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Register a new userBiomineral Amorphous Lasers through Light-Scattering Surfaces Assembled by Electrospun Fiber Templates
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Authors
Maria Moffa
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New materials aim at exploiting the great control of living organisms over molecular architectures and minerals. Optical biomimetics has been widely developed by microengineering, leading to photonic components with order resembling those found in plants and animals. These systems, however, are realized by complicated and adverse processes. Here we show how biomineralization might enable the one-step generation of components for amorphous photonics, in which light is made to travel through disordered scattering systems, and particularly of active devices such as random lasers, by using electrospun fiber templates. The amount of bio-enzymatically produced silica is related to light-scattering capacity and the resulting organosilica surfaces exhibit a transport mean free path for light as low as 3 micron, and lasing with linewidth below 0.2 nm. The resulting, complex optical material is characterized and modelled to elucidate scattered fields and lasing performance. Tightly-controlled nanofabrication of direct biological inspiration establishes a new concept for the additive manufacturing of engineered light-diffusing materials and photonic components, not addressed by existing technologies.
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Complex assemblies of light-emitting polymer nanofibers with molecular materials exhibiting optical gain can lead to important advance to amorphous photonics and to random laser science and devices. In disordered mats of nanofibers, multiple scattering and waveguiding might interplay to determine localization or spreading of optical modes as well as correlation effects. Here we study electrospun fibers embedding a lasing fluorene-carbazole-fluorene molecule and doped with titania nanoparticles, which exhibit random lasing with sub-nm spectral width and threshold of about 9 mJ cm^-2 for the absorbed excitation fluence. We focus on the spatial and spectral behavior of optical modes in the disordered and non-woven networks, finding evidence for the presence of modes with very large spatial extent, up to the 100 micrometer-scale. These findings suggest emission coupling into integrated nanofiber transmission channels as effective mechanism for enhancing spectral selectivity in random lasers and correlations of light modes in the complex and disordered material.
Solitons, as stable localized wave packets that can propagate long distance in dispersive media without changing their shapes, are ubiquitous in nonlinear physical systems. Since the first experimental realization of optical bright solitons in the anomalous dispersion single mode fibers (SMF) by Mollenauer et al. in 1980 and optical dark solitons in the normal dispersion SMFs by P. Emplit et al. in 1987, optical solitons in SMFs had been extensively investigated. In reality a SMF always supports two orthogonal polarization modes. Taking fiber birefringence into account, it was later theoretically predicted that various types of vector solitons, including the bright-bright vector solitons, dark-dark vector solitons and dark-bright vector solitons, could be formed in SMFs. However, except the bright-bright type of vector solitons, other types of vector solitons are so far lack of clear experimental evidence. Optical solitons have been observed not only in the SMFs but also in mode locked fiber lasers. It has been shown that the passively mode-locked erbium-doped fiber lasers offer a promising experimental platform for studying the scalar optical solitons. Vector solitons can also be formed in mode locked fiber lasers. In this dissertation, the author presents results of a series of theoretical and experimental investigations on the vector solitons in fiber lasers.
We report on a comprehensive study of the unique adhesive properties of mats of polymethylmethacrylate (PMMA) nanofibers produced by electrospinning. Fibers are deposited on glass, varying the diameter and the relative orientation of the polymer filaments (random vs aligned configuration). While no significant variation is observed in the static contact angle (about 130{deg}) of deposited water drops upon changing the average fiber diameter up to the micrometer scale, fibers are found to exhibit unequalled water adhesion. Placed vertically, they can hold up water drops as large as 60 microL, more than twice the values typically obtained with hairy surfaces prepared by different methods. For aligned fibers with anisotropic wetting behavior, the maximum volume measured in the direction perpendicular to the fibers goes up to 90 {mu}L. This work suggests new routes to tailor the wetting behavior on extended areas by nanofiber coatings, with possible applications in adsorbing and catalytic surfaces, microfluidic devices, and filtration technologies.
A laser is based on the electromagnetic modes of its resonator, which provides the feedback required for oscillation. Enormous progress has been made in controlling the interactions of longitudinal modes in lasers with a single transverse mode. For example, the field of ultrafast science has been built on lasers that lock many longitudinal modes together to form ultrashort light pulses. However, coherent superposition of many longitudinal and transverse modes in a laser has received little attention. The multitude of disparate frequency spacings, strong dispersions, and complex nonlinear interactions among modes greatly favor decoherence over the emergence of order. Here we report the locking of multiple transverse and longitudinal modes in fiber lasers to generate ultrafast spatiotemporal pulses. We construct multimode fiber cavities using graded-index multimode fiber (GRIN MMF). This causes spatial and longitudinal mode dispersions to be comparable. These dispersions are counteracted by strong intracavity spatial and spectral filtering. Under these conditions, we achieve spatiotemporal, or multimode (MM), mode-locking. A variety of other multimode nonlinear dynamical processes can also be observed. Multimode fiber lasers thus open new directions in studies of three-dimensional nonlinear wave propagation. Lasers that generate controllable spatiotemporal fields, with orders-of-magnitude increases in peak power over existing designs, should be possible. These should increase laser utility in many established applications and facilitate new ones.
The phase information provided by the beat note between frequency combs and two continuous-wave lasers is used to extrapolate the phase evolution of comb modes found in a spectral region obtained via nonlinear broadening. This thereafter enables using interferogram self-correction to fully retrieve the coherence of a dual-comb beat note between two independent fiber lasers. This approach allows to forego the $f - 2f$ self-referencing of both combs, which is a significant simplification. Broadband near-infrared methane spectroscopy has been conducted as a demonstration of the simplified systems preserved performance.
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