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Structure in the Event-by-Event Energy-Dependent Neutron-Gamma Multiplicity Correlations in $^{252}text{Cf}$(sf)

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 Added by Stefano Marin
 Publication date 2021
  fields
and research's language is English




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The emission of neutrons and gamma rays by fission fragments reveal important information about the properties of fragments immediately following scission. The initial fragment properties, correlations between fragments, and emission competition give rise to correlations in neutron-gamma emission. Neutron-gamma correlations are important in nonproliferation applications because the characterization of fissionable samples relies on the identification of signatures in the measured radiation. Furthermore, recent theoretical and experimental advances have proposed to explain the mechanism of angular momentum generation in fission. In this paper, we present a novel analysis method of neutrons and gamma rays emitted by fission fragments that allows us to discern structure in the observed correlations. We have analyzed data collected on ce{^{252}Cf}(sf) at the Chi-Nu array at the Los Alamos Neutron Science Center. Through our analysis of the energy-differential neutron-gamma multiplicity covariance, we have observed enhanced neutron-gamma correlations, corresponding to rotational band gamma-ray transitions, at gamma-ray energies of $0.7$ and $1.2$ MeV. To shed light on the origin of this structure, we compare the experimental data with the predictions of three model calculations. The origin of the observed correlation structure is understood in terms of a positive spin-energy correlation in the generation of angular momentum in fission.



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126 - R. Capote , D. Neudecker 2019
Small uncertainties obtained for the Neutron Standards have been associated with possible missing correlations in the input data, with an incomplete uncertainty budget of the employed experimental database or with unrecognized uncertainty sources common to many measurements. While further detailed studies may improve the first two issues, the issue of potential unrecognized uncertainties and correlations between different experiments has long been neglected. We address this gap with a test-case study ons the evaluation of the total neutron multiplicity of the $^{252}$Cf(sf) source, which is included in the evaluation of the Thermal Neutron Constants within the Neutron Standards.
Background: Spontaneous fission events emit prompt neutrons correlated with one another in emission angle and energy. Purpose: We explore the relationship in energy and angle between correlated prompt neutrons emitted from 252Cf spontaneous fission. Methods: Measurements with the Chi-Nu array provide experimental data for coincident neutrons tagged with a fission chamber signal with 10 degree angular resolution and 1 ns timing resolution for time-of-flight energy calculations. The experimental results are compared to simulations produced by the fission event generators CGMF, FREYA, and MCNPX-POLIMI IPOL(1)=1. Results: We find that the measurements and the simulations all exhibit anisotropic neutron emission, though differences exist between fission event generators. Conclusions: This work shows that the dependence of detected neutron energy on the energy of a neutron detected in coincidence, although weak, is non-negligible, indicating that there may be correlations in energy between two neutrons emitted in the same fission event.
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