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Register a new userNumerical simulations of self-diffusiophoretic colloids at fluid interfaces
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Added by
Paolo Malgaretti Mr
Publication date
2019
fields
Physics
and research's language is
English
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The dynamics of active colloids is very sensitive to the presence of boundaries and interfaces which therefore can be used to control their motion. Here we analyze the dynamics of active colloids adsorbed at a fluid-fluid interface. By using a mesoscopic numerical approach which relies on an approximated numerical solution of the Navier-Stokes equation, we show that when adsorbed at a fluid interface, an active colloid experiences a net torque even in the absence of a viscosity contrast between the two adjacent fluids. In particular, we study the dependence of this torque on the contact angle of the colloid with the fluid-fluid interface and on its surface properties. We rationalize our results via an approximate approach which accounts for the appearance of a local friction coefficient. By providing insight into the dynamics of active colloids adsorbed at fluid interfaces, our results are relevant for two-dimensional self assembly and emulsion stabilization by means of active colloids.
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A locally heated Janus colloid can achieve motion in a fluid through the coupling of dissolved ions and the mediums polarizibility to an imposed temperature gradient, an effect known as self-thermo(di)electrophoresis. We numerically study the self-propulsion of such a hot swimmer in a monovalent electrolyte solution using the finite-element method. The effect of electrostatic screening for intermediate and large Debye lengths is charted and we report on the fluid flow generated by self-thermoelectrophoresis. We obtain excellent agreement between our analytic theory and numerical calculations in the limit of high salinity, validating our approach. At low salt concentrations, we consider two analytic approaches and use Teubners integral formalism to arrive at expressions for the speed. These expressions agree semi-quantitatively with our numerical results for conducting swimmers, providing further validation. Our numerical approach provides a solid framework against the strengths and weaknesses of analytic theory can be appreciated and which should benefit the realization and analysis of further experiments on hot swimming.
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