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Register a new userSingle-shot d-scan technique for ultrashort laser pulse characterization using transverse second-harmonic generation in random nonlinear crystals
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Added by
\\'I\\~nigo J. Sola
Publication date
2020
fields
Physics
and research's language is
English
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We demonstrate a novel dispersion-scan (d-scan) scheme for single-shot temporal characterization of ultrashort laser pulses. The novelty of this method relies on the use of a highly dispersive crystal featuring antiparallel nonlinear domains with a random distribution and size. This crystal, capable of generating a transverse second-harmonic signal, acts simultaneously as the dispersive element and the nonlinear medium of the d-scan device. The resulting in-line architecture makes the technique very simple and robust, allowing the acquisition of single-shot d-scan traces in real time. In addition, the technique can be further simplified by avoiding the need of dispersion pre-compensation. The retrieved pulses are in very good agreement with independent FROG measurements. We also apply the new single-shot d-scan to a TW-class laser equipped with a programmable pulse shaper, obtaining an excellent agreement between the applied and the d-scan retrieved dispersions.
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Direct generation of ultrashort, transform-limited pulses in a laser resonator is observed theoretically and experimentally. This constitutes a new type of ultrashort pulse generation in mode-locked lasers: in contrast to the well-known solitons (hyperbolic secant like), dispersion-managed solitons (Gaussian-like), and parabolic pulses plus external compression, ultrashort pulse solutions to the nonlinear wave equations that describe pulse evolution in the laser cavity are observed. Stable ultrashort, transform-limited pulses exist with optical spectrum broader than the gain bandwidth of the amplifier, and this has practical application for other lasers.
The dispersion scan (d-scan) technique has emerged as a simple-to-implement characterization method for ultrashort laser pulses. D-scan traces are intuitive to interpret and retrieval algorithms that are both fast and robust have been developed to obtain the spectral phase and the temporal pulse profile. Here, we give a review of the d-scan technique based on second harmonic generation. We describe and compare recent implementations for the characterization of few- and multi-cycle pulses as well as two different approaches for recording d-scan traces in single-shot, thus showing the versatility of the technique.
We report the observations of unexpected layer-dependent, strong, and anisotropic second harmonic generations (SHGs) in atomically thin ReS2. Appreciable (negligible) SHGs are obtained from even (odd) numbers of ReS2 layers, which is opposite to the layer-dependence of SHGs in group VI transition metal dichalcogenides, such as MoS2 and WS2. The results are analyzed from ReS2s crystal structure, implying second harmonic polarizations generated from the interlayer coupling. Pumped by a telecomband laser, SHG from the bilayer ReS2 is almost one order of magnitude larger than that from the monolayer WS2. The estimated second-order nonlinear susceptibility of 900 pm/V is remarkably high among those reported in two-dimensional materials. The laser polarization dependence of ReS2s SHG is strongly anisotropic and indicates its distorted lattice structure with more unequal and non-zero second-order susceptibility elements.
On the basis of the Edward-Kornfeld formulation, we study the effective susceptibility of secondharmonic generation (SHG) in colloidal crystals, which are made of graded metallodielectric nanoparticles with an intrinsic SHG susceptibility suspended in a host liquid. We find a large enhancement and redshift of SHG responses, which arises from the periodic structure, local field effects and gradation in the metallic cores. The optimization of the Ewald-Kornfeld formulation is also investigated.
We demonstrate supermode-based second harmonic generation in an integrated nonlinear interferometer made of linear and nonlinear directional couplers. We use a fully-fibered pump shaper to demonstrate second harmonic generation pumped by the symmetric or anti- symmetric fundamental spatial modes. The selection of the pumping mode and thus of a specific SHG spectral profile is achieved through the selection of the fundamental wavelength and via a robust phase setting scheme. We use two methods: either post-selecting or actively setting the pumping mode. Such a modal phase matching paves the way for classical and quantum applications of coupled nonlinear photonic circuits, where multimode excitation, encoding and detection are a route for multiplexing and scaling up light-processing.
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