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Register a new userRelevance of magnetism to cuprate superconductivity: Lanthanides versus charge-compensated cuprates
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We address what seemed to be a contradiction between the lanthanide series REBa$_2$Cu$_3$O$_y$ (RE123) and the charge-compensated series (Ca$_{x}$La$_{1-x}$)(Ba$_{1.75-x}$La$_{0.25+x} $)Cu$_{3}$O$_{y}$ (CLBLCO) regarding the superexchange ($J$) dependence of the maximum superconductivity (SC) critical temperature $T_c^{max}(J)$; RE and $x$ are implicit variables. This is done by measuring the N{e}el temperature and the temperature dependence of the magnetic order parameter for RE=Nd, Sm, Eu, Gd, Dy, Yb, Y, and for Y(BaSr)Cu$_3$O$_y$, at various very light dopings. The doping is determined by thermopower, and the magnetic properties by muon spin rotation. We find that the normalized-temperature dependence of the order parameter is identical for all RE123 in the undoped limit (with the exception of Gd123) implying identical out-of-plane magnetic coupling. The extrapolation of $T_N$ to zero doping suggests that, despite the variations in ionic radii, $J$ varies too weakly in this system to test the relation between SC and magnetism. This stands in contrast to CLBLCO where both $T_c^{max}$ and $T_N^{max}$ vary considerably in the undoped limit, and a positive correlation between the two quantities was observed.
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We present a detailed investigation of the electronic phase diagram of effectively charge compensated Ba1-xKx(Fe1-yCoy)2As2 with x/2 = y. Our experimental study by means of x-ray diffraction, Mossbauer spectroscopy, muon spin relaxation and ac susceptibility measurements on polycrystalline samples is complemented by density functional electronic structure calculations. For low substitution levels of x/2 = y < 0.13, the system displays an orthorhombically distorted and antiferromagnetically ordered ground state. The low temperature structural and magnetic order parameters are successively reduced with increasing substitution level. We observe a linear relationship between the structural and the magnetic order parameter as a function of temperature and substitution level for x/2 = y < 0.13. At intermediate substitution levels in the range between 0.13 and 0.19, we find superconductivity with a maximum Tc of 15 K coexisting with static magnetic order on a microscopic length scale. For higher substitution levels x/2 = y > 0.25 a tetragonal non-magnetic ground state is observed. Our DFT calculations yield a signifcant reduction of the Fe 3d density of states at the Fermi energy and a strong suppression of the ordered magnetic moment in excellent agreement with experimental results. The appearance of superconductivity within the antiferromagnetic state can by explained by the introduction of disorder due to non-magnetic impurities to a system with a constant charge carrier density. Our experimental study by means of x-ray diffraction, Mossbauer spectroscopy, muon spin relaxation and ac susceptibility measurements on polycrystalline samples is complemented by density functional electronic structure calculations.
Superconductivity in layered cuprates is induced by doping holes into a parent antiferromagnetic insulator. It is now recognized that another common emergent order involves charge stripes, and our understanding of the relationship been charge stripes and superconductivity has been evolving. Here we review studies of 214 cuprate families obtained by doping La$_2$CuO$_4$. Charge-stripe order tends to compete with bulk superconductivity; nevertheless, there is plentiful evidence that it coexists with two-dimensional superconductivity. This has been interpreted in terms of pair-density-wave superconductivity, and the perspective has shifted from competing to intertwined orders. In fact, a new picture of superconductivity based on pairing within charge stripes has been proposed, as we discuss.
Absolute resistivity measurements as a function of temperature from optimally doped YBa_2Cu_3O_(7), La_(2-x)Sr_xCuO_4, Bi_2Sr_2CaCu_2O_(8-x), and (Ca_0.1La_0.9)(Ba_1.65La_0.35)Cu_3O_y thin films are reported. Special attention is given to the measurement geometrical factors and the resistivity slope between Tc and T^{*}. The results are compared with a strong coupling theory for the resistivity derivative near T_c, which is based on hard core bosons (HCB), and with several weak coupling theories, which are BCS based. Surprisingly, our results agree with both paradigms. The implications of these findings and the missing calculations needed to distinguish between the two paradigms are discussed.
One of the central issues in the recent study of cuprate superconductors is the interplay of charge order with superconductivity. Here the interplay of charge order with superconductivity in cuprate superconductors is studied based on the kinetic-energy-driven superconducting (SC) mechanism by taking into account the intertwining between the pseudogap and SC gap. It is shown that the appearance of the Fermi pockets is closely associated with the emergence of the pseudogap. However, the distribution of the spectral weight of the SC-state quasiparticle spectrum on the Fermi arc, or equivalently the front side of the Fermi pocket, and back side of Fermi pocket is extremely anisotropic, where the most part of the spectral weight is located around the tips of the Fermi arcs, which in this case coincide with the hot spots on the electron Fermi surface (EFS). In particular, as charge order in the normal-state, this EFS instability drives charge order in the SC-state, with the charge-order wave vector that is well consistent with the wave vector connecting the hot spots on the straight Fermi arcs. Furthermore, this charge-order state is doping dependent, with the charge-order wave vector that decreases in magnitude with the increase of doping. Although there is a coexistence of charge order and superconductivity, this charge order antagonizes superconductivity. The results from the SC-state dynamical charge structure factor indicate the existence of a quantitative connection between the low-energy electronic structure and collective response of the electron density. The theory also shows that the pseudogap and charge order have a root in common, they and superconductivity are a natural consequence of the strong electron correlation.
Using a dynamical cluster quantum Monte Carlo approximation, we investigate the effect of local disorder on the stability of d-wave superconductivity including the effect of electronic correlations in both particle-particle and particle-hole channels. With increasing impurity potential, we find an initial rise of the critical temperature due to an enhancement of anti-ferromagnetic spin correlations, followed by a decrease of Tc due to scattering from impurity-induced moments and ordinary pairbreaking. We discuss the weak initial dependence of Tc on impurity concentration found in comparison to experiments on cuprates.
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