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Orbital angular momentum from semiconductor high-order harmonics

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 Added by David Gauthier
 Publication date 2018
  fields Physics
and research's language is English




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Light beams carrying orbital angular momentum (OAM) have led to stunning applications in various fields from quantum information to microscopy. In this letter, we examine OAM from the recently discovered high-harmonic generation (HHG) in semiconductor crystals. HHG from solids could be a valuable approach for integrated high-flux short-wavelength coherent light sources. The solid state nature of the generation medium allows the possibility to tailor directly the radiation at the source of the emission and offers a substantial degree of freedom for spatial beam shaping. First, we verify the fundamental principle of the transfer and conservation of the OAM from the generation laser to the harmonics. Second, we create OAM beams by etching a spiral zone structure directly at the surface of a zinc oxide crystal. Such diffractive optics act on the generated harmonics and produces focused optical vortices with nanometer scale sizes that may have potential applications in nanoscale optical trapping and quantum manipulation.

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Optical vortices are currently one of the most intensively studied topics in optics. These light beams, which carry orbital angular momentum (OAM), have been successfully utilized in the visible and infrared in a wide variety of applications. Moving to shorter wavelengths may open up completely new research directions in the areas of optical physics and material characterization. Here, we report on the generation of extreme-ultraviolet optical vortices with femtosecond duration carrying a controllable amount of OAM. From a basic physics viewpoint, our results help to resolve key questions such as the conservation of angular momentum in highly-nonlinear light-matter interactions, and the disentanglement and independent control of the intrinsic and extrinsic components of the photons angular momentum at short-wavelengths. The methods developed here will allow testing some of the recently proposed concepts such as OAM-induced dichroism, magnetic switching in organic molecules, and violation of dipolar selection rules in atoms.
100 - F. Kong , C. Zhang , H. Larocque 2018
The interplay between spin and orbital angular momentum in the up-conversion process allows us to control the macroscopic wave front of high harmonics by manipulating the microscopic polarizations of the driving field. We demonstrate control of orbital angular momentum in high harmonic generation from both solid and gas phase targets using the selection rules of spin angular momentum. The gas phase harmonics extend the control of angular momentum to extreme-ultraviolet wavelength. We also propose a bi-color scheme to produce spectrally separated extreme-ultraviolet radiation carrying orbital angular momentum.
Manipulation of orbital angular momentum (OAM) of light is essential in OAM-based optical systems. Especially, OAM divider, which can convert the incoming OAM mode into one or several new smaller modes in proportion at different spatial paths, is very useful in OAM-based optical networks. However, this useful tool was never reported yet. For the first time, we put forward a passive OAM divider based on coordinate transformation. The device consists of a Cartesian to log-polar coordinate converter and an inverse converter. The first converter converts the OAM light into a rectangular-shaped plane light with a transverse phase gradient. And the second converter converts the plane light into multiple diffracted light. The OAM of zeroth-order diffracted light is the product of the input OAM and the scaling parameter. The residual light is output from other diffracted orders. Furthermore, we extend the scheme to realize equal N-dividing of OAM and arbitrary dividing of OAM. The ability of dividing OAM shows huge potential for OAM-based classical and quantum information processing.
Nanoscale amplification of non-linear processes in solid-state devices opens novel applications in nano-electronics, nano-medicine or high energy conversion for example. Coupling few nano-joules laser energy at a nanometer scale for strong field physics is demonstrated. We report enhancement of high harmonic generation in nano-structured semiconductors using nanoscale amplification of a mid-infrared laser in the sample rather than using large laser amplifier systems. Field amplification is achieved through light confinement in nano-structured semiconductor 3D waveguides. The high harmonic nano-converter consists of an array of zinc-oxide nanocones. They exhibit a large amplification volume, 6 orders of magnitude larger than previously reported and avoid melting observed in metallic plasmonic structures. The amplification of high harmonics is observed by coupling only 5-10 nano-joules of a 3.2 {mu}m high repetition-rate OPCPA laser at the entrance of each nanocone. Harmonic amplification (factor 30) depends on the laser energy input, wavelength and nanocone geometry.
Lights orbital angular momentum (OAM) is an unbounded degree of freedom emerging in helical beams that appears very advantageous technologically. Using a chiral microlaser, i.e. an integrated device that allows generating an emission carrying a net OAM, we demonstrate a regime of bistability involving two modes presenting distinct OAM (L = 0 and L = 2). Furthermore, thanks to an engineered spin-orbit coupling of light in the device, these modes also exhibit distinct polarization patterns, i.e. cirular and azimuthal polarizations. Using a dynamical model of rate euqations, we show that this bistability arises from polarization-dependent saturation of the gain medium. Such a bistable regime appears very promising for implementing ultrafast optical switches based on the OAM of light. As well, it paves the way to the exploration of dynamical processes involving phase and polarization vortices.
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