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Register a new userTransport properties of ultrathin YBa$_2$Cu$_3$O$_{7-delta}$ nanowires: a route to single photon detection
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We report on the growth and characterization of ultrathin YBa$_2$Cu$_3$O$_{7-delta}$ (YBCO) films on MgO (110) substrates, which exhibit superconducting properties at thicknesses down to 3 nm. YBCO nanowires, with thicknesses down to 10 nm and widths down to 65 nm, have been also successfully fabricated. The nanowires protected by a Au capping layer show superconducting properties close to the as-grown films, and critical current densities, which are only limited by vortex dynamics. The 10 nm thick YBCO nanowires without the Au capping present hysteretic current voltage characteristics, characterized by a voltage switch which drives the nanowires directly from the superconducting to the normal state. Such bistability is associated in NbN nanowires to the presence of localized normal domains within the superconductor. The presence of the voltage switch, in ultrathin nanostructures characterized by high sheet resistance values, though preserving high quality superconducting properties, make our nanowires very attractive devices to engineer single photon detectors.
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We use electromigration (EM) to tune the oxygen content of YBa$_2$Cu$_3$O$_{7-delta}$ nanowires. During EM, the dopant oxygen atoms in the nanowire are displaced under the combined effect of electrostatic force and Joule heating. The EM current can be tuned to either deplete or replenish nanowire with oxygen, allowing fine tuning of its doping level. Transport measurements show that the quality of the nanowires is not influenced by the EM process. Kelvin probe force microscopy (KPFM) is used to image the electric properties of the nanowire at the nanoscale. This technique confirms the good homogeneity of the doping along the nanowires. Thus, EM provides an effective method to reproduce a large portion of the phase diagram on nanoscale.
We present the fabrication and electrical transport characterization of underdoped YBa$_2$Cu$_3$O$_{7-{delta}}$ nanowires. The nanowires have been realized without any protective capping layer and they show transport properties similar to those of the parent thin film, demonstrating that they have not been damaged by the nanopatterning. The current-voltage characteristics of the underdoped nanowires show large hysteretic voltage switching at the critical current, in contrast to the flux-flow like characteristics of optimally doped nanostructures, indicating the formation of a self-stabilizing hot spot. These results open up new possibilities of using the underdoped nanowires for single photon detection and for exploring the underdoped side of the YBa$_2$Cu$_3$O$_{7-{delta}}$ phase diagram at the nanoscale.
Superconductivity of YBa$_2$Cu$_3$O$_{7-delta}$ single crystals was investigated in small magnetic fields. In magnetic measurements the superconducting transition for $textbf{H} | c$ appears 0.4 K higher than for $textbf{H} bot c$. In this temperature range superconductivity is two-dimensional and the total thickness of superconducting layers is about 0.83 of the sample thickness, which is a consequence of the occurrence of the quasi-insulating plane in the unit cell of the crystal structure. Resistivity in the textit{ab}-plane and along the textit{c}-axis was measured simultaneously. In these measurements two-dimensional superconductivity was observed in a temperature range of 0.6-0.8 K with the clear signs of the Berezinskii-Kosterlitz-Touless (BKT) transition which occurs approximately 0.15 K below $T_c$, the mean-field transition temperature.
Most measurements of critical current densities in YBa$_2$Cu$_3$O$_{7-delta}$ thin films to date have been performed on films where the textit{c}-axis is grown normal to the film surface. With such films, the analysis of the dependence of $j_c$ on the magnetic field angle is complex. The effects of extrinsic contributions to the angular field dependence of $j_c$, such as the measurement geometry and disposition of pinning centres, are convoluted with those intrinsically due to the anisotropy of the material. As a consequence of this, it is difficult to distinguish between proposed FLL structure models on the basis of angular critical current density measurements on textit{c}-axis films. Films grown on mis-cut (vicinal) substrates have a reduced measurement symmetry and thus provide a greater insight into the critical current anisotropy. In this paper previous descriptions of the magnetic field angle dependence of $j_c$ in YBa$_2$Cu$_3$O$_{7-delta}$ are reviewed. Measurements on YBa$_2$Cu$_3$O$_{7-delta}$ thin films grown on a range of vicinal substrates are presented and the results interpreted in terms of the structure and dimensionality of the FLL in YBa$_2$Cu$_3$O$_{7-delta}$. There is strong evidence for a transition in the structure of the flux line lattice depending on magnetic field magnitude, orientation and temperature. As a consequence, a simple scaling law can not, by itself, describe the observed critical current anisotropy in YBa$_2$Cu$_3$O$_{7-delta}$. The experimentally obtained $j_c(theta)$ behaviour of YBCO is successfully described in terms of a kinked vortex structure for fields applied near parallel to the textit{a-b} planes.
We have studied the normal-to-superconducting phase transition in optimally-doped YBa$_2$Cu$_3$O$_{7-delta}$ in zero external magnetic field using a variety of different samples and techniques. Using DC transport measurements, we find that the dynamical critical exponent $z=1.54pm0.14$, and the static critical exponent $ u=0.66pm0.10$ for both films (when finite-thickness effects are included in the data analysis) and single crystals (where finite-thickness effects are unimportant). We also measured thin films at different microwave frequencies and at different powers, which allowed us to systematically probe different length scales to avoid finite-thickness effects. DC transport measurements were also performed on the films used in the microwave experiments to provide a further consistency check. These microwave and DC measurements yielded a value of z consistent with the other results, $z=1.55pm0.15$. The neglect of finite-thickness, finite-current, and finite-frequency effects may account for the wide ranges of values for $ u$ and $z$ previously reported in the literature.
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