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Tunable chirality of noncentrosymmetric magnetic Weyl semimetals

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 Added by Rajyavardhan Ray
 Publication date 2020
  fields Physics
and research's language is English




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Even if Weyl semimetals are characterized by quasiparticles with well-defined chirality, exploiting this experimentally is severely hampered by Weyl lattice-fermions coming in pairs with opposite chirality, typically causing the net chirality picked up by experimental probes to vanish. Here we show this issue can be circumvented in a controlled manner when both time-reversal- and inversion- symmetry are broken. To this end, we investigate chirality-disbalance in the carbide family RMC$_2$ (R a rare-earth and M a transition metal), showing several members to be Weyl semimetals. Using the noncentrosymmetric ferromagnet NdRhC$_2$ as an illustrating example, we show that an odd number of Weyl nodes can be stabilized at its Fermi surface by properly tilting its magnetization. The tilt direction determines the sign of the resulting net chirality, opening up a simple route to control it.

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We describe a new type of the Chiral Magnetic Effect (CME) that should occur in Weyl semimetals with an asymmetry in the dispersion relations of the left- and right-handed chiral Weyl fermions. In such materials, time-dependent pumping of electrons from a non-chiral external source generates a non-vanishing chiral chemical potential. This is due to the different capacities of the left- and right-handed (LH and RH) chiral Weyl cones arising from the difference in the density of states in the LH and RH cones. The chiral chemical potential then generates, via the chiral anomaly, a current along the direction of an applied magnetic field even in the absence of an external electric field. The source of chirality imbalance in this new setup is thus due to the band structure of the system and the presence of (non-chiral) electron source, and not due to the parallel electric and magnetic fields. We illustrate the effect by an argument based on the effective field theory, and by the chiral kinetic theory calculation for a rotationally invariant Weyl semimetal with different Fermi velocities in the left and right chiral Weyl cones; we also consider the case of a Weyl semimetal with Weyl nodes at different energies. We argue that this effect is generically present in Weyl semimetals with different dispersion relations for LH and RH chiral Weyl cones, such as SrSi2 recently predicted as a Weyl semimetal with broken inversion and mirror symmetries, as long as the chiral relaxation time is much longer than the transport scattering time.
Smooth interfaces of topological systems are known to host massive surface states along with the topologically protected chiral one. We show that in Weyl semimetals these massive states, along with the chiral Fermi arc, strongly alter the form of the Fermi-arc plasmon, Most saliently, they yield further collective plasmonic modes that are absent in a conventional interfaces. The plasmon modes are completely anisotropic as a consequence of the underlying anisotropy in the surface model and expected to have a clear-cut experimental signature, e.g. in electron-energy loss spectroscopy.
We study the dynamic chiral magnetic conductivity (DCMC) and natural optical activity in an inversion-broken tilted Weyl semimetal (WSM). Starting from the Kubo formula, we derive the analytical expressions for the DCMC for two different directions of the incident electromagnetic wave. We show that the angle of rotation of the plane of polarization of the transmitted wave exhibits remarkable anisotropic behavior and is larger along the tilt direction. This striking anisotropy of DCMC which results in anisotropic optical activity and rotary power, can be experimentally observed as a topological magneto-electric effect of inversion-broken tilted WSMs. Finally, using the low energy Hamiltonian, we show that the DCMC follows the universal $frac{1}{omega^2}$ decay in the high frequency regime. In the low frequency regime, however, the DCMC shows sharp peaks at the tilt dependent effective chemical potentials of the left-handed and right-handed Weyl points. This can serve as a signature to distinguish between the type-I and type-II Weyl semimetals.
Topological Weyl semimetals (TWS) can be classified as type-I TWS, in which the density of states vanishes at the Weyl nodes, and type-II TWS where an electron and a hole pocket meet with finite density of states at the nodal energy. The dispersions of type-II Weyl nodes are tilted and break Lorentz invariance, allowing for physical properties distinct from those in a type-I TWS. We present minimal lattice models for both time-reversal-breaking and inversion-breaking type-II Weyl semimetals, and investigate their bulk properties and topological surface states. These lattice models capture the extended Fermi pockets and the connectivities of Fermi arcs. In addition to the Fermi arcs, which are topologically protected, we identify surface track states that arise out of the topological Fermi arc states at the transition from type-I to type-II with multiple Weyl nodes, and persist in the type-II TWS.
In Weyl semimetals the location of linear band crossings, the Weyl cones, is not bound to any high symmetry point of the Brillouin zone, unlike the Dirac nodes in graphene. This flexibility is advantageous for valleytronics, where information is encoded in the valleys of the band structure when intervalley scattering is weak. However, if numerous Weyl cones coexist the encoded information can decohere rapidly because of band mixing. Here, we investigate how the helical iso-spin texture of Weyl cones affects valleytronics in heterojunctions of Weyl materials, and show how the chirality of this iso-spin texture can serve to encode information.
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