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Register a new userSecond-harmonic generation via double topological valley-Hall kink modes in all-dielectric photonic crystals
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Nonlinear topological photonics, which explores topics common to the fields of topological phases and nonlinear optics, is expected to open up a new paradigm in topological photonics. Here, we demonstrate second-harmonic generation (SHG) via nonlinear interaction of double topological valley-Hall kink modes in all-dielectric photonic crystals (PhCs). We first show that two topological frequency bandgaps can be created around a pair of frequencies, $omega_0$ and $2omega_0$, by gapping out the corresponding Dirac points in two-dimensional honeycomb PhCs. Valley-Hall kink modes along a kink-type domain wall interface between two PhCs placed together in a mirror-symmetric manner are generated within the two frequency bandgaps. Importantly, through full-wave simulations and mode dispersion analysis, we demonstrate that tunable, bi-directional phase-matched SHG via nonlinear interaction of the valley-Hall kink modes inside the two bandgaps can be achieved. In particular, by using Stokes parameters associated to the magnetic part of the valley-Hall kink modes, we introduce a new concept, SHG directional dichroism, which is employed to characterize optical probes for sensing chiral molecules. Our work opens up new avenues towards topologically protected nonlinear frequency mixing and active photonic devices implemented in all-dielectric material platforms.
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We experimentally and theoretically investigate the second order nonlinear optical response of metallo-dielectric multilayer structures composed of Ag and Ta2O5 layers, deposited by magnetron sputtering. Second harmonic generation measurements were performed in reflection mode as a function of incidence angle, using femtosecond pulses originating from a Ti:Sapphire laser system tuned at 800 nm. The dependence of the generated signal was investigated as a function of pump intensity and polarization state. Our experimental results show that the conversion efficiency from a periodic metallo-dielectric sample may be enhanced by at least a factor of 30 with respect to the conversion efficiency from a single metal layer, thanks in part to the increased number of active surfaces, pump field localization and penetration inside the metal layers. The conversion efficiency maximum shifts from 70 degrees for the single silver layer down to approximately 55 degrees for the stack. The experimental results are found to be in good agreement with calculations based on coupled Maxwell-Drude oscillators under the action of a nonlinear Lorentz force term.
Extensive researches have revealed that valley, a binary degree of freedom (DOF), can be an excellent candidate of information carrier. Recently, valley DOF has been introduced into photonic systems, and several valley-Hall photonic topological insulators (PTIs) have been experimentally demonstrated. However, in the previous valley-Hall PTIs, topological kink states only work at a single frequency band, which limits potential applications in multiband waveguides, filters, communications, and so on. To overcome this challenge, here we experimentally demonstrate a valley-Hall PTI, where the topological kink states exist at two separated frequency bands, in a microwave substrate-integrated circuitry. Both the simulated and experimental results demonstrate the dual-band valley-Hall topological kink states are robust against the sharp bends of the internal domain wall with negligible inter-valley scattering. Our work may pave the way for multi-channel substrate-integrated photonic devices with high efficiency and high capacity for information communications and processing.
We demonstrate enhanced second harmonic generation in a gallium phosphide photonic crystal waveguide with a measured external conversion efficiency of 5$times10^{-7}$/W. Our results are promising for frequency conversion of on-chip integrated emitters having broad spectra or large inhomogeneous broadening, as well as for frequency conversion of ultrashort pulses.
We report the observations of unexpected layer-dependent, strong, and anisotropic second harmonic generations (SHGs) in atomically thin ReS2. Appreciable (negligible) SHGs are obtained from even (odd) numbers of ReS2 layers, which is opposite to the layer-dependence of SHGs in group VI transition metal dichalcogenides, such as MoS2 and WS2. The results are analyzed from ReS2s crystal structure, implying second harmonic polarizations generated from the interlayer coupling. Pumped by a telecomband laser, SHG from the bilayer ReS2 is almost one order of magnitude larger than that from the monolayer WS2. The estimated second-order nonlinear susceptibility of 900 pm/V is remarkably high among those reported in two-dimensional materials. The laser polarization dependence of ReS2s SHG is strongly anisotropic and indicates its distorted lattice structure with more unequal and non-zero second-order susceptibility elements.
On the basis of the Edward-Kornfeld formulation, we study the effective susceptibility of secondharmonic generation (SHG) in colloidal crystals, which are made of graded metallodielectric nanoparticles with an intrinsic SHG susceptibility suspended in a host liquid. We find a large enhancement and redshift of SHG responses, which arises from the periodic structure, local field effects and gradation in the metallic cores. The optimization of the Ewald-Kornfeld formulation is also investigated.
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