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Register a new userThe Molecular Chemistry of Diffuse and Translucent Clouds in the Line-of-Sight to Sgr B2
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The 1-50 GHz GBT PRIMOS data contains ~50 molecular absorption lines observed in diffuse and translucent clouds located in the Galactic Center, Bar, and spiral arms in the line-of-sight to Sgr B2(N). We measure the column densities and estimate abundances, relative to H2, of 11 molecules and additional isotopologues. We use absorption by optically thin transitions of c-C3H2 to estimate the N(H2), and argue that this method is preferable to more commonly used methods. We discuss the kinematic structure and abundance patterns of small molecules including the sulfur-bearing species CS, SO, CCS, H2CS, and HCS+; oxygen-bearing molecules OH, SiO, and H2CO; and simple hydrocarbon molecules c-C3H2, l-C3H, and l-C3H+. We discuss the implications of the observed chemistry for the structure of the gas and dust in the ISM. Highlighted results include the following. First, whereas gas in the disk has a molecular hydrogen fraction of 0.65, clouds on the outer edge of the Galactic Bar and in or near the Galactic Center have molecular fractions of 0.85 and >0.9, respectively. Second, we observe trends in isotope ratios with Galactocentric distance; while carbon and silicon show enhancement of the rare isotopes at low Galactocentric distances, sulfur exhibits no trend with Galactocentric distance; the ratio of c-C3H2/c-H13CCCH provides a good estimate of the 12C:13C ratio, whereas H2CO/H2^13CO exhibits fractionation. Third, we report the presence of l-C3H+ in diffuse clouds for the first time. Finally, we suggest that CS has an enhanced abundance within higher density clumps of material in the disk, and therefore may be diagnostic of cloud conditions. If this holds, the diffuse clouds in the Galactic disk contain multiple embedded hyperdensities in a clumpy structure, and the density profile is not a simple function of A_V.
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The diffuse and translucent molecular clouds traced in absorption along the line of sight to strong background sources have so far been investigated mainly in the spectral domain because of limited angular resolution or small sizes of the background sources. We aim to resolve and investigate the spatial structure of molecular clouds traced by several molecules detected in absorption along the line of sight to SgrB2(N). We have used spectral line data from the EMoCA survey performed with ALMA, taking advantage of the high sensitivity and angular resolution. We identify, on the basis of the spectral analysis of c-C3H2 across the field of view, 15 main velocity components along the line of sight to SgrB2(N) and several components in the envelope of SgrB2. The c-C3H2 column densities reveal two categories of clouds. Clouds in Category I (3 kpc arm, 4 kpc arm, and some GC clouds) have smaller c-C3H2 column densities, smaller linewidths, and smaller widths of their column density PDFs than clouds in Category II (Scutum arm, Sgr arm, and other GC clouds). To investigate the spatial structure we derive opacity maps for the following molecules: c-C3H2, H13CO+, 13CO, HNC, HN13C, HC15N, CS, C34S, 13CS, SiO, SO, and CH3OH. These maps reveal that most molecules trace relatively homogeneous structures that are more extended than the field of view defined by the background continuum emission (about 15, that is 0.08-0.6pc depending on the distance). SO and SiO show more complex structures with smaller clumps of size ~5-8. Our analysis suggests that the driving of the turbulence is mainly solenoidal in the investigated clouds. On the basis of HCO+, we conclude that most line-of-sight clouds towards SgrB2 are translucent, including all clouds where complex organic molecules were recently detected. We also conclude that CCH and CH are good probes of H2 in both diffuse and translucent clouds.
Context. Insight into the conditions that drive the physics and chemistry in interstellar clouds is gained from determining the abundance and charge state of their components. Aims. We propose an evaluation of the C60:C60+ ratio in diffuse and translucent interstellar clouds that exploits electronic absorption bands so as not to rely on ambiguous IR emission measurements. Methods. The ratio is determined by analyzing archival spectra and literature data. Information on the cation population is obtained from published characteristics of the main diffuse interstellar bands attributed to C60+ and absorption cross sections already reported for the vibronic bands of the cation. The population of neutral molecules is described in terms of upper limit because the relevant vibronic bands of C60 are not brought out by observations. We revise the oscillator strengths reported for C60 and measure the spectrum of the molecule isolated in Ne ice to complete them. Results. We scale down the oscillator strengths for absorption bands of C60 and find an upper limit of approximately 1.3 for the C60:C60+ ratio. Conclusions. We conclude that the fraction of neutral molecules in the buckminsterfullerene population of diffuse and translucent interstellar clouds may be notable despite the non-detection of the expected vibronic bands. More certainty will require improved laboratory data and observations.
We present a general parameter study, in which the abundance of interstellar argonium (ArH$^+$) is predicted using a model for the physics and chemistry of diffuse interstellar gas clouds. Results have been obtained as a function of UV radiation field, cosmic-ray ionization rate, and cloud extinction. No single set of cloud parameters provides an acceptable fit to the typical ArH$^+$, OH$^+$ and $rm H_2O^+$ abundances observed in diffuse clouds within the Galactic disk. Instead, the observed abundances suggest that ArH$^+$ resides primarily in a separate population of small clouds of total visual extinction of at most 0.02 mag per cloud, within which the column-averaged molecular fraction is in the range $10^{-5} - 10^{-2}$, while OH$^+$ and $rm H_2O^+$ reside primarily in somewhat larger clouds with a column-averaged molecular fraction $sim 0.2$. This analysis confirms our previous suggestion that the argonium molecular ion is a unique tracer of almost purely atomic gas.
One of the surprises of the Herschel mission was the detection of ArH+ towards the Crab Nebula in emission and in absorption towards strong Galactic background sources. Although these detections were limited to the first quadrant of the Galaxy, the existing data suggest that ArH+ ubiquitously and exclusively probes the diffuse atomic regions of the ISM. In this study, we extend the coverage of ArH+ to other parts of the Galaxy with new observations of its J = 1-0 transition along seven Galactic sight lines towards bright sub-mm continuum sources. We aim to benchmark its efficiency as a tracer of purely atomic gas by evaluating its correlation (or lack there of) with other well-known atomic and molecular gas tracers. The observations of ArH+ near 617.5 GHz were made feasible with the new, sensitive SEPIA660 receiver on the APEX 12 m telescope. The two sidebands of this receiver allowed us to observe p-H2O+ transitions of at 607.227 GHz simultaneously with the ArH+ line. By analysing the steady state chemistry of OH+ and o-H2O+, we derive on average a cosmic-ray ionisation rate (CRIR), of 2.3e-16 s^-1 towards the sight lines studied in this work. Using the derived values of the CRIR and the observed ArH+ abundances we constrain the molecular fraction of the gas traced by ArH+ to lie below 2e-2 with a median value of 8.8e-4. Combined, our observations of ArH+, OH+, H2O+, and CH probe different regimes of the ISM, from diffuse atomic to diffuse and translucent molecular clouds. Over Galactic scales, we see that the distribution of N(ArH+) is associated with that of N(H), particularly in the inner Galaxy with potentially even contributions from the warm neutral medium phase of atomic gas at larger galactocentric distances. We derive an average o/p-ratio for H2O+ of 2.1, which corresponds to a nuclear spin temperature of 41 K, consistent with the typical gas temperatures of diffuse clouds.
Recent submillimeter and far-infrared wavelength observations of absorption in the rotational ground-state lines of various simple molecules against distant Galactic continuum sources have opened the possibility of studying the chemistry of diffuse molecular clouds throughout the Milky Way. In order to calculate abundances, the column densities of molecular and atomic hydrogen, HI, must be known. We aim at determining the atomic hydrogen column densities for diffuse clouds located on the sight lines toward a sample of prominent high-mass star-forming regions that were intensely studied with the HIFI instrument onboard Herschel. Based on Jansky Very Large Array data, we employ the 21 cm HI absorption-line technique to construct profiles of the HI opacity versus radial velocity toward our target sources. These profiles are combined with lower resolution archival data of extended HI emission to calculate the HI column densities of the individual clouds along the sight lines. We employ Bayesian inference to estimate the uncertainties of the derived quantities. Our study delivers reliable estimates of the atomic hydrogen column density for a large number of diffuse molecular clouds at various Galactocentric distances. Together with column densities of molecular hydrogen derived from its surrogates observed with HIFI, the measurements can be used to characterize the clouds and investigate the dependence of their chemistry on the molecular fraction, for example.
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