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Register a new userTricritical wings and modulated magnetic phases in LaCrGe$ _{3}$ under pressure
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Added by
Udhara Kaluarachchi
Publication date
2016
fields
Physics
and research's language is
English
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We determined on the temperature-pressure-magnetic field ($T$-$p$-$H$) phase diagram of the ferromagnet LaCrGe$_3$ from electrical resistivity measurements on single crystals. In ferromagnetic systems, quantum criticality is avoided either by a change of the transition order, becoming of the first order at a tricritical point, or by the appearance of modulated magnetic phases. In the first case, the application of a magnetic field reveals a wing-structure phase diagram as seen in itinerant ferromagnets such as ZrZn$_2$ and UGe$_2$. In the second case, no tricritical wings have been observed so far. Our investigation of LaCrGe$_3$ reveals a double-wing structure indicating strong similarities with ZrZn$_2$ and UGe$_2$. But, unlike these, simpler systems, LaCrGe$_3$ is thought to exhibit a modulated magnetic phase under pressure which already precludes it from a pressure-driven paramagnetic-ferromagnetic quantum phase transition in zero field. As a result, the $T$-$p$-$H$ phase diagram of LaCrGe$_3$ shows both the wing structure as well as the appearance of new magnetic phases, providing the first example of this new possibility for the phase diagram of metallic quantum ferromagnets.
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Magnetism induced by external pressure ($p$) was studied in a FeSe crystal sample by means of muon-spin rotation. The magnetic transition changes from second-order to first-order for pressures exceeding the critical value $p_{{rm c}}simeq2.4-2.5$ GPa. The magnetic ordering temperature ($T_{{rm N}}$) and the value of the magnetic moment per Fe site ($m_{{rm Fe}}$) increase continuously with increasing pressure, reaching $T_{{rm N}}simeq50$~K and $m_{{rm Fe}}simeq0.25$ $mu_{{rm B}}$ at $psimeq2.6$ GPa, respectively. No pronounced features at both $T_{{rm N}}(p)$ and $m_{{rm Fe}}(p)$ are detected at $psimeq p_{{rm c}}$, thus suggesting that the stripe-type magnetic order in FeSe remains unchanged above and below the critical pressure $p_{{rm c}}$. A phenomenological model for the $(p,T)$ phase diagram of FeSe reveals that these observations are consistent with a scenario where the nematic transitions of FeSe at low and high pressures are driven by different mechanisms.
The temperature-pressure phase diagram of the ferromagnet LaCrGe$_3$ is determined for the first time from a combination of magnetization, muon-spin-rotation and electrical resistivity measurements. The ferromagnetic phase is suppressed near $2.1$~GPa, but quantum criticality is avoided by the appearance of a magnetic phase, likely modulated, AFM$_Q$. Our density functional theory total energy calculations suggest a near degeneracy of antiferromagnetic states with small magnetic wave vectors $Q$ allowing for the potential of an ordering wave vector evolving from $Q=0$ to finite $Q$, as expected from the most recent theories on ferromagnetic quantum criticality. Our findings show that LaCrGe$_3$ is a very simple example to study this scenario of avoided ferromagnetic quantum criticality and will inspire further study on this material and other itinerant ferromagnets.
We report the temperature-pressure-magnetic field phase diagram of the ferromagnetic Kondo-lattice CeTiGe$_3$ determined by means of electrical resistivity measurements. Measurements up to $sim$ 5.8 GPa reveal a rich phase diagram with multiple phase transitions. At ambient pressure, CeTiGe$_3$ orders ferromagnetically at $T_text{C}$ = 14 K. Application of pressure suppresses $T_text{C}$, but a pressure induced ferromagnetic quantum criticality is avoided by the appearance of two new successive transitions for $p$ $>$ 4.1 GPa that are probably antiferromagnetic in nature. These two transitions are suppressed under pressure, with the lower temperature phase being fully suppressed above 5.3 GPa. The critical pressures for the presumed quantum phase transitions are $p_1$ $cong$ 4.1 GPa and $p_2$ $cong$ 5.3 GPa. Above 4.1 GPa, application of magnetic field shows a tricritical point evolving into a wing structure phase with a quantum tricritical point at 2.8 T at 5.4 GPa, where the first order antiferromagnetic-ferromagnetic transition changes into the second order antiferromagnetic-ferromagnetic transition.
Building on the growing evidence based on NMR, magnetization, neutron scattering, ESR, and specific heat that, under pressure, SrCu$_2$(BO$_3$)$_2$ has an intermediate phase between the dimer and the Neel phase, we study the competition between two candidate phases in the context of a minimal model that includes two types of intra- and inter-dimer interactions without enlarging the unit cell. We show that the empty plaquette phase of the Shastry-Sutherland model is quickly replaced by a quasi-1D full plaquette phase when intra- and/or inter-dimer couplings take different values, and that this full plaquette phase is in much better agreement with available experimental data than the empty plaquette one.
The charge transfer antiferromagnetic (T$_{N}$ =220 K) insulator EuNiO$_{3}$ undergoes, at ambient pressure, a temperature-induced metal insulator MI transition at T$_{MI}$=463 K. We have investigated the effect of pressure (up to p~20 GPa) on the electronic, magnetic and structural properties of EuNiO$_{3}$ using electrical resistance measurements, ${151}^$Eu nuclear resonance scattering of synchrotron radiation and x-ray diffraction, respectively. With increasing pressure we find at p$_{c}$ =5.8 GPa a transition from the insulating state to a metallic state, while the orthorhombic structure remains unchanged up to 20 GPa. The results are explained in terms of a gradual increase of the electronic bandwidth with increasing pressure, which results in a closing of the charge transfer gap. It is further shown that the pressure-induced metallic state exhibits magnetic order with a lowervalue of T$_{N}$ (T$_{N}$ ~120 K at 9.4 GPa) which disappears between 9.4 and 14.4 GPa.
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