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Register a new userElectric-field-dependent $g$ factor for the ground state of lead monofluoride, PbF
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The electric-field-dependent $g$ factor and the electron electric dipole moment (eEDM)-induced Stark splittings for the lowest rotational levels of $^{207,208}$PbF are calculated. Observed and calculated Zeeman shifts for $^{207}$PbF are found to be in very good agreement. It is shown that the $^{207}$PbF hyperfine sublevels provide a promising system for the eEDM search and related experiments.
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We report the results of our theoretical study and analysis of earlier experimental data for the g-factor tensor components of the ground $^2Pi_{1/2}$ state of free PbF radical. The values obtained both within the relativistic coupled-cluster method combined with the generalized relativistic effective core potential approach and with our fit of the experimental data from [R.J. Mawhorter, B.S. Murphy, A.L. Baum, T.J. Sears, T. Yang, P.M. Rupasinghe, C.P. McRaven, N.E. Shafer-Ray, L.D. Alphei, J.-U. Grabow, Phys. Rev. A 84, 022508 (2011); A. Baum, B.S. thesis, Pomona College, 2011]. The obtained results agree very well with each other but contradict the previous fit performed in the cited works. Our final prediction for g-factors is $G_{parallel}= 0.081(5)$, $G_{perp}=-0.27(1)$.
We here report on the realization of an electrodynamic trap, capable of trapping neutral atoms and molecules in both low-field and high-field seeking states. Confinement in three dimensions is achieved by switching between two electric field configurations that have a saddle-point at the center of the trap, i.e., by alternating a focusing and a defocusing force in each direction. AC trapping of 15ND3 molecules is experimentally demonstrated, and the stability of the trap is studied as a function of the switching frequency. A 1 mK sample of 15ND3 molecules in the high-field seeking component of the |J,K>=|1,1> level, the ground-state of para-ammonia, is trapped in a volume of about 1 mm^3.
The X$^{1}Sigma ^{+}$ state of NaRb was studied by Fourier transform spectroscopy. An accurate potential energy curve was derived from more than 8800 transitions in isotopomers $^{23}$Na$^{85}$Rb and $^{23}$Na$^{87}$Rb. This potential reproduces the experimental observations within their uncertainties of 0.003 rcm to 0.007 rcm. The outer classical turning point of the last observed energy level ($v=76$, $J=27$) lies at $approx 12.4$ AA, leading to a energy of 4.5 rcm below the ground state asymptote.
We report the first results of ab initio relativistic correlation calculation of the effective electric field on the electron, E_eff, in the ground state of the HI$^+$ cation. This value is required for interpretation of the suggested experiment on search for the electron electric dipole moment. The generalized relativistic effective core potential, Fock-space relativistic coupled cluster with single and double cluster amplitudes and spin-orbit direct configuration interaction methods are used, followed by nonvariational one-center restoration of the four-component wavefunction in the iodine core. The calculated value of E_eff by the coupled cluster method is E_eff=0.345times 10^{24}Hz/e*cm. Configuration interaction study gives E_eff=0.336times 10^{24}Hz/e*cm (our final value). The structure of chemical bonding and contributions to E_eff in HI$^+$ is clarified and significant deviation of our value from that obtained in Ravaine etal Phys.Rev.Lett., 94, 013001 (2005) is explained.
A method is proposed to determine the $M1$ nuclear transition amplitude and hence the lifetime of the nuclear clock transition between the low-lying ($sim 8$ eV) first isomeric state and the ground state of $^{229}$Th from a measurement of the ground-state $g$ factor of few-electron $^{229}$Th ions. As a tool, the effect of nuclear hyperfine mixing (NHM) in highly charged $^{229}$Th-ions such as $^{229}$Th$^{89+}$ or $^{229}$Th$^{87+}$ is utilized. The ground-state-only $g$-factor measurement would also provide first experimental evidence of NHM in atomic ions. Combining the measurements for H-, Li-, and B-like $^{229}$Th ions has a potential to improve the initial result for a single charge state and to determine the nuclear magnetic moment to a higher accuracy than that of the currently accepted value. The calculations include relativistic, interelectronic-interaction, QED, and nuclear effects.
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