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Register a new userTowards photoassociation processes of ultracold rubidium trimers
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We theoretically investigate the prospects for photoassociation (PA) of Rb$_3$, in particular at close range. We provide an overview of accessible states and possible transitions. The major focus is placed on the calculation of equilibrium structures, the survey of spin-orbit effects and the investigation of transition dipole moments. Furthermore we discuss Franck-Condon overlaps and special aspects of trimers including the (pseudo) Jahn-Teller effect and the resulting topology of adiabatic potential-energy surfaces. With this we identify concrete and suitable PA transitions to potentially produce long-lived trimer bound states. Calculations are performed using the multireference configuration-interaction method together with a large-core effective core potential and a core-polarization potential with a large uncontracted even-tempered basis set.
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We perform photoassociation spectroscopy in an ultracold $^{23}$Na-$^6$Li mixture to study the $c^3Sigma^+$ excited triplet molecular potential. We observe 50 vibrational states and their substructure to an accuracy of 20 MHz, and provide line strength data from photoassociation loss measurements. An analysis of the vibrational line positions using near-dissociation expansions and a full potential fit is presented. This is the first observation of the $c^3Sigma^+$ potential, as well as photoassociation in the NaLi system.
MOLSCAT is a general-purpose package for performing non-reactive quantum scattering calculations for atomic and molecular collisions using coupled-channel methods. Simple atom-molecule and molecule-molecule collision types are coded internally and additional ones may be handled with plug-in routines. Plug-in routines may include external magnetic, electric or photon fields (and combinations of them). Simple interaction potentials are coded internally and more complicated ones may be handled with plug-in routines. BOUND is a general-purpose package for performing calculations of bound-state energies in weakly bound atomic and molecular systems using coupled-channel methods. It solves the same sets of coupled equations as MOLSCAT, and can use the same plug-in routines if desired, but with different boundary conditions. FIELD is a development of BOUND that locates external fields at which a bound state exists with a specified energy. One important use is to locate the positions of magnetically tunable Feshbach resonance positions in ultracold collisions. Versions of these programs before version 2019.0 were released separately. However, there is a significant degree of overlap between their internal structures and usage specifications. This manual therefore describes all three, with careful identification of parts that are specific to one or two of the programs.
The experimental realisation of large scale many-body systems has seen immense progress in recent years, rendering full tomography tools for state identification inefficient, especially for continuous systems. In order to work with these emerging physical platforms, new technologies for state identification are required. In this work, we present first steps towards efficient experimental quantum field tomography. We employ our procedure to capture ultracold atomic systems using atom chips, a setup that allows for the quantum simulation of static and dynamical properties of interacting quantum fields. Our procedure is based on cMPS, the continuous analogues of matrix product states (MPS), ubiquitous in condensed-matter theory. These states naturally incorporate the locality present in realistic physical settings and are thus prime candidates for describing the physics of locally interacting quantum fields. The reconstruction procedure is based on two- and four-point correlation functions, from which we predict higher-order correlation functions, thus validating our reconstruction for the experimental situation at hand. We apply our procedure to quenched prethermalisation experiments for quasi-condensates. In this setting, we can use the quality of our tomographic reconstruction as a probe for the non-equilibrium nature of the involved physical processes. We discuss the potential of such methods in the context of partial verification of analogue quantum simulators.
Penning traps, with their ability to control planar crystals of tens to hundreds of ions, are versatile quantum simulators. Thermal occupations of the motional drumhead modes, transverse to the plane of the ion crystal, degrade the quality of quantum simulations. Laser cooling using electromagnetically induced transparency (EIT cooling) is attractive as an efficient way to quickly initialize the drumhead modes to near ground-state occupations. We numerically investigate the efficiency of EIT cooling of planar ion crystals in a Penning trap, accounting for complications arising from the nature of the trap and from the simultaneous cooling of multiple ions. We show that, in spite of challenges, the large bandwidth of drumhead modes (hundreds of kilohertz) can be rapidly cooled to near ground-state occupations within a few hundred microseconds. Our predictions for the center-of-mass mode include a cooling time constant of tens of microseconds and an enhancement of the cooling rate with increasing number of ions. Successful experimental demonstrations of EIT cooling in the NIST Penning trap [E. Jordan, K. A. Gilmore, A. Shankar, A. Safavi-Naini, M. J. Holland, and J. J. Bollinger, Near ground-state cooling of two-dimensional trapped-ion crystals with more than 100 ions, (2018), submitted.] validate our predictions.
We study the time-resolved photoassociation of ultracold sodium in an optical dipole trap. The photoassociation laser excites pairs of atoms to molecular states of large total angular momentum at high intensities (above 20 kW/cm$^{2}$). Such transitions are generally suppressed at ultracold temperatures by the centrifugal barriers for high partial waves. Time-resolved ionization measurements reveal that the atoms are accelerated by the dipole potential of the photoassociation beam. We change the collision energy by varying the potential depth, and observe a strong variation of the photoassociation rate. These results demonstrate the important role of light forces in cw photoassociation at high intensities.
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