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Register a new userThe First Measurement of the $2^{3}S_{1} rightarrow 3^{3}P - 2^{3}P$ Tune-Out Wavelength in He*
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B. M. Henson
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The workhorse of atomic physics, quantum electrodynamics, is one of the best-tested theories in physics. However recent discrepancies have shed doubt on its accuracy for complex atomic systems. To facilitate the development of the theory further we aim to measure transition dipole matrix elements of metastable helium (He*) (the ideal 3 body test-bed) to the highest accuracy thus far. We have undertaken a measurement of the `tune-out wavelength which occurs when the contributions to the dynamic polarizability from all atomic transitions sum to zero; thus illuminating an atom with this wavelength of light then produces no net energy shift. This provides a strict constraint on the transition dipole matrix elements without the complication and inaccuracy of other methods. Using a novel atom-laser based technique we have made the first measurement of the tune-out wavelength in metastable helium between the $3^{3}P_{1,2,3}$ and $2^{3}P_{1,2,3}$ states at 413.07(2) nm which compares well with the predicted valuecite{Mitroy2013} of 413.02(9) nm. We have additionally developed many of the methods necessary to improve this measurement to the 100 fm level of accuracy where it will form the most accurate determination of transition rate information ever made in He* and provide a stringent test for atomic QED simulations. We believe this measurement to be one of the most sensitive ever made of an optical dipole potential, able to detect changes in potentials of $sim$200 pK and is widely applicable to other species and areas of atom optics.
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Despite quantum electrodynamics (QED) being one of the most stringently tested theories underpinning modern physics, recent precision atomic spectroscopy measurements have uncovered several small discrepancies between experiment and theory. One particularly powerful experimental observable that tests QED independently of traditional energy level measurements is the `tune-out frequency, where the dynamic polarizability vanishes and the atom does not interact with applied laser light. In this work, we measure the `tune-out frequency for the $2^{3!}S_1$ state of helium between transitions to the $2^{3!}P$ and $3^{3!}P$ manifolds and compare it to new theoretical QED calculations. The experimentally determined value of $725,736,700,$$(40_{mathrm{stat}},260_{mathrm{syst}})$ MHz is within ${sim} 2.5sigma$ of theory ($725,736,053(9)$ MHz), and importantly resolves both the QED contributions (${sim} 30 sigma$) and novel retardation (${sim} 2 sigma$) corrections.
Two anomalously weak transitions within the $2 ^3{rm S}_1~-~3 ^3{rm P}_J$ manifolds in $^3$He have been identified. Their transition strengths are measured to be 1,000 times weaker than that of the strongest transition in the same group. This dramatic suppression of transition strengths is due to the dominance of the hyperfine interaction over the fine structure interaction. An alternative selection rule based on textit{IS}-coupling (where the nuclear spin is first coupled to the total electron spin) is proposed. This provides qualitative understanding of the transition strengths. It is shown that the small deviations from the textit{IS}-coupling model are fully accounted for by an exact diagonalization of the strongly interacting states.
We present the detection of the highly forbidden $2^{3!}S_1 rightarrow 3^{3!}S_1$ atomic transition in helium, the weakest transition observed in any neutral atom. Our measurements of the transition frequency, upper state lifetime, and transition strength agree well with published theoretical values, and can lead to tests of both QED contributions and different QED frameworks. To measure such a weak transition, we developed two methods using ultracold metastable ($2^{3!}S_1$) helium atoms: low background direct detection of excited then decayed atoms for sensitive measurement of the transition frequency and lifetime; and a pulsed atom laser heating measurement for determining the transition strength. These methods could possibly be applied to other atoms, providing new tools in the search for ultra-weak transitions and precision metrology.
Ab initio calculations of QED radiative corrections to the $^2P_{1/2}$ - $^2P_{3/2}$ fine-structure transition energy are performed for selected F-like ions. These calculations are nonperturbative in $alpha Z$ and include all first-order and many-electron second-order effects in $alpha$. When compared to approximate QED computations, a notable discrepancy is found especially for F-like uranium for which the predicted self-energy contributions even differ in sign. Moreover, all deviations between theory and experiment for the $^2P_{1/2}$ - $^2P_{3/2}$ fine-structure energies of F-like ions, reported recently by Li et al., Phys. Rev. A 98, 020502(R) (2018), are resolved if their highly accurate, non-QED fine-structure values are combined with the QED corrections ab initially evaluated here.
We realize an experimental facility for cooling and trapping strontium (Sr) atoms and measure the Lande g factor of $^{3}$D$_{1}$ of $^{88}$Sr. Thanks to a novel repumping scheme with the $^{3}$P$_{2}$$rightarrow$$^{3}$S$_{1}$ and $^{3}$P$_{0}$$rightarrow$$^{3}$D$_{1}$ combination and the permanent magnets based self-assembled Zeeman slower, the peak atom number in the continuously repumped blue MOT is enhanced by a factor of 15 with respect to the non-repumping case, and reaches $sim$1 billion. Furthermore, using the resolved-sideband Zeeman spectroscopy, the Lande g factor of $^{3}$D$_{1}$ is measured to be 0.4995(88) showing a good agreement with the theoretical value of 0.4988. The results will have an impact on various applications including atom laser, dipolar interactions, quantum information and precision measurements.
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