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Spin and Charge Resolved Quantum Gas Microscopy of Antiferromagnetic Order in Hubbard Chains

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 Added by Christian Gross
 Publication date 2016
  fields Physics
and research's language is English




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The repulsive Hubbard Hamiltonian is one of the foundational models describing strongly correlated electrons and is believed to capture essential aspects of high temperature superconductivity. Ultracold fermions in optical lattices allow for the simulation of the Hubbard Hamiltonian with a unique control over kinetic energy, interactions and doping. A great challenge is to reach the required low entropy and to observe antiferromagnetic spin correlations beyond nearest neighbors, for which quantum gas microscopes are ideal. Here we report on the direct, single-site resolved detection of antiferromagnetic correlations extending up to three sites in spin-$1/2$ Hubbard chains, which requires an entropy well below $s^*=ln(2)$. Finally, the simultaneous detection of spin and density opens the route towards the study of the interplay between magnetic ordering and doping in various dimensions.



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Elementary particles such as the electron carry several quantum numbers, for example, charge and spin. However, in an ensemble of strongly interacting particles, the emerging degrees of freedom can fundamentally differ from those of the individual constituents. Paradigmatic examples of this phenomenon are one-dimensional systems described by independent quasiparticles carrying either spin (spinon) or charge (holon). Here we report on the dynamical deconfinement of spin and charge excitations in real space following the removal of a particle in Fermi-Hubbard chains of ultracold atoms. Using space- and time-resolved quantum gas microscopy, we track the evolution of the excitations through their signatures in spin and charge correlations. By evaluating multi-point correlators, we quantify the spatial separation of the excitations in the context of fractionalization into single spinons and holons at finite temperatures.
Quantum gas microscopy has emerged as a powerful new way to probe quantum many-body systems at the microscopic level. However, layered or efficient spin-resolved readout methods have remained scarce as they impose strong demands on the specific atomic species and constrain the simulated lattice geometry and size. Here we present a novel high-fidelity bilayer readout, which can be used for full spin- and density-resolved quantum gas microscopy of two-dimensional systems with arbitrary geometry. Our technique makes use of an initial Stern-Gerlach splitting into adjacent layers of a highly-stable vertical superlattice and subsequent charge pumping to separate the layers by $21,mu$m. This separation enables independent high-resolution images of each layer. We benchmark our method by spin- and density-resolving two-dimensional Fermi-Hubbard systems. Our technique furthermore enables the access to advanced entropy engineering schemes, spectroscopic methods or the realization of tunable bilayer systems.
The attractive Fermi-Hubbard model is the simplest theoretical model for studying pairing and superconductivity of fermions on a lattice. Although its s-wave pairing symmetry excludes it as a microscopic model for high-temperature superconductivity, it exhibits much of the relevant phenomenology, including a short-coherence length at intermediate coupling and a pseudogap regime with anomalous properties. Here we study an experimental realization of this model using a two-dimensional (2D) atomic Fermi gas in an optical lattice. Our site-resolved measurements on the normal state reveal checkerboard charge-density-wave correlations close to half-filling. A hidden SU(2) pseudo-spin symmetry of the Hubbard model at half-filling guarantees superfluid correlations in our system, the first evidence for such correlations in a single-band Hubbard system of ultracold fermions. Compared to the paired atom fraction, we find the charge-density-wave correlations to be a much more sensitive thermometer, useful for optimizing cooling into superfluid phases in future experiments.
Topological phases, like the celebrated Haldane phase in spin-1 chains, defy characterization through local order parameters. Instead, non-local string order parameters can be employed to reveal their hidden order. Similar diluted magnetic correlations appear in doped one-dimensional lattice systems due to the phenomenon of spin-charge separation. Here we report on the direct observation of such hidden magnetic correlations via quantum gas microscopy of hole-doped ultracold Fermi-Hubbard chains. The measurement of non-local spin-density correlation functions reveals a hidden finite-range antiferromagnetic order, a direct consequence of spin-charge separation. Our technique demonstrates how topological order can directly be measured in experiments and it can be extended to higher dimensions to study the complex interplay between magnetic order and density fluctuations.
The Fermi-Hubbard model is one of the key models of condensed matter physics, which holds a potential for explaining the mystery of high-temperature superconductivity. Recent progress in ultracold atoms in optical lattices has paved the way to studying the models phase diagram using the tools of quantum simulation, which emerged as a promising alternative to the numerical calculations plagued by the infamous sign problem. However, the temperatures achieved using elaborate laser cooling protocols so far have been too high to show the appearance of antiferromagnetic and superconducting quantum phases directly. In this work, we demonstrate that using the machinery of dissipative quantum state engineering, one can efficiently prepare antiferromagnetic order in present-day experiments with ultracold fermions. The core of the approach is to add incoherent laser scattering in such a way that the antiferromagnetic state emerges as the dark state of the driven-dissipative dynamics. In order to elucidate the development of the antiferromagnetic order we employ two complementary techniques: Monte Carlo wave function simulations for small systems and a recently proposed variational method for open quantum systems, operating in the thermodynamic limit. The controlled dissipation channels described in this work are straightforward to add to already existing experimental setups.
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