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Weak measurement (WM) with state pre- and post-selection can amplify otherwise undetectable small signals and thus promise great potentials in precision measurements. Although frequency measurements offer the hitherto highest precision owing to stable narrow atomic transitions, it remains a long-standing interest to develop new schemes to further escalate their performance. Here, we propose and demonstrate a WM-enhanced spectroscopy technique which is capable of narrowing the resonance to 0.1 Hz in a room-temperature atomic vapor cell. Potential of this technique for precision measurement is demonstrated through weak magnetic field sensing. By judiciously pre- and post-selecting frequency-modulated input and output optical states in a nearly-orthogonal manner, a sensitivity of $text{7 fT/}sqrt{text{Hz}}$ near DC is achieved, using only one laser beam of $text{7 }text{mu W}$ power. Additionally, our results extend the WM framework to a non-Hermitian Hamiltonian, and shed new light in metrology and bio-magnetic field sensing applications.
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Optical interferometers with suspended mirrors are the archetype of all current audio-frequency gravitational-wave detectors. The radiation pressure interaction between the motion of the mirror and the circulating optical field in such interferometers represents a pristine form of light-matter coupling, largely due to 30 years of effort in developing high quality optical materials with low mechanical dissipation. However, in all current suspended interferometers, the radiation pressure interaction is too weak to be useful as a resource, and too strong to be neglected. Here, we demonstrate a meter-long interferometer with suspended mirrors, of effective mass $~ 125$ g, where the radiation pressure interaction is enhanced by strong optical pumping to realize a cooperativity of $50$. We probe this regime by observing optomechanically-induced transparency of a weak on-resonant probe. The low resonant frequency and high-Q of the mechanical oscillator allows us to demonstrate transparency windows barely $100$ mHz wide at room temperature. Together with a near-unity ($sim 99.9%$) out-coupling efficiency, our system saturates the theoretical delay-bandwidth product, rendering it an optical buffer capable of seconds-long storage times.
To date no experiment has reached the level of sensitivity required to observe weak nuclear force induced parity violation (PV) energy differences in chiral molecules. In this paper, we present the approach, adopted at Laboratoire de Physique des Lasers (LPL), to measure frequency differences in the vibrational spectrum of enantiomers. We review different spectroscopic methods developed at LPL leading to the highest resolutions, as well as 20 years of CO2 laser stabilization work enabling such precise measurements. After a first attempt to observe PV vibrational frequency shifts using sub-Doppler saturated absorption spectroscopy in a cell, we are currently aiming at an experiment based on Doppler-free two-photon Ramsey interferometry on a supersonic beam. We report on our latest progress towards observing PV with chiral organo-metallic complexes containing a heavy rhenium atom.
The problem of Freeman resonances [R. R. Freeman textit{et al.}, Phys. Rev. Lett. textbf{59}, 1092 (1987)] when strong field ionization is enhanced due to the transient population of excited states during the ionization, is revisited. An intuitive model is put forward which explains the mechanism of the intermediate population of excited states during nonadiabatic tunneling ionization via the under-the-barrier recollision and recombination. The theoretical model is based on perturbative strong-field approximation (SFA), where the sub-barrier bound-continuum-bound pathway is described in the second-order SFA, while the further ionization from the excited state by an additional perturbative step. The enhancement of ionization is shown to arise due to the constructive interference of contributions into the excitation amplitudes originating from different laser cycles. The applied model provides an intuitive understanding of the electron dynamics during a Freeman resonance in strong-field ionization, as well as means of enhancing the process and possible applications to related processes.
We demonstrate a novel approach to obtain resonance linewidth below that limited by coherence lifetime. Cross correlation between induced intensity modulation of two lasers coupling the target resonance exhibits a narrow spectrum. 1/30 of the lifetime-limited width was achieved in a proof-of-principle experiment where two ground states are the target resonance levels. Attainable linewidth is only limited by laser shot noise in principle. Experimental results agree with an intuitive analytical model and numerical calculations qualitatively. This technique can be easily implemented and should be applicable to many atomic, molecular and solid state spin systems for spectroscopy, metrology and resonance based sensing and imaging.
We propose an efficient scheme for the generation and the manipulation of Raman fields in an homogeneously broadened atomic vapor in a closed three levels $Lambda$-configuration. The key concept in generating the Raman and sub-Raman fields efficiently at lower optical densities involve the microwave induced atomic coherence of the lower levels. We show explicitly that, generation efficiency of the Raman fields can be controlled by manipulating the coherences via phase and amplitude of the microwave field.
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