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Register a new userContinuously-tunable light-matter coupling in optical microcavities with 2D semiconductors
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A theoretical variation between the two distinct light-matter coupling regimes, namely weak and strong coupling, becomes uniquely feasible in open optical Fabry-Perot microcavities with low mode volume, as discussed here. In combination with monolayers of transition-metal dichalcogenides (TMDCs) such as WS2, which exhibits a large exciton oscillator strength and binding energy, the room-temperature observation of hybrid bosonic quasiparticles, referred to as exciton-polaritons and characterized by a Rabi splitting, comes into reach. In this context, our simulations using the transfer-matrix method show how to tailor and alter the coupling strength actively by varying the relative field strength at the excitons position - exploiting a tunable cavity length, a transparent PMMA spacer layer and angle-dependencies of optical resonances. Continuously tunable coupling for future experiments is hereby proposed, capable of real-time adjustable Rabi splitting as well as switching between the two coupling regimes. Being nearly independent of the chosen material, the suggested structure could also be used in the context of light-matter-coupling experiments with quantum dots, molecules or quantum wells. While the adjustable polariton energy levels could be utilized for polariton-chemistry or optical sensing, cavities that allow working at the exceptional point promise the exploration of topological properties of that point.
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Quasi-two-dimensional (2D) films of layered metal-chalcogenides have attractive optoelectronic properties. However, photonic applications of thin films may be limited owing to weak light absorption and surface effects leading to reduced quantum yield. Integration of 2D films in optical microcavities will permit these limitations to be overcome owing to modified light coupling with the films. Here we present tunable microcavities with embedded monolayer MoS2 or few monolayer GaSe films. We observe significant modification of spectral and temporal properties of photoluminescence (PL): PL is emitted in spectrally narrow and wavelength-tunable cavity modes with quality factors up to 7400; PL life-time shortening by a factor of 10 is achieved, a consequence of Purcell enhancement of the spontaneous emission rate. This work has potential to pave the way to microcavity-enhanced light-emitting devices based on layered 2D materials and their heterostructures, and also opens possibilities for cavity QED in a new material system of van der Waals crystals.
In this work, we demonstrate that the nonlinear response of certain soft-matter systems can be tailored at will by appropriately engineering their optical polarizability. In particular, we deliberately synthesize stable colloidal suspensions with negative polarizabilities, and observe for the first time robust propagation and enhanced transmission of self-trapped light over long distances that would have been otherwise impossible in conventional suspensions with positive polarizabilities. What greatly facilitates this behavior is an induced saturable nonlinear optical response introduced by the thermodynamic properties of these colloidal systems. This in turn leads to a substantial reduction in scattering via self-activated transparency effects. Our results may open up new opportunities in developing soft-matter systems with tunable optical nonlinearities.
Magnetic nanoparticles (MNPs) exhibiting superparamagnetic properties might generate large magnetic dipole-dipole interaction with electron spins in organic semiconductors (OSECs). This concept could be considered analogous to the effect of hyperfine interaction (HFI). In order to investigate this model, Fe3O4 MNPs are used as a dopant for generating random hyperfine-like magnetic fields in a HFI-dominant {pi}-conjugated polymer host, poly(2-methoxy-5-(2-ethylhexyloxy)-1,4-phenylenevinylene) (MeH-PPV). The magnetoconductance (MC) response in organic light emitting diodes made by MeH-PPV/MNP blends is used to estimate the effective hyperfine field in the blends. Firstly, we find that the shape of the MC response essentially remains the same regardless of the MNP concentration, which is attributed to the similar functionality between the nuclear spins and the MNPs. Secondly, the width of MC increases with increasing MNP concentration. Magneto-optical Kerr effect experiments and micromagnetic simulation indicate that the additional increase of the MC width is associated with the strength of the magnetization of the blend. Finally, the MC broadening has the same temperature dependent trend as the magnetization of the MNPs where the unique effect of the MNPs in their superparamagnetic and ferromagnetic regimes on the MC response is observed. Magneto-photoinduced absorption (MPA) spectroscopy confirms that the MC broadening is not due to defects introduced by the MNPs, but is a result of unique superparamagnetic behavior. Our study yields a new pathway for tuning OSECs magnetic functionality, which is essential to organic optoelectronic devices and magnetic sensor applications.
In this paper, we propose a continuously tunable acoustic metasurface composed of identical anisotropic resonant units, each of which contains a rigid pedestal and a rotatable inclusion with space coiling-up structure. The metasurface can manipulate the reflected phase by adjusting the rotational angle of inclusion. The theoretical analysis shows that the polarization-dependent phase change can be induced by the even-order standing wave modes inside inclusion. By utilizing the rotatable inclusion, we design a tunable acoustic carpet cloaking device, which works with a wide range for incident angle. When incident waves come from different directions, the cloaking effect can be obtained by arrange the rotational angle of each inclusion.
Chiral edge modes in photonic topological insulators host great potential to realize slow-light waveguides with topological protection. Increasing the winding of the chiral edge mode around the Brillouin zone can lead to broadband topological slow light with ultra-low group velocity. However, this effect usually requires careful modifications on a relatively large area around the lattice edge. Here we present a simple and general scheme to achieve broadband topological slow light through coupling the chiral edge modes with flat bands. In this approach, modifications inside the topological lattice are not required. Instead, only several additional resonators that support the flat bands need to be attached at the lattice edge. We demonstrate our idea numerically using a gyromagnetic photonic crystal, which is ready to be tested at microwave frequencies.
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