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Register a new userThe generation of warm dense matter using a magnetic anvil cell
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Added by
Pierre-Alexandre Gourdain
Publication date
2018
fields
Physics
and research's language is
English
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Warm dense matter is present at the heart of gas giants and large exo-planets. Yet, its most basic properties are unknown and limit our understanding of planetary formation and evolution. In this state, where pressure climbs above 1 Mbar, matter is strongly coupled and quantum degenerate. This combination invalidates most theories capable of predicting the equation of state, the viscosity or heat conductivity of the material. When such properties are missing, understanding planetary evolution becomes an arduous endeavor. Henceforth, research in this field is actively growing, using high power laser or heavy ion beams to produce samples dense enough to overcome the 1 Mbar limit. These samples are not actively confined and tend to expand rapidly, precluding the existence of any thermodynamically stable equilibrium. However, a mega-ampere-class pulsed-power generator can produce confined matter in the Mbar range, providing two conditions are being met. First, the sample needs to be compressed cylindrically, to maximize magnetic pressure (compared to slab compression). Second, a damper must be used to preclude the formation of a corona around the sample. This corona robs the main sample from valuable current and limits the homogeneity of the compression. According to numerical simulations, the setup proposed here, and called a magnetic anvil cell, can reach pressure on the order of 1 Mbar using a mega-ampere pulsed power driver. These samples span several millimeters in length. Unlike diamond anvil cell, which pressure is limited below 1 Mbar due to materials strength, the magnetic anvil cell has virtually no pressure limit. Further, the current heats the sample to several eV, a temperature well beyond diamond anvil cell capabilities.
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Warm dense matter is difficult to generate since it corresponds to a state of matter which pressure is order of magnitude larger than can be handled by natural materials. A diamond anvil can be used to pressurize matter up to one Gbar, this matter is at high density but at room temperature. High power lasers and heavy ion beams can generate warm dense matter but they cannot confine it long enough to allow measurements of quasi-static transport coefficients such as viscosity or heat conduction. We present here a third method to generate warm dense matter. It uses a pulsed-power driver which current rise time is substantially shortened by using a plasma opening switch, limiting the development of electrothermal instabilities. The switch relies on the implosion of a gas puff Z-pinch which carries most of the discharge current until the pinch reaches the sample. After that, the sample is compressed until it reaches the warm dense matter regime. Three-dimensional magnetohydrodynamics computations show that if the density of the gas is low enough no detectable instabilities (e.g. kinks and sausages modes) impede the remainder of the implosion.
Warm dense matter (WDM) -- an exotic state of highly compressed matter -- has attracted high interest in recent years in astrophysics and for dense laboratory systems. At the same time, this state is extremely difficult to treat theoretically. This is due to the simultaneous appearance of quantum degeneracy, Coulomb correlations and thermal effects, as well as the overlap of plasma and condensed phases. Recent breakthroughs are due to the successful application of density functional theory (DFT) methods which, however, often lack the necessary accuracy and predictive capability for WDM applications. The situation has changed with the availability of the first textit{ab initio} data for the exchange-correlation free energy of the warm dense uniform electron gas (UEG) that were obtained by quantum Monte Carlo (QMC) simulations, for recent reviews, see Dornheim textit{et al.}, Phys. Plasmas textbf{24}, 056303 (2017) and Phys. Rep. textbf{744}, 1-86 (2018). In the present article we review recent further progress in QMC simulations of the warm dense UEG: namely, textit{ab initio} results for the static local field correction $G(q)$ and for the dynamic structure factor $S(q,omega)$. These data are of key relevance for the comparison with x-ray scattering experiments at free electron laser facilities and for the improvement of theoretical models. In the second part of this paper we discuss simulations of WDM out of equilibrium. The theoretical approaches include Born-Oppenheimer molecular dynamics, quantum kinetic theory, time-dependent DFT and hydrodynamics. Here we analyze strengths and limitations of these methods and argue that progress in WDM simulations will require a suitable combination of all methods. A particular role might be played by quantum hydrodynamics, and we concentrate on problems, recent progress, and possible improvements of this method.
We present a model for electron-ion transport in Warm Dense Matter that incorporates Coulomb coupling effects into the quantum Boltzmann equation of Uehling and Uhlenbeck through the use of a statistical potential of mean force. Although this model has been derived rigorously in the classical limit [S.D. Baalrud and J. Daligault, Physics of Plasmas 26, 8, 082106 (2019)], its quantum generalization is complicated by the uncertainty principle. Here we apply an existing model for the potential of mean force based on the quantum Ornstein-Zernike equation coupled with an average-atom model [C. E. Starrett, High Energy Density Phys. 25, 8 (2017)]. This potential contains correlations due to both Coulomb coupling and exchange, and the collision kernel of the kinetic theory enforces Pauli blocking while allowing for electron diffraction and large-angle collisions. By solving the Uehling-Uhlenbeck equation for electron-ion relaxation rates, we predict the momentum and temperature relaxation time and electrical conductivity of solid density aluminum plasma based on electron-ion collisions. We present results for density and temperature conditions that span the transition from classical weakly-coupled plasma to degenerate moderately-coupled plasma. Our findings agree well with recent quantum molecular dynamics simulations.
Exploring and understanding ultrafast processes at the atomic level is a scientific challenge. Femtosecond X-ray Absorption Spectroscopy (XAS) is an essential experimental probing technic, as it can simultaneously reveal both electronic and atomic structures, and thus unravel their non-equilibrium dynamic interplay which is at the origin of most of the ultrafast mechanisms. However, despite considerable efforts, there is still no femtosecond X-ray source suitable for routine experiments. Here we show that betatron radiation from relativistic laser-plasma interaction combines ideal features for femtosecond XAS. It has been used to investigate the non-equilibrium transition of a copper sample brought at extreme conditions of temperature and pressure by a femtosecond laser pulse. We measured a rise time of the electron temperature below 100 fs. This first experiment demonstrates the great potential of the betatron source and paves the way to a new class of ultrafast experiments.
We present an emph{Effective Static Approximation} (ESA) to the local field correction (LFC) of the electron gas that enables highly accurate calculations of electronic properties like the dynamic structure factor $S(q,omega)$, the static structure factor $S(q)$, and the interaction energy $v$. The ESA combines the recent neural-net representation [textit{J. Chem. Phys.} textbf{151}, 194104 (2019)] of the temperature dependent LFC in the exact static limit with a consistent large wave-number limit obtained from Quantum Monte-Carlo data of the on-top pair distribution function $g(0)$. It is suited for a straightforward integration into existing codes. We demonstrate the importance of the LFC for practical applications by re-evaluating the results of the recent {X-ray Thomson scattering experiment on aluminum} by Sperling textit{et al.}~[textit{Phys. Rev. Lett.} textbf{115}, 115001 (2015)]. We find that an accurate incorporation of electronic correlations {in terms of the ESA} leads to a different prediction of the inelastic scattering spectrum than obtained from state-of-the-art models like the Mermin approach or linear-response time-dependent density functional theory. Furthermore, the ESA scheme is particularly relevant for the development of advanced exchange-correlation functionals in density functional theory.
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