation dynamics. The even-order harmonic radiation that we measure appears on a zero background, enabling us to accurately follow the temporal evolution of the wave packet. Our measurements reveal that, for the conditions optimum for harmonic generation, the orientation is produced by preferential ionization which depletes the sample of molecules of one orientation.
comments
Fetching comments Fetching comments
Sign in to be able to follow your search criteria
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا