Unitary transformations are the fundamental building blocks of gates and operations in quantum information processing allowing the complete manipulation of quantum systems in a coherent manner. In the case of photons, optical elements that can perform unitary transformations are readily available only for some degrees of freedom, e.g. wave plates for polarisation. However for high-dimensional states encoded in the transverse spatial modes of light, performing arbitrary unitary transformations remains a challenging task for both theoretical proposals and actual implementations. Following the idea of multi-plane light conversion, we show that it is possible to perform a broad variety of unitary operations when the number of phase modulation planes is comparable to the number of modes. More importantly, we experimentally implement several high-dimensional quantum gates for up to 5-dimensional states encoded in the full-field mode structure of photons. In particular, we realise cyclic and quantum Fourier transformations, known as Pauli $hat{X}$-gates and Hadamard $hat{H}$-gates, respectively, with an average visibility of more than 90%. In addition, we demonstrate near-perfect unitarity by means of quantum process tomography unveiling a process purity of 99%. Lastly, we demonstrate the benefit of the two independent spatial degrees of freedom, i.e. azimuthal and radial, and implement a two-qubit controlled-NOT quantum operation on a single photon. Thus, our demonstrations open up new paths to implement high-dimensional quantum operations, which can be applied to various tasks in quantum communication, computation and sensing schemes.
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