Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userCharge state dynamics of the nitrogen vacancy center in diamond under 1064 nm laser excitation
225
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
The photophysics and charge state dynamics of the nitrogen vacancy (NV) center in diamond has been extensively investigated but is still not fully understood. In contrast to previous work, we find that NV$^{0}$ converts to NV$^{-}$ under excitation with low power near-infrared (1064 nm) light, resulting in $increased$ photoluminescence from the NV$^{-}$ state. We used a combination of spectral and time-resolved photoluminescence experiments and rate-equation modeling to conclude that NV$^{0}$ converts to NV$^{-}$ via absorption of 1064 nm photons from the valence band of diamond. We report fast quenching and recovery of the photoluminescence from $both$ charge states of the NV center under low power 1064 nm laser excitation, which has not been previously observed. We also find, using optically detected magnetic resonance experiments, that the charge transfer process mediated by the 1064 nm laser is spin-dependent.
rate research
Read More
Optical and microwave double resonance techniques are used to obtain the excited state structure of single nitrogen-vacancy centers in diamond. The excited state is an orbital doublet and it is shown that it can be split and associated transition strengths varied by external electric fields and by strain. A group theoretical model is developed. It gives a good account of the observations and contributes to an improved understanding of the electronic structure of the center. The findings are important for quantum information processing and other applications of the center.
Symmetry considerations are used in presenting a model of the electronic structure and the associated dynamics of the nitrogen-vacancy center in diamond. The model accounts for the occurrence of optically induced spin polarization, for the change of emission level with spin polarization and for new measurements of transient emission. The rate constants given are in variance to those reported previously.
Quantum state tomography (QST) is the procedure for reconstructing unknown quantum states from a series of measurements of different observables. Depending on the physical system, different sets of observables have been used for this procedure. In the case of spin-qubits, the most common procedure is to measure the transverse magnetization of the system as a function of time. Here, we present a different scheme that relies on time-independent observables and therefore does not require measurements at different evolution times, thereby greatly reducing the overall measurement time. To recover the full density matrix, we use a set of unitary operations that transform the density operator elements into the directly measurable observable. We demonstrate the performance of this scheme in the electron-nuclear spin system of the nitrogen vacancy center in diamond.
Coherent communication over mesoscale distances is a necessary condition for the application of solid-state spin qubits to scalable quantum information processing. Among other routes under study, one possibility entails the generation of magnetostatic surface spin waves (MSSW) dipolarly coupled to shallow paramagnetic defects in wide-bandgap semiconductors. As an initial step in this direction, here we make use of room-temperature MSSWs to mediate the interaction between the microwave field from an antenna and the spin of a nitrogen-vacancy (NV) center in diamond. We show that this transport spans distances exceeding 3 mm, a manifestation of the MSSW robustness and long diffusion length. Using the NV spin as a local sensor, we find that the MSSW amplitude grows linearly with the applied microwave power, suggesting this approach could be extended to amplify the signal from neighboring spin qubits by several orders of magnitude.
The nitrogen-vacancy (NV) colour centre in diamond is an important physical system for emergent quantum technologies, including quantum metrology, information processing and communications, as well as for various nanotechnologies, such as biological and sub-diffraction limit imaging, and for tests of entanglement in quantum mechanics. Given this array of existing and potential applications and the almost 50 years of NV research, one would expect that the physics of the centre is well understood, however, the study of the NV centre has proved challenging, with many early assertions now believed false and many remaining issues yet to be resolved. This review represents the first time that the key empirical and ab initio results have been extracted from the extensive NV literature and assembled into one consistent picture of the current understanding of the centre. As a result, the key unresolved issues concerning the NV centre are identified and the possible avenues for their resolution are examined.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
