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Register a new userCoherent Control of Penning and Associative Ionization: Insights from Symmetries
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Added by
Juan Jos\\'e Omiste
Publication date
2018
fields
Physics
and research's language is
English
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Coherent control of reactive atomic and molecular collision processes remains elusive experimentally due to quantum interference-based requirements. Here, with insights from symmetry conditions, a viable method for controlling Penning and Associative ionization in atomic collisions is proposed. Computational applications to He$^*({}^3text{S})$-Li(${^2text{S}}$) and Ne$^*{}(^3text{P}_2$)-Ar($^1text{S}_0$) show extensive control over the ionization processes under experimentally feasible conditions.
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We explore coherent control of Penning and associative ionization in cold collisions of metastable He$^*({2}^3text{S})$ atoms via the quantum interference between different states of the He$_2^*$ collision complex. By tuning the preparation coefficients of the initial atomic spin states, we can benefit from the quantum interference between molecular channels to maximize or minimize the cross sections for Penning and associative ionization. In particular, we find that we can enhance the ionization ratio by 30% in the cold regime. This work is significant for the coherent control of chemical reactions in the cold and ultracold regime.
We show that quantum interference-based coherent control is a highly efficient tool for tuning ultracold molecular collision dynamics, and is free from the limitations of commonly used methods that rely on external electromagnetic fields. By varying {the relative populations and} phases of an initial coherent superpositions of degenerate molecular states, we demonstrate complete coherent control over integral scattering cross sections in the ultracold $s$-wave regime of both the initial and final collision channels. The proposed control methodology is applied to ultracold O$_2$~+~O$_2$ collisions, showing extensive control over $s$-wave spin-exchange cross sections and product branching ratios over many orders of magnitude.
Quantum entanglement between an arbitrary number of remote qubits is examined analytically. We show that there is a non-probabilistic way to address in one context the management of entanglement of an arbitrary number of mixed-state qubits by engaging quantitative measures of entanglement and a specific external control mechanism. Both all-party entanglement and weak inseparability are considered. We show that for $Nge4$, the death of all-party entanglement is permanent after an initial collapse. In contrast, weak inseparability can be deterministically managed for an arbitrarily large number of qubits almost indefinitely. Our result suggests a picture of the path that the system traverses in the Hilbert space.
Penning ionization reactions in merged beams with precisely controlled collision energies have been shown to accurately probe quantum mechanical effects in reactive collisions. A complete microscopic understanding of the reaction is, however, faced with two major challenges---the highly excited character of the reactions entrance channel and the limited precision of even the best state-of-the-art ab initio potential energy surfaces. Here, we suggest photoassociation spectroscopy as a tool to identify the character of orbiting resonances in the entrance channel and probe the ionization width as a function of inter-particle separation. We introduce the basic concept and discuss the general conditions under which this type of spectroscopy will be successful.
The new generation of planar Penning traps promises to be a flexible and versatile tool for quantum information studies. Here, we propose a fully controllable and reversible way to change the typical trapping harmonic potential into a double-well potential, in the axial direction. In this configuration a trapped particle can perform coherent oscillations between the two wells. The tunneling rate, which depends on the barrier height and width, can be adjusted at will by varying the potential difference applied to the trap electrodes. Most notably, tunneling rates in the range of kHz are achievable even with a trap size of the order of 100 microns.
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