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Field-angle dependent vortex lattice phase diagram in MgB2

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 Publication date 2021
  fields Physics
and research's language is English




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Using small-angle neutron scattering we have studied the superconducting vortex lattice (VL) phase diagram in MgB2 as the applied magnetic field is rotated away from the c axis and towards the basal plane. The field rotation gradually suppresses the intermediate VL phase which exists between end states aligned with two high symmetry directions in the hexagonal basal plane for H || c. Above a critical angle, the intermediate state disappears, and the previously continuous transition becomes discontinuous. The evolution towards the discontinuous transition can be parameterized by a vanishing twelvefold anisotropy term in the VL free energy.



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We have studied non-equilibrium phase transitions in the vortex lattice in superconducting MgB2, where metastable states are observed in connection with an intrinsically continuous rotation transition. Using small-angle neutron scattering and a stop-motion technique, we investigated the manner in which the metastable vortex lattice returns to the equilibrium state under the influence of an ac magnetic field. This shows a qualitative difference between the supercooled case which undergoes a discontinuous transition, and the superheated case where the transition to the equilibrium state is continuous. In both cases the transition may be described by an an activated process, with an activation barrier that increases as the metastable state is suppressed, as previously reported for the supercooled vortex lattice [E. R. Louden et al., Phys. Rev. B 99, 060502(R) (2019)]. Separate preparations of superheated metastable vortex lattices with different domain populations showed an identical transition towards the equilibrium state. This provides further evidence that the vortex lattice metastability, and the kinetics associated with the transition to the equilibrium state, is governed by nucleation and growth of domains and the associated domain boundaries.
The vortex lattice (VL) symmetry and orientation in clean type-II superconductors depends sensitively on the host material anisotropy, vortex density and temperature, frequently leading to rich phase diagrams. Typically, a well-ordered VL is taken to imply a ground state configuration for the vortex-vortex interaction. Using neutron scattering we studied the VL in MgB2 for a number of field-temperature histories, discovering an unprecedented degree of metastability in connection with a known, second-order rotation transition. This allows, for the first time, structural studies of a well-ordered, non-equilibrium VL. While the mechanism responsible for the longevity of the metastable states is not resolved, we speculate it is due to a jamming of VL domains, preventing a rotation to the ground state orientation.
Recently, extensive vortex lattice metastability was reported in MgB2 in connection with a second-order rotational phase transition. However, the mechanism responsible for these well-ordered metastable vortex lattice phases is not well understood. Using small-angle neutron scattering, we studied the vortex lattice in MgB2 as it was driven from a metastable to the ground state through a series of small changes in the applied magnetic field. Our results show that metastable vortex lattice domains persist in the presence of substantial vortex motion and directly demonstrate that the metastability is not due to vortex pinning. Instead, we propose that it is due to the jamming of counterrotated vortex lattice domains which prevents a rotation to the ground state orientation.
The superconducting phase diagram of MgB2 was determined from magnetization, magneto-transport and the first single-crystal specific heat measurements. A zero-temperature in-plane coherence length of 8 nm is determined. The superconducting anisotropy increases from a value around 2 near Tc to above 4.5 at 22 K. For H||c a pronounced peak effect in the critical current occurs at the upper critical field. Evidence for a surface superconducting state is presented for H||c which might account for the wide spread in reported values of the anisotropy.
The vortex lattice in MgB2 is characterized by the presence of long-lived metastable states, which arise from cooling or heating across the equilibrium phase boundaries. A return to the equilibrium configuration can be achieved by inducing vortex motion. Here we report on small-angle neutron scattering studies of MgB2, focusing on the structural properties of the vortex lattice as it is gradually driven from metastable to equilibrium states by an AC magnetic field. Measurements were performed using initial metastable states obtained either by cooling or heating across the equilibrium phase transition. In all cases, the longitudinal correlation length remains constant and comparable to the sample thickness. Correspondingly, the vortex lattice may be considered as a system of straight rods, where the formation and growth of equilibrium state domains only occurs in the two-dimensional plane perpendicular to the applied field direction. Spatially resolved raster scans of the sample were performed with apertures as small as 80 microns, corresponding to only 1.2*10^6 vortices for an applied field of 0.5 T. These revealed spatial variations in the metastable and equilibrium vortex lattice populations, but individual domains were not directly resolved. A statistical analysis of the data indicates an upper limit on the average domain size of approximately 50 microns.
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