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Register a new userOptimal two-photon excitation of bound states in non-Markovian waveguide QED
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Bound states arise in waveguide QED systems with a strong frequency-dependence of the coupling between emitters and photonic modes. While exciting such bound-states with single photon wave-packets is not possible, photon-photon interactions mediated by the emitters can be used to excite them with two-photon states. In this letter, we use scattering theory to provide upper limits on this excitation probability for a general non-Markovian waveguide QED system and show that this limit can be reached by a two-photon wave-packet with vanishing uncertainty in the total photon energy. Furthermore, we also analyze multi-emitter waveguide QED systems with multiple bound states and provide a systematic construction of two-photon wave-packets that can excite a given superposition of these bound states. As specific examples, we study bound state trapping in waveguide QED systems with single and multiple emitters and a time-delayed feedback.
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We develop a formalism for modelling exact time dynamics in waveguide quantum electrodynamics (QED) using the real-space approach. The formalism does not assume any specific configuration of emitters and allows the study of Markovian dynamics fully analytically and non-Markovian dynamics semi-analytically with a simple numerical integration step. We use the formalism to study subradiance, superradiance and bound states in continuum. We discuss new phenomena such as subdivision of collective decay rates into symmetric and anti-symmetric subsets and non-Markovian superradiance effects that can lead to collective decay stronger than Dicke superradiance. We also discuss possible applications such as pulse-shaping and coherent absorption. We thus broaden the range of applicability of real-space approaches beyond steady-state photon transport.
We discuss the properties of bound states in finite-bandwidth waveguide QED beyond the Rotating Wave Approximation or excitation number conserving light-matter coupling models. Therefore, we extend the emph{standard} calculations to a broader range of light-matter strengths, in particular, in the so-called ultrastrong coupling regime. We do this using the Polaron technique. Our main results are as follows. We compute the spontaneous emission rate, which is renormalized as compared to the Fermi Golden Rule formula. We generalise the existence criteria for bound states, their properties and their role in the qubits thermalization. We discuss effective spin-spin interactions through both vacuum fluctuations and bound states. Finally, we sketch a perfect state-transfer protocol among distant emitters.
We give an exposure to diagrammatic techniques in waveguide QED systems. A particular emphasis is placed on the systems with delayed coherent quantum feedback. Specifically, we show that the $N$-photon scattering matrices in single-qubit waveguide QED systems, within the rotating wave approximation, admit for a parametrization in terms of $N-1$-photon effective vertex functions and provide a detailed derivation of a closed hierarchy of generalized Bethe-Salpeter equations satisfied by these vertex functions. The advantage of this method is that the above mentioned integral equations hold independently of the number of radiation channels, their bandwidth, the dispersion of the modes they are supporting, and the structure of the radiation-qubit coupling interaction, thus enabling one to study multi-photon scattering problems beyond the Born-Markov approximation. Further, we generalize the diagrammatic techniques to the systems containing more than a single emitter by presenting an exact set of equations governing the generic two and three-photon scattering operators. The above described theoretical machinery is then showcased on the example of a three-photon scattering on a giant acoustic atom, recently studied experimentally [Nat. Phys. 15, 1123 (2019)].
We develop an approach to light-matter coupling in waveguide QED based upon scattering amplitudes evaluated via Dyson series. For optical states containing more than single photons, terms in this series become increasingly complex and we provide a diagrammatic recipe for their evaluation, which is capable of yielding analytic results. Our method fully specifies a combined emitter-optical state that permits investigation of light-matter entanglement generation protocols. We use our expressions to study two-photon scattering from a $Lambda$-system and find that the pole structure of the transition amplitude is dramatically altered as the two ground states are tuned from degeneracy.
We report a system where fixed interactions between non-computational levels make bright the otherwise forbidden two-photon 00 --> 11 transition. The system is formed by hand selection and assembly of two discrete component transmon-style superconducting qubits inside a rectangular microwave cavity. The application of a monochromatic drive tuned to this transition induces two-photon Rabi-like oscillations between the ground and doubly-excited states via the Bell basis. The system therefore allows all-microwave two-qubit universal control with the same techniques and hardware required for single qubit control. We report Ramsey-like and spin echo sequences with the generated Bell states, and measure a two-qubit gate fidelity of 90% (unconstrained) and 86% (maximum likelihood estimator).
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