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The Kitaev model is a beautiful example of frustrated interactions giving rise to deep and unexpected phenomena. In particular, its classical version has remarkable properties stemming from exponentially large ground state degeneracy. Here, we present a study of magnetic clusters with spin-$S$ moments coupled by Kitaev interactions. We focus on two cluster geometries -- the Kitaev square and the Kitaev tetrahedron -- that allow us to explicitly enumerate all classical ground states. In both cases, the classical ground state space (CGSS) is large and self-intersecting, with non-manifold character. The Kitaev square has a CGSS of four intersecting circles that can be embedded in four dimensions. The tetrahedron CGSS consists of eight spheres embedded in six dimensions. In the semi-classical large-$S$ limit, we argue for effective low energy descriptions in terms of a single particle moving on these non-manifold spaces. Remarkably, at low energies, the particle is tied down in bound states formed around singularities at self-intersection points. In the language of spins, the low energy physics is determined by a distinct set of states that lies well below other eigenstates. These correspond to `Cartesian states, a special class of classical ground states that are constructed from dimer covers of the underlying lattice. They completely determine the low energy physics despite being a small subset of the classical ground state space. This provides an example of order by singularity, where state selection becomes stronger upon approaching the classical limit.
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We identify and discuss the ground state of a quantum magnet on a triangular lattice with bond-dependent Ising-type spin couplings, that is, a triangular analog of the Kitaev honeycomb model. The classical ground-state manifold of the model is spanned by decoupled Ising-type chains, and its accidental degeneracy is due to the frustrated nature of the anisotropic spin couplings. We show how this subextensive degeneracy is lifted by a quantum order-by-disorder mechanism and study the quantum selection of the ground state by treating short-wavelength fluctuations within the linked cluster expansion and by using the complementary spin-wave theory. We find that quantum fluctuations couple next-nearest-neighbor chains through an emergent four-spin interaction, while nearest-neighbor chains remain decoupled. The remaining discrete degeneracy of the ground state is shown to be protected by a hidden symmetry of the model.
Geometrically frustrated quantum impurities coupled to metallic leads have been shown to exhibit rich behavior with a quantum phase transition separating Kondo screened and local moment phases. Frustration in the quantum impurity can alternatively be introduced via Kitaev-couplings between different spins of the impurity cluster. We use the Numerical Renormalization Group (NRG) to study a range of systems where the quantum impurity comprising a Kitaev cluster is coupled to a bath of non-interacting fermions. The models exhibits a competition between Kitaev and Kondo dominated physics depending on whether the Kitaev couplings are greater or less than the Kondo temperature. We characterize the ground state properties of the system and determine the temperature dependence of the crossover scale for the emergence of fractionalized degrees of freedom in the model. We also demonstrate qualitatively as well as quantitatively that in the Kondo limit, the complex impurity can be mapped to an effective two-impurity system, where the emergent spin $1/2$ comprises of both Majorana and flux degrees of freedom. For a tetrahedral-shaped Kitaev cluster, an extra orbital degree of freedom closely related to a flux degree of freedom remains unscreened even in the presence of both Heisenberg and Kondo interactions.
We show that the topological Kitaev spin liquid on the honeycomb lattice is extremely fragile against the second-neighbor Kitaev coupling $K_2$, which has recently been shown to be the dominant perturbation away from the nearest-neighbor model in iridate Na$_2$IrO$_3$, and may also play a role in $alpha$-RuCl$_3$ and Li$_2$IrO$_3$. This coupling naturally explains the zigzag ordering (without introducing unrealistically large longer-range Heisenberg exchange terms) and the special entanglement between real and spin space observed recently in Na$_2$IrO$_3$. Moreover, the minimal $K_1$-$K_2$ model that we present here holds the unique property that the classical and quantum phase diagrams and their respective order-by-disorder mechanisms are qualitatively different due to the fundamentally different symmetries of the classical and quantum counterparts.
A quantum spin-liquid might be realized in $alpha$-RuCl$_{3}$, a honeycomb-lattice magnetic material with substantial spin-orbit coupling. Moreover, $alpha$-RuCl$_{3}$ is a Mott insulator, which implies the possibility that novel exotic phases occur upon doping. Here, we study the electronic structure of this material when intercalated with potassium by photoemission spectroscopy, electron energy loss spectroscopy, and density functional theory calculations. We obtain a stable stoichiometry at K$_{0.5}$RuCl$_3$. This gives rise to a peculiar charge disproportionation into formally Ru$^{2+}$ (4$d^6$) and Ru$^{3+}$ (4$d^5$). Every Ru 4$d^5$ site with one hole in the $t_{2g}$ shell is surrounded by nearest neighbors of 4$d^6$ character, where the $t_{2g}$ level is full and magnetically inert. Thus, each type of Ru sites forms a triangular lattice and nearest-neighbor interactions of the original honeycomb are blocked.
Magnetic systems with frustration often have large classical degeneracy. We show that their low-energy physics can be understood as dynamics within the space of classical ground states. We demonstrate this mapping in a family of quantum spin clusters where every pair of spins is connected by an $XY$ antiferromagnetic bond. The dimer with two spin-$S$ spins provides the simplest example, it maps to a quantum particle on a ring ($S^1$). The trimer is more complex, equivalent to a particle that lives on two disjoint rings ($S^1otimes mathbb{Z}_2$). It has an additional subtlety for half-integer $S$ values, wherein both rings must be threaded by $pi$-fluxes to obtain a satisfactory mapping. This is a consequence of the geometric phase incurred by spins. For both the dimer and the trimer, the effective theory can be seen from a path-integral-based derivation. This approach cannot be extended to the quadrumer which has a non-manifold ground state space, consisting of three tori that touch pairwise along lines. In order to understand the dynamics of a particle in this space, we develop a tight-binding model with this connectivity. Remarkably, this successfully reproduces the low-energy spectrum of the quadrumer. For half-integer spins, a geometric phase emerges which can be mapped to two $pi$-flux tubes that reside in the space between the tori. The non-manifold character of the space leads to a remarkable effect - the dynamics at low energies is not ergodic as the particle is localized around singular lines of the ground state space. The low-energy spectrum consists of an extensive number of bound states formed around singularities. Physically, this manifests as an order-by-disorder-like preference for collinear ground states. However, unlike order-by-disorder, this `order by singularity persists even in the classical limit. We discuss consequences for field theoretic studies of magnets.
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