The dynamics of superfluid 4He at and above the Landau quasiparticle regime is investigated by high precision inelastic neutron scattering measurements of the dynamic structure factor. A highly structured response is observed above the familiar phonon-maxon-roton spectrum, characterized by sharp thresholds for phonon-phonon, maxon-roton and roton-roton coupling processes. The experimental dynamic structure factor is compared to the calculation of the same physical quantity by a Dynamic Many-body theory including three-phonon processes self-consistently. The theory is found to provide a quantitative description of the dynamics of the correlated bosons for energies up to about three times that of the Landau quasiparticles.
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