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Crystal field Hamiltonian and anisotropy in KErSe2 and CsErSe2

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 Added by Allen Scheie
 Publication date 2020
  fields Physics
and research's language is English




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We use neutron scattering and bulk property measurements to determine the single-ion crystal-field Hamiltonians of delafossites $rm KErSe_2$ and $rm CsErSe_2$. These two systems contains planar equilateral triangular Er lattices arranged in two stacking variants: rhombohedral (for K) or hexagonal (Cs). Our analysis shows that regardless the stacking order both compound exhibit an easy-plane ground state doublet with large $J_z=1/2$ terms and the potential for significant quantum effects, making them candidates for quantum spin liquid or other exotic ground states.

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We investigate the effects of an applied magnetic field on the magnetic properties of the antiferromagnet GdCoIn$_5$. The prominent anisotropy observed in the susceptibility below $T_N$ is rapidly suppressed by a field of just a few Tesla. Further evidence of this low energy-scale is obtained from magnetoresistance and magnetostriction experiments. The lattice lenght, particulary, shows a sudden change below 2 Tesla when the magnetic field is applied perpendicular to the crystallographic $hat{c}$-axis. The experimental results as a whole can be attributed to a small but non negligible higher-order crystalline electric field.
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