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Register a new userDissipation induced dipole blockade and anti-blockade in driven Rydberg systems
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We study theoretically and experimentally the competing blockade and anti-blockade effects induced by spontaneously generated contaminant Rydberg atoms in driven Rydberg systems. These contaminant atoms provide a source of strong dipole-dipole interactions and play a crucial role in the systems behavior. We study this problem theoretically using two different approaches. The first is a cumulant expansion approximation, in which we ignore third-order and higher connected correlations. Using this approach for the case of resonant drive, a many-body blockade radius picture arises, and we find qualitative agreement with previous experimental results. We further predict that as the atomic density is increased, the Rydberg populations dependence on Rabi frequency will transition from quadratic to linear dependence at lower Rabi frequencies. We study this behavior experimentally by observing this crossover at two different atomic densities. We confirm that the larger density system has a smaller crossover Rabi frequency than the smaller density system. The second theoretical approach is a set of phenomenological inhomogeneous rate equations. We compare the results of our rate equation model to the experimental observations in [E. A. Goldschmidt, et al., PRL 116, 113001 (2016)] and find that these rate equations provide quantitatively good scaling behavior of the steady-state Rydberg population for both resonant and off-resonant drive.
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The resonant dipole-dipole interaction between highly excited Rydberg levels dominates the interaction of neutral atoms at short distances scaling as $1/r^3$. Here we take advantage of the combined effects of strong dipole-dipole interaction and multifrequency driving fields to propose one type of selective Rydberg pumping mechanism. In the computational basis of two atoms ${|00rangle, |01rangle,|10rangle,|11rangle}$, this mechanism allows $|11rangle$ to be resonantly pumped upwards to the single-excited Rydberg states while the transitions of the other three states are suppressed. From the perspective of mathematical form, we achieve an analogous F{o}ster resonance for ground states of neutral atoms. The performance of this selective Rydberg pumping is evaluated using the definition of fidelity for controlled-$Z$ gate, which manifests a characteristic of robustness to deviation of interatomic distance, fluctuation of F{o}ster resonance defect, and spontaneous emission of double-excited Rydberg states. As applications of this mechanism, we discuss in detail the preparation of the maximally entangled symmetric state for two atoms via ground-state blockade, and the maximally entangled antisymmetric state via engineered spontaneous emission, within the state-of-the-art experiments, respectively.
We present a combined experimental and theoretical study of the effects of Rydberg interactions on Autler-Townes spectra of ultracold gases of atomic strontium. Realizing two-photon Rydberg excitation via a long-lived triplet state allows us to probe the thus far unexplored regime where Rydberg state decay presents the dominant decoherence mechanism. The effects of Rydberg interactions are observed in shifts, asymmetries, and broadening of the measured atom-loss spectra. The experiment is analyzed within a one-body density matrix approach, accounting for interaction-induced level shifts and dephasing through nonlinear terms that approximately incorporate correlations due to the Rydberg blockade. This description yields good agreement with our experimental observations for short excitation times. For longer excitation times, the loss spectrum is altered qualitatively, suggesting additional dephasing mechanisms beyond the standard blockade mechanism based on pure van der Waals interactions.
We perform a comprehensive investigation of the coupling between a Rydberg-dressed atomic gas and an ultra-cold plasma. Using simultaneous time-resolved measurements of both neutral atoms and ions, we show that plasma formation occurs via a Coulomb anti-blockade mechanism, in which background ions DC Stark shift nearby atoms into resonance at specific distances. The result is a highly correlated growth of the Rydberg population that shares some similarities with that previously observed for van der Waals interactions. We show that a rate equation model that couples the laser-driven Rydberg gas to the ultra-cold plasma via a Coulomb anti-blockade mechanism accurately reproduces both the plasma formation and its subsequent decay. Using long-lived high angular momentum states as a probe, we also find evidence of a crossover from Coulomb anti-blockade to Coulomb blockade at high density. As well as shedding light on loss mechanisms in Rydberg-dressed gases, our results open new ways to create low-entropy states in ultra-cold plasmas.
We report on the local control of the transition frequency of a spin-$1/2$ encoded in two Rydberg levels of an individual atom by applying a state-selective light shift using an addressing beam. With this tool, we first study the spectrum of an elementary system of two spins, tuning it from a non-resonant to a resonant regime, where bright (superradiant) and dark (subradiant) states emerge. We observe the collective enhancement of the microwave coupling to the bright state. We then show that after preparing an initial single spin excitation and letting it hop due to the spin-exchange interaction, we can freeze the dynamics at will with the addressing laser, while preserving the coherence of the system. In the context of quantum simulation, this scheme opens exciting prospects for engineering inhomogeneous XY spin Hamiltonians or preparing spin-imbalanced initial states.
The dipole blockade phenomenon is a direct consequence of strong dipole-dipole interaction, where only single atom can be excited because the doubly excited state is shifted out of resonance. The corresponding two-body entanglement with non-zero concurrence induced by the dipole blockade effect is an important resource for quantum information processing. Here, we propose a novel physical mechanism for realizing dipole blockade without the dipole-dipole interaction, where two qubits coupled to a cavity, are driven by a coherent field. By suitably chosen placements of the qubits in the cavity and by adjusting the relative decay strengths of the qubits and cavity field, we kill many unwanted excitation pathways. This leads to dipole blockade. In addition, we show that these two qubits are strongly entangled over a broad regime of the system parameters. We show that a strong signature of this dipole blockade is the bunching property of the cavity photons which thus provides a possible measurement of the dipole blockade. We present dynamical features of the dipole blockade without dipole-dipole interaction. The proposal presented in this work can be realized not only in traditional cavity QED, but also in non-cavity topological photonics involving edge modes.
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