We investigate the role of domain walls in the ultrafast magnon dynamics of an antiferromagnetic NiO single crystal in a pump-probe experiment with variable pump photon energy. Analysing the amplitude of the energy-dependent photo-induced ultrafast spin dynamics, we detect a yet unreported coupling between the materials characteristic THz- and a GHz-magnon modes. We explain this unexpected coupling between two orthogonal eigenstates of the corresponding Hamiltonian by modelling the magneto-elastic interaction between spins in different domains. We find that such interaction, in the non-linear regime, couples the two different magnon modes via the domain walls and it can be optically exploited via the exciton-magnon resonance.
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