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Register a new userHigh-Harmonic Generation and Spin-Orbit Interaction of Light in a Relativistic Oscillating Window
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Authors
Longqing Yi
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When a high power laser beam irradiates a small aperture on a solid foil target, the strong laser field drives surface plasma oscillation at the periphery of this aperture, which acts as a relativistic oscillating window. The diffracted light that travels though such an aperture contains high-harmonics of the fundamental laser frequency. When the driving laser beam is circularly polarised, the high-harmonic generation (HHG) process facilitates a conversion of the spin angular momentum of the fundamental light into the intrinsic orbital angular momentum of the harmonics. By means of theoretical modeling and fully 3D particle-in-cell simulations, it is shown the harmonic beams of order $n$ are optical vortices with topological charge $|l| = n-1$, and a power-law spectrum $I_npropto n^{-3.5}$ is produced for sufficiently intense laser beams, where $I_n$ is the intensity of the $n$th harmonic. This work opens up a new realm of possibilities for producing intense extreme ultraviolet vortices, and diffraction-based HHG studies at relativistic intensities.
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We report the enhancement of individual harmonics generated at a relativistic ultra-steep plasma vacuum interface. Simulations show the harmonic emission to be due to the coupled action of two high velocity oscillations -- at the fundamental $omega_L$ and at the plasma frequency $omega_P$ of the bulk plasma. The synthesis of the enhanced harmonics can be described by the reflection of the incident laser pulse at a relativistic mirror oscillating at $omega_L$ and $omega_P$.
We observe the generation of high harmonics in the plane perpendicular to the driving laser polarization and show that these are driven by the spin-orbit interaction. Using R-Matrix with time-dependence theory, we demonstrate that for certain initial states either circularly- or linearly- polarized harmonics arise via well-known selection rules between atomic states controlled by the spin-orbit interaction. Finally, we elucidate the connection between the observed harmonics and the phase of the intial state.
We study high-harmonic generation in two-dimensional electron systems with Rashba and Dresselhaus spin-orbit coupling and derive harmonic generation selection rules with the help of group theory. Based on the bandstructures of these minimal models and explicit simulations we reveal how the spin-orbit parameters control the cutoff energy in the high-harmonic spectrum. We also show that the magnetic field and polarization dependence of this spectrum provides information on the magnitude of the Rashba and Dresselhaus spin-orbit coupling parameters. The shape of the Fermi surface can be deduced at least qualitatively and if only one type of spin-orbit coupling is present, the coupling strength can be determined.
Experiments on the excitation of propagating surface plasmons (SPs) by ultrashort, high intensity laser interaction with grating targets are reviewed. At intensities exceeding $10^{19}~mbox{W cm}^{-2}$ on target, i.e. in the strongly relativistic regime of electron dynamics, multi-MeV electrons are accelerated by the SP field as dense bunches collimated in a near-tangent direction. By the use of a suitable blazed grating, the bunch charge can be increased up to $simeq $660 picoCoulomb. Intense XUV high harmonics (HH) diffracted by the grating are observed when a plasma with sub-micrometer scale is produced at the target surface by a controlled prepulse. When the SP is excited, the HH are strongly enhanced in a direction quasi-parallel to the electrons. Simulations show that the HH are boosted by nanobunching in the SP field of the electrons which scatter the laser field. Besides the static and dynamic tailoring of the target density profile, further control of electron and HH emission might be achieved by changing the SP duration using a laser pulse with rotating wavefront. This latter technique may be capable to produce nearly single-cycle SPs.
A new physical mechanism to achieve spin-to-orbital angular momentum conversion based on the interaction of an intense circularly polarized (CP) laser beam with a plane foil is presented and studied for the first time. It has been verified by both simulation and theoretical analysis that vortex harmonics carrying orbital angular momentum (OAM) are generated after a relativistic CP laser beam, even a Gaussian beam, impinges normally on a plane foil. The generation of this vortex harmonics is attributed to the vortex oscillation of the plasma surface driven harmonically by the vortex longitudinal electric field of the CP beam. During the process of harmonic generation, the spin angular momenta of fundamental-frequency photons are converted to OAM of harmonic photon because of the conservation of total angular momentum. In addition, if an initially vortex beam or a spiral phase plate is used, the OAM of harmonic photon can be more tunable and controllable.
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