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Modelling spin waves in noncollinear antiferromagnets: spin-flop states, spin spirals, skyrmions and antiskyrmions

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 Publication date 2020
  fields Physics
and research's language is English




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Spin waves in antiferromagnetic materials have great potential for next-generation magnonic technologies. However, their properties and their dependence on the type of ground-state antiferromagnetic structure are still open questions. Here, we investigate theoretically spin waves in one- and two-dimensional model systems with a focus on noncollinear antiferromagnetic textures such as spin spirals and skyrmions of opposite topological charges. We address in particular the nonreciprocal spin excitations recently measured in bulk antiferromagnet $alpha$--$text{Cu}_2text{V}_2text{O}_7$ utilizing inelastic neutron scattering experiments [Phys. Rev. Lett. textbf{119}, 047201 (2017)], where we help to characterize the nature of the detected spin-wave modes. Furthermore, we discuss how the Dzyaloshinskii-Moriya interaction can lift the degeneracy of the spin-wave modes in antiferromagnets, resembling the electronic Rashba splitting. We consider the spin-wave excitations in antiferromagnetic spin-spiral and skyrmion systems and discuss the features of their inelastic scattering spectra. We demonstrate that antiskyrmions can be obtained with an isotropic Dzyaloshinskii-Moriya interaction in certain antiferromagnets.

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Optically induced spin currents have proven to be useful in spintronics applications, allowing for sub-ps all-optical control of magnetization. However, the mechanism responsible for their generation is still heavily debated. Here we use the excitation of spin-current induced THz spin-waves in noncollinear bilayer structures to directly study optical spin-currents in the time domain. We measure a significant laser-fluence dependence of the spin-wave phase, which can quantitatively be explained assuming the spin current is proportional to the time derivative of the magnetization. Measurements of the absolute spin-wave phase, supported by theoretical calculations and micromagnetic simulations, suggest that a simple ballistic transport picture is sufficient to properly explain spin transport in our experiments and that the damping-like optical STT dominates THz spin-wave generation. Our findings suggest laser-induced demagnetization and spin-current generation share the same microscopic origin.
The classical spin-flop is the field-driven first-order reorientation transition in easy-axis antiferromagnets. A comprehensive phenomenological theory of easy-axis antiferromagnets displaying spin-flops is developed. It is shown how the hierarchy of magnetic coupling strengths in these antiferromagnets causes a strongly pronounced two-scale character in their magnetic phase structure. In contrast to the major part of the magnetic phase diagram, these antiferromagnets near the spin-flop region are described by an effective model akin to uniaxial ferromagnets. For a consistent theoretical description both higher-order anisotropy contributions and dipolar stray-fields have to be taken into account near the spin-flop. In particular, thermodynamically stable multidomain states exist in the spin-flop region, owing to the phase coexistence at this first-order transition. For this region, equilibrium spin-configurations and parameters of the multidomain states are derived as functions of the external magnetic field. The components of the magnetic susceptibility tensor are calculated for homogeneous and multidomain states in the vicinity of the spin-flop. The remarkable anomalies in these measurable quantities provide an efficient method to investigate magnetic states and to determine materials parameters in bulk and confined antiferromagnets, as well as in nanoscale synthetic antiferromagnets. The method is demonstrated for experimental data on the magnetic properties near the spin-flop region in the orthorhombic layered antiferromagnet (C_2H_5NH_3)_2CuCl_4.
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