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Register a new userStatic and dynamic properties of multi-ionic plasma mixtures
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Complex plasma mixtures with three or more components are often encountered in astrophysics or in inertial confinement fusion (ICF) experiments. For mixtures containing species with large differences in atomic number Z, the modeling needs to consider at the same time the kinetic theory for low-Z elements combined with the theory of strongly coupled plasma for high-Z elements, as well as all the intermediate situations that can appear in multi-component systems. For such cases, we study the pair distribution functions, self-diffusions, mutual diffusion and viscosity for ternary mixtures at extreme conditions. These quantities can be produced from first principles using orbital free molecular dynamics at the computational expense of very intensive simulations to reach good statistics. Utilizing the first-principles results as reference data, we assess the merit of a global analytic model for transport coefficients, Pseudo-Ions in Jellium (PIJ), based on an iso-electronic assumption ( iso-n e ). With a multi-component hypernetted-chain integral equation, we verify the quality of the iso-n e prescription for describing the static structure of the mixtures. This semi-analytical modeling compares well with the simulation results and allows one to consider plasma mixtures not accessible to simulations. Applications are given for the mix of materials in ICF experiments. A reduction of a multicomponent mixture to an effective binary mixture is also established in the hydrodynamic limit and compared with PIJ estimations for ICF relevant mixtures.
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Using the results of extensive Monte Carlo simulations we discuss corrections to the linear mixing rule in strongly coupled binary ionic mixtures. We analyze the plasma screening function at zero separation, H_{jk}(0), for two ions (of types j=1,2 and k=1,2) in a strongly coupled binary mixture. The function H_{jk}(0) is estimated by two methods: (1) from the difference of Helmholtz Coulomb free energies at large and zero separations; (2) by fitting the Widom expansion of H_{jk}(x) in powers of interionic distance x to Monte Carlo data on the radial pair distribution function g_{jk}(x). These methods are shown to be in good agreement. For illustration, we analyze the plasma screening enhancement of nuclear burning rates in dense stellar matter.
It is well-known that room temperature ionic liquids (RTILs) often adopt a charge-separated layered structure, i.e., with alternating cation- and anion-rich layers, at electrified interfaces. However, the dynamic response of the layered structure to temporal variations in applied potential is not well understood. We used in situ, real-time X-ray reflectivity (XR) to study the potential-dependent electric double layer (EDL) structure of an imidazolium-based RTIL on charged epitaxial graphene during potential cycling as a function of temperature. The results suggest that the graphene-RTIL interfacial structure is bistable in which the EDL structure at any intermediate potential can be described by the combination of two extreme-potential structures whose proportions vary depending on the polarity and magnitude of the applied potential. This picture is supported by the EDL structures obtained by fully atomistic molecular dynamics (MD) simulations at various static potentials. The potential-driven transition between the two structures is characterized by an increasing width but with an approximately fixed hysteresis magnitude as a function of temperature. The results are consistent with the coexistence of distinct anion and cation adsorbed structures separated by an energy barrier (~0.15 eV).
We develop analytic approximations of thermodynamic functions of fully ionized nonideal electron-ion plasma mixtures. In the regime of strong Coulomb coupling, we use our previously developed analytic approximations for the free energy of one-component plasmas with rigid and polarizable electron background and apply the linear mixing rule (LMR). Other thermodynamic functions are obtained through analytic derivation of this free energy. In order to obtain an analytic approximation for the intermediate coupling and transition to the Debye-Hueckel limit, we perform hypernetted-chain calculations of the free energy, internal energy, and pressure for mixtures of different ion species and introduce a correction to the LMR, which allows a smooth transition from strong to weak Coulomb coupling in agreement with the numerical results.
The paper presents a review of dynamic stabilization mechanisms for plasma instabilities. One of the dynamic stabilization mechanisms for plasma instability was proposed in the papers [Phys. Plasmas 19, 024503(2012) and references therein], based on a perturbation phase control. In general, instabilities emerge from the perturbations of the physical quantity. Normally the perturbation phase is unknown so that the instability growth rate is discussed. However, if the perturbation phase is known, the instability growth can be controlled by a superimposition of perturbations imposed actively: if the perturbation is introduced by, for example, a driving beam axis oscillation or so, the perturbation phase can be controlled and the instability growth is mitigated by the superimposition of the growing perturbations. Based on this mechanism we present the application results of the dynamic stabilization mechanism to the Rayleigh-Taylor (R-T) instability and to the filamentation instability as typical examples in this paper. On the other hand, in the paper [Comments Plasma Phys. Controlled Fusion 3, 1(1977)] another mechanism was proposed to stabilize the R-T instability based on the strong oscillation of acceleration, which was realized by the laser intensity modulation in laser inertial fusion [Phys. Rev. Lett. 71, 3131(1993)]. In the latter mechanism, the total acceleration strongly oscillates, so that the additional oscillating force is added to create a new stable window in the system. Originally the latter mechanism was proposed by P. L. Kapitza, and it was applied to the stabilization of an inverted pendulum. In this paper we review the two dynamic stabilization mechanisms, and present the application results of the former dynamic stabilization mechanism.
Recently developed analytic approximation for the equation of state of fully ionized nonideal electron-ion plasma mixtures [Potekhin et al., Phys. Rev. E, 79, 016411 (2009); arXiv:0812.4344], which covers the transition between the weak and strong Coulomb coupling regimes and reproduces numerical results obtained in the hypernetted chain (HNC) approximation, is modified in order to fit the small deviations from the linear mixing in the strong coupling regime, revealed by recent Monte Carlo simulations. In addition, a mixing rule is proposed for the regime of weak coupling, which generalizes post-Debye density corrections to the case of mixtures and numerically agrees with the HNC approximation in that regime.
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