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Register a new userNonclassical optical properties of mesoscopic gold
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Gold nanostructures have important applications in nanoelectronics, nano-optics as well as in precision metrology due to their intriguing opto-electronic properties. These properties are governed by the bulk band structure but to some extend are tunable via geometrical resonances. Here we show that the band structure of gold itself exhibits significant size-dependent changes already for mesoscopic critical dimensions below 30 nm. To suppress the effects of geometrical resonances and grain boundaries, we prepared atomically flat ultrathin films of various thicknesses by utilizing large chemically grown single-crystalline gold platelets. We experimentally probe thickness-dependent changes of the band structure by means of two-photon photoluminescence and observe a surprising 100-fold increase of the nonlinear signal when the gold film thickness is reduced below 30 nm allowing us to optically resolve single-unit-cell steps. The effect is well explained by density functional calculations of the thickness-dependent 2D band structure of gold.
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The energy levels of a quasi-continuous spectrum in mesoscopic systems fluctuate in positions, and the distribution of the fluctuations reveals information about the microscopic nature of the structure under consideration. Here, we investigate mesoscopic fluctuations of the secondary smile gap, that appears in the quasiclassical spectrum of a chaotic cavity coupled to one or more superconductors. Utilizing a random matrix model, we compute numerically the energies of Andreev levels and access the distribution of the gap widths. We mostly concentrate on the universal regime $E_{mathrm{Th}}ggDelta$ with $E_{mathrm{Th}}$ being the Thouless energy of the cavity and $Delta$ being the superconducting gap. We find that the distribution is determined by an intermediate energy scale $Delta_g$ with the value between the level spacing in the cavity $delta_s$ and the quasiclassical value of the gap $E_g$. From our numerics we extrapolate the first two cumulants of the gap distribution in the limit of large level and channel number. We find that the scaled distribution in this regime is the Tracy-Widom distribution: the same as found by Vavilov at al. [Phys. Rev. Lett. textbf{86}, 874 (2001)] for the distribution of the minigap edge in the opposite limit $E_{mathrm{Th}}ll Delta$. This leads us to the conclusion that the distribution found is a universal property of chaotic proximity systems at the edge of a continuous spectrum.
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