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Optical Control of Topological Polariton Phase in a Perovskite Lattice

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 Added by Rui Su
 Publication date 2020
  fields Physics
and research's language is English




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Strong light-matter interaction enriches topological photonics by dressing light with matter, which provides the possibility to realize tuneable topological devices with immunity to defects. Topological exciton polaritons, half-light half-matter quasiparticles with giant optical nonlinearity represent a unique platform for active topological photonics with phase tunability. Previous demonstrations of exciton polariton topological insulators still demand cryogenic temperatures and their topological properties are usually fixed without phase tunability. Here, we experimentally demonstrate a room-temperature exciton polariton topological insulator with active phase tunability in a perovskite zigzag lattice. Polarization serves as a degree of freedom to control the reversible transition between distinct topological phases, thanks to the polarization-dependent anisotropy in halide perovskite microcavities. The topologically nontrivial polariton states localized in the edges persist in the presence of a natural defect, showing strong immunity to disorder. We further demonstrate that exciton polaritons can condense into the topological edge states under optical pumping. These results provide an ideal platform for realizing tuneable topological polaritonic devices with room-temperature operation, which can find important applications in optical control, modulation and switching.



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Topological insulators are a class of electronic materials exhibiting robust edge states immune to perturbations and disorder. This concept has been successfully adapted in photonics, where topologically nontrivial waveguides and topological lasers were developed. However, the exploration of topological properties in a given photonic system is limited to a fabricated sample, without the flexibility to reconfigure the structure in-situ. Here, we demonstrate an all-optical realization of the orbital Su-Schrieffer-Heeger (SSH) model in a microcavity exciton-polariton system, whereby a cavity photon is hybridized with an exciton in a GaAs quantum well. We induce a zigzag potential for exciton polaritons all-optically, by shaping the nonresonant laser excitation, and measure directly the eigenspectrum and topological edge states of a polariton lattice in a nonlinear regime of bosonic condensation. Furthermore, taking advantage of the tunability of the optically induced lattice we modify the intersite tunneling to realize a topological phase transition to a trivial state. Our results open the way to study topological phase transitions on-demand in fully reconfigurable hybrid photonic systems that do not require sophisticated sample engineering.
We developed planar multilayered photonic-plasmonic structures, which support topologically protected optical states on the interface between metal and dielectric materials, known as optical Tamm states. Coupling of incident light to the Tamm states can result in perfect absorption within one of several narrow frequency bands, which is accompanied by a singular behavior of the phase of electromagnetic field. In the case of near-perfect absorptance, very fast local variation of the phase can still be engineered. In this work, we theoretically and experimentally demonstrate how these drastic phase changes can improve sensitivity of optical sensors. A planar Tamm absorber was fabricated and used to demonstrate remote near-singular-phase temperature sensing with an over an order of magnitude improvement in sensor sensitivity and over two orders of magnitude improvement in the figure of merit over the standard approach of measuring shifts of resonant features in the reflectance spectra of the same absorber. Our experimentally demonstrated phase-to-amplitude detection sensitivity improvement nearly doubles that of state-of-the-art nano-patterned plasmonic singular-phase detectors, with further improvements possible via more precise fabrication. Tamm perfect absorbers form the basis for robust planar sensing platforms with tunable spectral characteristics, which do not rely on low-throughput nano-patterning techniques.
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The phase and the frequency of an exciton polariton condensate excited by a nonresonant pump can be efficiently manipulated by an external coherent light. Being tuned close to the resonance with the condensate eigenfrequency, the external laser light imposes its frequency to the condensate and locks its phase, thereby manifesting a synchronization effect. The conditions of formation of the phase synchronized regime are determined. The synchronization of a couple of closely spaced polariton condensates by a spatially uniform coherent light is examined. At the moderate strength of the coherent driving the synchronization is accompanied by the appearance of symmetry-breaking states of the polariton dyad, while these states are superseded by the symmetric state at the high-intensity driving. By employing a zero-dimensional model of coupled dissipative oscillators with both dissipative and conservative coupling, we study the bifurcation scenario of the symmetry-breaking state formation.
We find an optical Raman lattice without spin-orbit coupling showing chiral topological orders for cold atoms. Two incident plane-wave lasers are applied to generate simultaneously a double-well square lattice and periodic Raman couplings, the latter of which drive the nearest-neighbor hopping and create a staggered flux pattern across the lattice. Such a minimal setup is can yield the quantum anomalous Hall effect in the single particle regime, while in the interacting regime it achieves the $J_1$-$J_2$-$K$ model with all parameters controllable, which supports a chiral spin liquid phase. We further show that heating in the present optical Raman lattice is reduced by more than one order of magnitude compared with the conventional laser-assisted tunneling schemes. This suggests that the predicted topological states be well reachable with the current experimental capability.
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