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Register a new userNegative Kerr nonlinearity of graphene as seen via chirped-pulse-pumped self-phase modulation
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We experimentally demonstrate a negative Kerr nonlinearity for quasi-undoped graphene. Hereto, we introduce the method of chirped-pulse-pumped self-phase modulation and apply it to graphene-covered silicon waveguides at telecom wavelengths. The extracted Kerr-nonlinear index for graphene equals n2,gr = -10^(-13) m^2/W. Whereas the sign of n2,gr turns out to be negative in contrast to what has been assumed so far, its magnitude is in correspondence with that observed in earlier experiments. Graphenes negative Kerr nonlinearity strongly impacts how graphene should be exploited for enhancing the nonlinear response of photonic (integrated) devices exhibiting a positive nonlinearity. It also opens up the possibility of using graphene to annihilate unwanted nonlinear effects in such devices, to develop unexplored approaches for establishing Kerr processes, and to extend the scope of the periodic poling method often used for second-order nonlinearities towards third-order Kerr processes. Because of the generic nature of the chirped-pulse-pumped self-phase modulation method, it will allow fully characterizing the Kerr nonlinearity of essentially any novel (2D) material.
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Kerr microresonators driven in the normal dispersion regime typically require the presence of localized dispersion perturbations, such as those induced by avoided mode crossings, to initiate the formation of optical frequency combs. In this work, we experimentally demonstrate that this requirement can be lifted by driving the resonator with a pulsed pump source. We also show that controlling the desynchronization between the pump repetition rate and the cavity free-spectral range (FSR) provides a simple mechanism to tune the center frequency of the output comb. Using a fiber mini-resonator with a radius of only 6 cm we experimentally present spectrally flat combs with a bandwidth of 3 THz whose center frequency can be tuned by more than 2 THz. By driving the cavity at harmonics of its 0.54 GHz FSR, we are able to generate combs with line spacings selectable between 0.54 and 10.8 GHz. The ability to tune both the center frequency and frequency spacing of the output comb highlights the flexibility of this platform. Additionally, we demonstrate that under conditions of large pump-cavity desynchronization, the same cavity also supports a new form of Raman-assisted anomalous dispersion cavity soliton.
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Phase-stabilized 12-fs, 1-nJ pulses from a commercial Ti:sapphire oscillator are directly amplified in a chirped-pulse optical parametric amplifier and recompressed to yield near-transform-limited 17.3-fs pulses. The amplification process is demonstrated to be phase preserving and leads to 85-uJ, carrier-envelope-offset phase-locked pulses at 1 kHz for 0.9 mJ of pump, corresponding to a single-pass gain of 8.5 x 10^4.
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