Electronic correlations in the van der Waals ferromagnet Fe$_3$GeTe$_2$ revealed by its charge dynamics


Abstract in English

The layered van der Waals ferromagnetic Fe$_3$GeTe$_2$ harbours an unconventional interplay between topology and magnetism, leading to a large anomalous Hall conductivity at low temperatures. Here, we investigate the temperature dependence of its charge dynamics and reveal that upon entering the ferromagnetic state at $T_C sim 200$ K and further lowering the temperature there is the onset of a gradual spectral weight reshuffling from the mid-infrared range towards far- as well as near-infrared frequencies. This two-fold spectral weight transfer indicates the important role of the Hunds coupling as primary source for electronic correlations and signals an incoherent-coherent crossover at low temperatures. Our findings also convey the electronic environment, based on nodal-line topological states, favouring the large anomalous Hall conductivity.

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