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Register a new userOrbital angular momentum multiplication in plasmonic vortex cavities
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Orbital angular momentum of light is a core feature in photonics. Its confinement to surfaces using plasmonics has unlocked many phenomena and potential applications. Here we introduce the reflection from structural boundaries as a new degree of freedom to generate and control plasmonic orbital angular momentum. We experimentally demonstrate plasmonic vortex cavities, generating a succession of vortex pulses with increasing topological charge as a function of time. We track the spatio-temporal dynamics of these angularly decelerating plasmon pulse train within the cavities for over 300 femtoseconds using time-resolved Photoemission Electron Microscopy, showing that the angular momentum grows by multiples of the chiral order of the cavity. The introduction of this degree of freedom to tame orbital angular momentum delivered by plasmonic vortices, could miniaturize pump-probe-like quantum initialization schemes, increase the torque exerted by plasmonic tweezers and potentially achieve vortex lattice cavities with dynamically evolving topology.
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Understanding the near-field electromagnetic interactions that produce optical orbital angular momentum (OAM) is central to the integration of twisted light into nanotechnology. Here, we examine the cathodoluminescence (CL) of plasmonic vortices carrying OAM generated in spiral nanostructures through scanning transmission electron microscopy (STEM). The nanospiral geometry defines the photonic local density of states (LDOS) sampled by STEM-CL, which provides access to the phase and amplitude of the plasmonic vortex with nanometer spatial and meV spectral resolution. We map the full spectral dispersion of the plasmonic vortex in the spiral structure and examine the effects of increasing topological charge on the plasmon phase and amplitude in the detected CL signal. The vortex is mapped in CL over a broad spectral range, and deviations between the predicted and detected positions of near-field optical signatures of as much as 5 per cent are observed. Finally, enhanced luminescence is observed from concentric spirals of like handedness compared to that from concentric spirals of opposite handedness, indicating the potential to couple plasmonic vortices to chiral nanostructures for sensitive detection and manipulation of optical OAM.
Lights orbital angular momentum (OAM) is an unbounded degree of freedom emerging in helical beams that appears very advantageous technologically. Using a chiral microlaser, i.e. an integrated device that allows generating an emission carrying a net OAM, we demonstrate a regime of bistability involving two modes presenting distinct OAM (L = 0 and L = 2). Furthermore, thanks to an engineered spin-orbit coupling of light in the device, these modes also exhibit distinct polarization patterns, i.e. cirular and azimuthal polarizations. Using a dynamical model of rate euqations, we show that this bistability arises from polarization-dependent saturation of the gain medium. Such a bistable regime appears very promising for implementing ultrafast optical switches based on the OAM of light. As well, it paves the way to the exploration of dynamical processes involving phase and polarization vortices.
Quantum theory of surface plasmons is very important for studying the interactions between light and different metal nanostructures in nanoplasmonics. In this work, using the canonical quantization method, the SPPs on nanowires and their orbital and spin angular momentum are investigated. The results show that the SPPs on nanowire carry both orbital and spin momentum during propagation. Later, the result is applied on the plasmonic nanowire waveguide to show the agreement of the theory. The study is helpful for the nano wire based plasmonic interactions and the quantum information based optical circuit in the future.
We theoretically and experimentally investigated transformations of vortex beams subjected to sector perturbations in the form of hard-edged aperture. The transformations of the vortex spectra, the orbital angular momentum, and the informational entropy of the perturbed beam were studied. We found that relatively small angular sector perturbations have almost no effect on OAM, although the informational entropy is rapidly increasing due to the birth of new optical vortices caused by diffraction by diaphragm edges. At large perturbation angles, the uncertainty principle between the angle and OAM involves vortices, with both positive and negative topological charges, so that the OAM decreases to almost zero, and the entropy increases sharply.
Chiral surface states along the zigzag edge of a valley photonic crystal in the honeycomb lattice are demonstrated. By decomposing the local fields into orbital angular momentum (OAM) modes, we find that the chiral surface states present OAM-dependent unidirectional propagation characteristics. Particularly, the propagation directivities of the surface states are quantified by the local OAM decomposition and are found to depend on the chiralities of both the source and surface states. These findings allow for the engineering control of the unidirectional propagation of electromagnetic energy without requiring an ancillary cladding layer. Furthermore, we examine the propagation of the chiral surface states against sharp bends. It turns out that although only certain states successfully pass through the bend, the unidirectional propagation is well maintained due to the topology of the structure.
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