No Arabic abstract
Under optical cooling of nuclei, a strongly correlated nuclear-spin polaron state can form in semiconductor nanostructures with localized charge carriers due to the strong hyperfine interaction of the localized electron spin with the surrounding nuclear spins. Here we develop a kinetic-equation formalism describing the nuclear-spin polaron formation. We present a derivation of the kinetic equations for an electron-nuclear spin system coupled to reservoirs of different electron and nuclear spin temperatures which generate the exact thermodynamic steady state for equal temperatures independent of the system size. We illustrate our approach using the analytical solution of the central spin model in the limit of an Ising form of the hyperfine coupling. For homogeneous hyperfine coupling constants, i.e., the box model, the model is reduced to an analytically solvable form. Based on the analysis of the nuclear-spin distribution function and the electron-nuclear spin correlators, we derive a relation between the electron and nuclear spin temperatures, where the correlated nuclear-spin polaron state is formed. In the limit of large nuclear baths, this temperature line coincides with the critical temperature of the mean-field theory for polaron formation. The criteria of the polaron formation in a finite-size system are discussed. We demonstrate that the systems behavior at the transition temperature does not depend on details of the hyperfine-coupling distribution function but only on the effective number of coupled bath spins. In addition, the kinetic equations enable the analysis of the temporal formation of the nuclear-polaron state, where we find the build-up process predominated by the nuclear spin-flip dynamics.
The physics of interacting nuclear spins arranged in a crystalline lattice is typically described using a thermodynamic framework: a variety of experimental studies in bulk solid-state systems have proven the concept of a spin temperature to be not only correct but also vital for the understanding of experimental observations. Using demagnetization experiments we demonstrate that the mesoscopic nuclear spin ensemble of a quantum dot (QD) can in general not be described by a spin temperature. We associate the observed deviations from a thermal spin state with the presence of strong quadrupolar interactions within the QD that cause significant anharmonicity in the spectrum of the nuclear spins. Strain-induced, inhomogeneous quadrupolar shifts also lead to a complete suppression of angular momentum exchange between the nuclear spin ensemble and its environment, resulting in nuclear spin relaxation times exceeding an hour. Remarkably, the position dependent axes of quadrupolar interactions render magnetic field sweeps inherently non-adiabatic, thereby causing an irreversible loss of nuclear spin polarization.
In this paper we study the phonons effect on the position of the 1s excitonic resonance of the fundamental absorption transition line in two-dimensional transition metal dichalcogenides. We apply our theory to WS$_{2}$a two-dimensional material where the shift in absorption peak position has been measured as a function of temperature. The theory is composed of two ingredients only: i) the effect of longitudinal optical phonons on the absorption peak position, which we describe with second order perturbation theory; ii) the effect of phonons on the value of the single particle energy gap, which we describe with the Huang Rhys model. Our results show an excellent agreement with the experimentally measured shift of the absorption peak with the temperature.
We consider the use of a Kinetic Monte Carlo approach for the description of non-equilibrium bosonic systems, taking non-resonantly excited exciton-polariton condensates and bosonic cascade lasers as examples. In the former case, the considered approach allows the study of the cross-over between incoherent and coherent regimes, which represents the formation of a quasi-condensate that forms purely from the action of energy relaxation processes rather than interactions between the condensing particles themselves. In the latter case, we show that a bosonic cascade can theoretically develop an output coherent state.
We study the formation of magnon-polaron excitations and the consequences of different time scales between the magnon and lattice dynamics. The spin-spin interactions along the 1D lattice are ruled by a Heisenberg Hamiltonian in the anisotropic form XXZ, in which each spin exhibits a vibrational degree of freedom around its equilibrium position. By considering a magnetoelastic coupling as a linear function of the relative displacement between nearest-neighbor spins, results provide an original framework for achieving a hybridized state of magnon-polaron. Such state is characterized by high cooperation between the underlying excitations, where the traveling or stationary formation of magnon-polaron depends on the effective magnetoelastic coupling. A systematic investigation reveals the critical amount of the magnon-lattice interaction ($chi_c$) necessary to emergence of the stationary magnon-polaron quasi-particle. Different characteristic time scales of the magnon and the vibrational dynamics unveiled the threshold between the two regimes, as well as a limiting value of critical magnetoelastic interaction, above which the magnon velocity no longer interferes at the critical magnetoelastic coupling capable of inducing the stationary regime.
We develop a Boltzmann transport theory of coupled magnon-phonon transport in ferromagnetic insulators. The explicit treatment of the magnon-phonon coupling within the Boltzmann approach allows us to calculate the low-temperature magnetic-field dependence of the spin-Seebeck voltage. Within the Boltzmann theory we find that this magnetic field dependence shows similar features as found by Flebus et al. [Phys. Rev. B 95, 144420 (2017)] for a strongly coupled magnon phonon system that forms magnon-polarons, and consistent with experimental findings in yttrium iron garnet by Kikkawa et al. [Phys. Rev. Lett. 117, 207203 (2016)]. In addition to the anomalous magnetic-field dependence of the spin Seebeck effect, we also predict a dependence on the system size.