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Register a new userThe quest of shape coexistence in Zr isotopes
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Jose Enrique Garc\\'ia-Ramos
Publication date
2019
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English
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The mass region with A~100 and Z~40 is known to experience a sudden onset of deformation. The presence of the subshell closure $Z=40$ makes feasible to create particle-hole excitations at a moderate excitation energy and, therefore, likely intruder states could be present in the low-lying spectrum. In other words, shape coexistence is expected to be a key ingredient to understand this mass region. The aim of this work is to describe excitation energies, transition rates, radii, and two-neutron separation energies for the even-even 94-110Zr nuclei and, moreover, to obtain information about wave functions and deformation. The interacting boson model with configuration mixing will be the framework to study the even-even Zr nuclei, considering only two types of configurations: 0particle-0hole and 2p-2h excitations. On one hand, the parameters appearing in the Hamiltonian and in the E2 transition operator are fixed trough a least-squares fit to the whole available experimental information. On the other hand, once the parameters have been fixed, the calculations allow to obtain a complete set of observables for the whole even-even Zr chain of isotopes. Spectra, transition rates, radii, $rho^2(E0)$, and two-neutron separation energies have been calculated and a good agreement with the experimental information has been obtained. Moreover, a detailed study of the wave function has been conducted and mean-field energy surfaces and deformation have been computed too. The importance of shape coexistence has been shown to correctly describe the A~100 mass area for even-even Zr nuclei. This work confirmed the rather spherical nature of the ground state of 94-98Zr and its deformed nature for 100-110Zr isotopes. The sudden onset of deformation in 100Zr is owing to the rapid lowering of a deformed (intruder) configuration which is high-lying in lighter isotopes.
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The rapid shape change in Zr isotopes near neutron number $N$=60 is identified to be caused by type II shell evolution associated with massive proton excitations to its $0g_{9/2}$ orbit, and is shown to be a quantum phase transition. Monte Carlo shell-model calculations are carried out for Zr isotopes of $N$=50-70 with many configurations spanned by eight proton orbits and eight neutron orbits. Energy levels and B(E2) values are obtained within a single framework in a good agreement with experiments, depicting various shapes in going from $N$=50 to 70. Novel coexistence of prolate and triaxial shapes is suggested.
The goal of this contribution is to analyze the connection between shape coexistence and quantum phase transition, two seemingly unrelated phenomena that share common aspects, namely, the rapid change in the ground state structure along an isotope chain or the presence of several minima at the mean-field level. To illustrate the similarities and differences between both phenomena, we will focus in the Pb region, in particular in Pt and Hg isotopes, as well as in Zr isotopes.
The evolution of the total energy surface and the nuclear shape in the isotopic chain $^{172-194}$Pt are studied in the framework of the interacting boson model, including configuration mixing. The results are compared with a self-consistent Hartree-Fock-Bogoliubov calculation using the Gogny-D1S interaction and a good agreement between both approaches shows up. The evolution of the deformation parameters points towards the presence of two different coexisting configurations in the region 176 $leq$ A $leq$ 186.
Background: The lead region, Po, Pb, Hg, and Pt, shows up the presence of coexisting structures having different deformation and corresponding to different particle-hole configurations in the Shell Model language. Purpose: We intend to study the importance of configuration mixing in the understanding of the nuclear structure of even-even Po isotopes, where the shape coexistence phenomena are not clear enough. Method: We study in detail a long chain of polonium isotopes, 190-208Po, using the interacting boson model with configuration mixing (IBM-CM). We fix the parameters of the Hamiltonians through a least-squares fit to the known energies and absolute B(E2) transition rates of states up to 3 MeV. Results: We obtained the IBM-CM Hamiltonians and we calculate excitation energies, B(E2)s, electric quadrupole moments, nuclear radii and isotopic shifts, quadrupole shape invariants, wave functions, and deformations. Conclusions: We obtain a good agreement with the experimental data for all the studied observables and we conclude that shape coexistence phenomenon is hidden in Po isotopes, very much as in the case of the Pt isotopes.
Background: Zr region is characterized by very rapid changes in the ground state structure of the nuclei. In particular, the onset of deformation when passing from $^{98}$Zr to $^{100}$Zr is one of the fastest ever observed in the nuclear chart. It has been probed both experimental and theoretically that certain low-lying excited states of Zr isotopes own different shapes than the ground state. Purpose: We intend to disentangle the interplay between the sudden changes in the ground state shape, i.e., the existence of a quantum phase transition, and the presence in the spectra of coexisting states with very different deformation, i.e., the presence of shape coexistence. Method: We rely on a previous calculation using the Interacting Boson Model with Configuration Mixing (IBM-CM) which reproduces in detail the spectroscopic properties of $^{96-110}$Zr. This IBM-CM calculation allows to compute mean-field energy surfaces, wave functions and any other observable related with the presence of shape coexistence or with a quantum phase transition. Results: We obtain energy surfaces and the equilibrium value of the deformation parameter $beta$, the U(5) decomposition of the wave functions and the density of states. Conclusions: We confirm that Zr is a clear example of quantum phase transition that originates from the crossing of two configurations with a very different degree of deformation. Moreover, we observe how the intruder configuration exhibits its own evolution which resembles a quantum phase transition too.
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