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Register a new userEfficient self-compression of ultrashort UV pulses in air-filled hollow-core photonic crystal fiber
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We report generation of ultrashort UV pulses by soliton self-compression in kagome-style hollow-core photonic crystal fiber filled with ambient air. Pump pulses with energy 2.6 uJ and duration 54 fs at 400 nm were compressed temporally by a factor of 5, to a duration of ~11 fs. The experimental results are supported by numerical simulations, showing that both Raman and Kerr effects play a role in the compression dynamics. The convenience of using ambient air, and the absence of glass windows that would distort the compressed pulses, makes the setup highly attractive as the basis of an efficient table-top UV pulse compressor.
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We report on a highly-efficient experimental scheme for the generation of deep-ultraviolet ultrashort light pulses using four-wave mixing in gas-filled kagome-style photonic crystal fiber. By pumping with ultrashort, few $mu$J, pulses centered at 400 nm, we generate an idler pulse at 266 nm, and amplify a seeded signal at 800 nm. We achieve remarkably high pump-to-idler energy conversion efficiencies of up to 38%. Although the pump and seed pulse durations are ~100 fs, the generated ultraviolet spectral bandwidths support sub-15 fs pulses. These can be further extended to support few-cycle pulses. Four-wave mixing in gas-filled hollow-core fibres can be scaled to high average powers and different spectral regions such as the vacuum ultraviolet (100-200 nm).
Gas-filled hollow-core photonic crystal fiber (PCF) is used for efficient nonlinear temporal compression of femtosecond laser pulses, two main schemes being direct soliton-effect self-compression, and spectral broadening followed by phase compensation. To obtain stable compressed pulses, it is crucial to avoid decoherence through modulational instability (MI) during spectral broadening. Here we show that changes in dispersion due to spectral anti-crossings between the fundamental core mode and core wall resonances in anti-resonant-guiding hollow-core PCF can strongly alter the MI gain spectrum, enabling MI-free pulse compression for optimized fiber designs. In addition, higher-order dispersion can introduce MI even when the pump pulses lie in the normal dispersion region.
A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond pulses of only few {mu}J energy generate vacuum ultraviolet (VUV) radiation between 5.5 and 9 eV inside the gas-filled fiber. These pulses are used to measure the band structure of the topological insulator Bi2Se3 with a signal to noise ratio comparable to that obtained with high order harmonics from a gas jet. The two-order-of-magnitude gain in efficiency promises time-resolved ARPES measurements at repetition rates of hundreds of kHz or even MHz, with photon energies that cover the first Brillouin zone of most materials.
The resonance band in hollow-core photonic crystal fiber (HC-PCF), while leading to high-loss region in the fiber transmission spectrum, has been successfully used for generating phase-matched dispersive wave (DW). Here, we report that the spectral width of the resonance-induced DW can be largely broadened due to plasma-driven blueshifting soliton. In the experiment, we observed that in a short length of Ar-filled single-ring HC-PCF the soliton self-compression and photoionization effects caused a strong spectral blueshift of the pump pulse, changing the phase-matching condition of the DW emission process. Therefore, broadening of DW spectrum to the longer-wavelength side was obtained with several spectral peaks, which correspond to the generation of DW at different positions along the fiber. In the simulation, we used super-Gauss windows with different central wavelengths to filter out these DW spectral peaks, and studied the time-domain characteristics of these peaks respectively using Fourier transform method. The simulation results verified that these multiple-peaks on the DW spectrum have different delays in the time domain, agreeing well with our theoretical prediction. Remarkably, we found that the whole time-domain DW trace can be compressed to ~29 fs using proper chirp compensation. The experimental and numerical results reported here provide some insight into the resonance-induced DW generation process in gas-filled HC-PCFs, they could also pave the way to ultrafast pulse generation using DW-emission mechanism.
An optical trapping scheme is proposed by which ultrashort low-amplitude radiations, co-propagating with a continuous train of temporal pulses in a hollow-core photonic crystal fiber filled with Raman-inactive noble gases, can be trapped and reshaped into optical soliton trains by means of cross-phase modulation interactions. The scheme complements and extends a recently proposed idea that a single-pulse soliton could trap an ultrashort small-amplitude radiation in a symmetric hollow-core photonic crystal fiber filled with a noble gas, thus preventing its dispersion [M. F. Saleh and F. Biancalana, Phys. Rev. A87, 043807 (2013)]. We find a family of three distinct soliton-train boundstates with different propagation constants, one being a duplicate of the trapping pulse train. We analyze the effects of self-steepening on the trapping (i.e. pump) and trapped (i.e. probe) field profiles and find that self-steepening causes a uniform shift in position of the pump soliton train, but a complex motion for the probe dominanted by anharmonic oscillations of their temporal positions and phases. The new trapping scheme is intended for optical applications involving optical-field cloning and duplication via wave-guided-wave processes, in photonic fiber media in which interplay time-division multiplexed high-intensity pulses coexisting with continuous-wave radiations.
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