No Arabic abstract
We determine the nonlocal stress autocorrelation tensor in an homogeneous and isotropic system of interacting Brownian particles starting from the Smoluchowski equation of the configurational probability density. In order to relate stresses to particle displacements as appropriate in viscoelastic states, we go beyond the usual hydrodynamic description obtained in the Zwanzig-Mori projection operator formalism by introducing the proper irreducible dynamics following Cichocki and Hess, and Kawasaki. Differently from these authors, we include transverse contributions as well. This recovers the expression for the stress autocorrelation including the elastic terms in solid states as found for Newtonian and Langevin systems, in case that those are evaluated in the overdamped limit. Finally, we argue that the found memory function reduces to the shear and bulk viscosity in the hydrodynamic limit of smooth and slow fluctuations and derive the corresponding hydrodynamic equations.
Active Brownian particles (ABPs) and Run-and-Tumble particles (RTPs) both self-propel at fixed speed $v$ along a body-axis ${bf u}$ that reorients either through slow angular diffusion (ABPs) or sudden complete randomisation (RTPs). We compare the physics of these two model systems both at microscopic and macroscopic scales. Using exact results for their steady-state distribution in the presence of external potentials, we show that they both admit the same effective equilibrium regime perturbatively that breaks down for stronger external potentials, in a model-dependent way. In the presence of collisional repulsions such particles slow down at high density: their propulsive effort is unchanged, but their average speed along ${bf u}$ becomes $v(rho) < v$. A fruitful avenue is then to construct a mean-field description in which particles are ghost-like and have no collisions, but swim at a variable speed $v$ that is an explicit function or functional of the density $rho$. We give numerical evidence that the recently shown equivalence of the fluctuating hydrodynamics of ABPs and RTPs in this case, which we detail here, extends to microscopic models of ABPs and RTPs interacting with repulsive forces.
We study the linear response of interacting active Brownian particles in an external potential to simple shear flow. Using a path integral approach, we derive the linear response of any state observable to initiating shear in terms of correlation functions evaluated in the unperturbed system. For systems and observables which are symmetric under exchange of the $x$ and $y$ coordinates, the response formula can be drastically simplified to a form containing only state variables in the corresponding correlation functions (compared to the generic formula containing also time derivatives). In general, the shear couples to the particles by translational as well as rotational advection, but in the aforementioned case of $xy$ symmetry only translational advection is relevant in the linear regime. We apply the response formulas analytically in solvable cases and numerically in a specific setup. In particular, we investigate the effect of a shear flow on the morphology and the stress of $N$ confined active particles in interaction, where we find that the activity as well as additional alignment interactions generally increase the response.
The shear stress relaxation modulus $G(t)$ may be determined from the shear stress $tau(t)$ after switching on a tiny step strain $gamma$ or by inverse Fourier transformation of the storage modulus $G^{prime}(omega)$ or the loss modulus $G^{primeprime}(omega)$ obtained in a standard oscillatory shear experiment at angular frequency $omega$. It is widely assumed that $G(t)$ is equivalent in general to the equilibrium stress autocorrelation function $C(t) = beta V langle delta tau(t) delta tau(0)rangle$ which may be readily computed in computer simulations ($beta$ being the inverse temperature and $V$ the volume). Focusing on isotropic solids formed by permanent spring networks we show theoretically by means of the fluctuation-dissipation theorem and computationally by molecular dynamics simulation that in general $G(t) = G_{eq} + C(t)$ for $t > 0$ with $G_{eq}$ being the static equilibrium shear modulus. A similar relation holds for $G^{prime}(omega)$. $G(t)$ and $C(t)$ must thus become different for a solid body and it is impossible to obtain $G_{eq}$ directly from $C(t)$.
The equilibrium properties of a system of passive diffusing particles in an external magnetic field are unaffected by the Lorentz force. In contrast, active Brownian particles exhibit steady-state phenomena that depend on both the strength and the polarity of the applied magnetic field. The intriguing effects of the Lorentz force, however, can only be observed when out-of-equilibrium density gradients are maintained in the system. To this end, we use the method of stochastic resetting on active Brownian particles in two dimensions by resetting them to the line $x=0$ at a constant rate and periodicity in the $y$ direction. Under stochastic resetting, an active system settles into a nontrivial stationary state which is characterized by an inhomogeneous density distribution, polarization and bulk fluxes perpendicular to the density gradients. We show that whereas for a uniform magnetic field the properties of the stationary state of the active system can be obtained from its passive counterpart, novel features emerge in the case of an inhomogeneous magnetic field which have no counterpart in passive systems. In particular, there exists an activity-dependent threshold rate such that for smaller resetting rates, the density distribution of active particles becomes non-monotonic. We also study the mean first-passage time to the $x$ axis and find a surprising result: it takes an active particle more time to reach the target from any given point for the case when the magnetic field increases away from the axis. The theoretical predictions are validated using Brownian dynamics simulations.
Active particles may happen to be confined in channels so narrow that they cannot overtake each other (Single File conditions). This interesting situation reveals nontrivial physical features as a consequence of the strong inter-particle correlations developed in collective rearrangements. We consider a minimal model for active Brownian particles with the aim of studying the modifications introduced by activity with respect to the classical (passive) Single File picture. Depending on whether their motion is dominated by translational or rotational diffusion, we find that active Brownian particles in Single File may arrange into clusters which are continuously merging and splitting ({it active clusters}) or merely reproduce passive-motion paradigms, respectively. We show that activity convey to self-propelled particles a strategic advantage for trespassing narrow channels against external biases (e.g., the gravitational field).