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Register a new userSpin Order and Entropy in Antiferromagnetic Films Subjected to Magnetic Fields
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Christoph Peter Hofmann
Publication date
2020
fields
Physics
and research's language is
English
Authors
Christoph P. Hofmann
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Using systematic effective field theory, we explore the properties of antiferromagnetic films subjected to magnetic and staggered fields that are either mutually aligned or mutually orthogonal. We provide low-temperature series for the entropy density in either case up to two-loop order. Invoking staggered, uniform and sublattice magnetizations of the bipartite antiferromagnet, we investigate the subtle order-disorder phenomena in the spin arrangement, induced by temperature, magnetic and staggered fields -- some of which are quite counterintuitive. In the figures we focus on the spin-$frac{1}{2}$ square-lattice antiferromagnet, but our results are valid for any other bipartite two-dimensional lattice.
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The thermal properties of antiferromagnetic films -- in particular, the square-lattice antiferromagnet -- subjected to an external magnetic field pointing into the direction of the staggered magnetization are explored. The effective field theory analysis of the free energy density is carried out to two-loop order. While the emphasis is on finite temperature, we also discuss the behavior of the magnetization and staggered magnetization at zero temperature. Our results imply that the staggered magnetization increases in presence of the magnetic field -- reminiscent of magnetic catalysis. Most remarkably, if staggered and magnetic field strength are kept fixed, the magnetization initially grows when temperature increases.
We analyze the thermodynamic properties of antiferromagnetic solids subjected to a combination of mutually orthogonal uniform magnetic and staggered fields. Low-temperature series for the pressure, order parameter and magnetization up to two-loop order in the effective expansion are established. We evaluate the self-energy and the dispersion relation of the dressed magnons in order to discuss the impact of spin-wave interactions on thermodynamic observables.
We explore the behavior of the order parameter and the magnetization of antiferromagnetic solids subjected to mutually parallel staggered and magnetic fields. The effective field theory analysis of the partition function is taken up to the two-loop level, where the magnon-magnon interaction comes into play. These interaction effects, however, are small. A phenomenon that comes rather unexpectedly is that the finite-temperature magnetization increases with temperature when the strengths of the staggered and magnetic field are held constant.
We report extensive measurements on a new compound (Yb0.24Sn0.76)Ru that crystallizes in the cubic CsCl structure. Valence band photoemission and L3 x-ray absorption show no divalent component in the 4f configuration of Yb. Inelastic neutron scattering (INS) indicates that the eight-fold degenerate J-multiplet of Yb3+ is split by the crystalline electric field (CEF) into a {Gamma}7 doublet ground state and a {Gamma}8 quartet at an excitation energy 20 meV. The magnetic susceptibility can be fit very well by this CEF scheme under the assumption that a {Gamma}6 excited state resides at 32 meV; however, the {Gamma}8/{Gamma}6 transition expected at 12 meV was not observed in the INS. The resistivity follows a Bloch- Gruneisen law shunted by a parallel resistor, as is typical of systems subject to phonon scattering with no apparent magnetic scattering. All of these properties can be understood as representing simple local moment behavior of the trivalent Yb ion. At 1 K, there is a peak in specific heat that is too broad to represent a magnetic phase transition, consistent with absence of magnetic reflections in neutron diffraction. On the other hand, this peak also is too narrow to represent the Kondo effect in the {Gamma}7 ground state doublet. On the basis of the field-dependence of the specific heat, we argue that antiferromagnetic shortrange order (possibly co-existing with Kondo physics) occurs at low temperatures. The long-range magnetic order is suppressed because the Yb site occupancy is below the percolation threshold for this disordered compound.
A review of recent state-of-the-art pulsed field experiments performed on URu$_2$Si$_2$ under a magnetic field applied along its easy magnetic axis $mathbf{c}$ is given. Resistivity, magnetization, magnetic susceptibility, Shubnikov-de Haas, and neutron diffraction experiments are presented, permitting to emphasize the relationship between Fermi surface reconstructions, the destruction of the hidden-order and the appearance of a spin-density wave state in a high magnetic field.
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